In this study, the optimal performance based seismic retrofit method for fiber-reinforced polymer (FRP) jackets in existing reinforced concrete (RC) frames is presented. This optimal method minimizes the amount of FRP material while satisfying the constraints on the maximum inter-story drift, maximum strain of concrete, and shear failure prevention of columns. Both of shear reinforcement for preventing shear failure of columns and flexural reinforcement for improving the flexural capacity of columns are simultaneously considered. This method is applied to 3-story RC frame and the reinforced locations and the numbers of FRP reinforcement plies are obtained.