Recently, the properties of nanostructured materials as advanced engineering materials have received great attention. These properties include fracture toughness and a high degree of hardness. To hinder grain growth during sintering, it is necessary to fabricate nanostructured materials. In this respect, a high-frequency induction-heated sintering method has been presented as an effective technique for making nanostructured materials at a lower temperature in a very short heating period. Nanopowders of W and Al2O3 are synthesized from WO3 and Al powders during high-energy ball milling. Highly dense nanostructured W-Al2O3 composites are made within three minutes by high-frequency induction-heated sintering method and materials are evaluated in terms of hardness, fracture toughness, and microstructure. The hardness and fracture toughness of the composite are 1364 kg/mm2 and 7.1 MPa·m1/2, respectively. Fracture toughness of nanostructured W-Al2O3 is higher than that of monolithic Al2O3. The hardness of this composite is higher than that of monolithic W.