Spent nuclear fuel continues to be generated domestically and abroad, and various studies are actively being conducted for interim dry storage and disposal of spent nuclear fuel. The characteristics vary depending on the type of spent nuclear fuel and the initial specifications, and based on these characteristics, it is essential to estimate the burnup and enrichment of spent nuclear fuel as a nondestructive assay. In particular, it is important to estimate the characteristics of spent nuclear fuel with non-destructive tests because destructive tests cannot be performed on all encapsulated spent nuclear fuel in case of intrusion traces in safeguards. Data is made by measuring spent nuclear fuel directly to evaluate burnup of spent nuclear fuel, but computer simulation research is also important to understand its characteristics because past burnup history is not accurately written, and destructive testing is difficult. In Sweden, the dependency of the burnup history in source strength and mass of light-water reactor-type spent nuclear fuel was evaluated, and this part was also applied to MAGNOX in consideration of the possibility of being used to verify DPRK’s denuclearization. SCALE 6.2 TRITON modeling was performed based on public information on DPRK’s 5 MWe Yongbyon reactor, and the source strength of Nb-95, Zr-95, Ru-106, Cs-134, Cs-137, Ce-141, Ce- 144, Eu-154 nuclides were evaluated. Since the burnup of MAGNOX is lower than that of lightwater reactors, major nuclides in decay heat were not considered. The cooling period was evaluated based on 0, 5, 10, and 20 years. In case the discharge timing was different, the total period of discharge and reloading was the same, and the end-cycle burnup was the same, calculations showed that the source strength emitted from major nuclides was evaluated within 2-3% except for Ru-106 and Ce-144 nuclides. Even the burnup step of nuclear fuel is the same, and the reloaded length after discharge is different, i.e., the cooling period between is different at 5, 10, and 20, the source strength of Nb-95, Zr-95, Ce-144, and Cs-137 was evaluated as an error of 1%. Except for Ru-106 and Ce-144, nuclides are highly dependent on burnup. Compared to the case of light-water reactors, the possibility of a decrease in error needs to be considered later because the specific power is low. As a result, radionuclides in released fuel depend on the effects of burnup, discharged and reloaded period, and a cooling period after release, and research is needed to correct the cooling period within the future burnup history. In addition, in this study, it is necessary to select a scenario -based burnup because the standard burnup due to the statistical treatment of discharged fuels was not considered as conducted in previous studies.

Nuclear inspection is necessary to verify nuclear activities. If North Korea takes denuclearization, North Korea’s nuclear materials should be verified through non-destructive testing and destructive testing for nuclear material production. Since destructive testing of all substances is impossible, nondestructive testing is essential. Most non-destructive tests are performed by measuring the energy of gamma rays, but the characteristics of nuclear fuel can be evaluated by measuring neutron sources when enclosed with thick shields and when shielding structures are difficult to remove. Before the neutron source evaluation of MAGNOX used by North Korea, the relative characteristics will be evaluated later by analyzing the burnup, enrichment, and cooling time of the spent nuclear fuels discharged from the domestic nuclear power plant. This study evaluated the source strength and major nuclides according to burnup for the WH17×17 nuclear fuel assembly. The depletion calculation was conducted using SCALE 6.2 ORIGEN, and 3.5wt% enrichment, 10, 20, 30, 40, 50, 60 MWd/kg burnup, and five years cooling time, the minimum requirement for transport specified in the notice of the Nuclear Safety Commission, was applied. Although the impact assessment on enrichment should be evaluated with MCNP Tally to consider the fission reaction of the generated neutrons, this study only evaluated the spontaneous fission and (a, n) reactions that occurred first because it only evaluates the burnup impact. As burnup increased, neutron generation increased, and most of the total neutron strength occurred through spontaneous fission from the 10 MWd/kg burnup step. The influence of Pu-240 nuclides was dominant in the 10 MWd/kg burnup step but most neutrons were generated in tiny amounts of Cm- 244 generated from 20 MWd/kg burnup. Since DPRK’s 5 MWe Yongbyon MAGNOX has very low burnup (about 0.7 MWd/kg), the primary neutron sources of 10 MWd/kg, Am-241 and Pu isotopes, especially Pu-240, are expected to be used as indicators for evaluating spent nuclear fuel characteristics. If only specific nuclides are evaluated as major neutron sources at lower burnup than those evaluated in this study, in that case, the accuracy of non-destructive testing can be improved. Additionally, the evaluation according to the enrichment and cooling time should be considered as well.

The purpose of this study was to assess an alternative method to characterize indoor environmental factors by multiple indoor and outdoor measurements. Using a mass balance model and regression analysis, penetration factor and source strength factor were calculated using multiple indoor and outdoor measurements. This study was performed in 30 selected apartments in Seoul, Asan, and Daegu area which were constructed within 4 years and over 4 years, to measure the concentration of NO₂ from July, 2004 to September. The results of this study are as follows. The average concentration of NO₂ in Seoul, Asan, and Daegu area in the apartment constructed within 4 years are nitrogen dioxide 48.01㎍/m³ and in the apartment over 4 years are nitrogen dioxide 46.54㎍/m³. Mean ratios of indoor to outdoor NO₂ concentrations are Seoul 0.99, Asan 0.83, Daegu 1.18. The deposition constant and the source strength of NO₂ were 0.97±0.55 hr-1 and 16.33±12.30 ppb/h, respectively. In conclusion, indoor environmental factors were effectively characterized by this method using multiple indoor and outdoor measurements.

This study was performed in 30 selected apartments in Seoul, Asan and Daegu area which were constructed within 4 years and over 4 years, to measure the concentration of VOCs(benzene, toluene, xylene) from July, 2004 to September. Mean ratios of indoor to outdoor VOCs concentrations in the construction under 4 years were higher in 1 than average, I/O ratio of over 4 years were lower in 1. This was considered that the VOCs density influences indoor pollutant. For the indoor air quality estimation, the deposition constant and the source strength factor of toluene were 1.49±2.05 hr-1 and 36.95±52.26 ppb/h, respectively.