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Effect of Steady-State Oxidation on Tensile Failure of Zircaloy Cladding KCI 등재 SCOPUS

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방사성폐기물학회지 (Journal of the Korean Radioactive Waste Society)
한국방사성폐기물학회 (Korean Radioactive Waste Society)
초록

The effect of oxidation time on the characteristics and mechanical properties of spent nuclear fuel cladding was investigated using Raman spectroscopy, tube rupture test, and tensile test. As oxidation time increased, the Raman peak associated with the tetragonal zirconium oxide phase diminished and merged with the Raman peak associated with the monoclinic zirconium oxide phase near 333 cm−1. Additionally, the other tetragonal zirconium oxide phase peak at 380 cm−1 decreased after 100 d of oxidation, whereas the zirconium monoclinic oxide peak became the dominant peak. The oxidation time had no effect on the tube rupture pressure of the oxidized zirconium alloy tube. However, the yield and tensile stresses of the oxidized nuclear fuel cladding tube decreased after 100 d of oxidation. The results of the scanning electron microscopy and transmission electron microscopy were represented with the in-situ Raman analysis result for the oxide characteristics generated on the cladding of spent nuclear fuel.

목차
1. Introduction
2. Experimental
    2.1 Materials and Specimen Preparation
    2.2 Experimental System
    2.3 Experimental Procedure
3. Results and Discussion
    3.1 Mechanical Tests With Oxidized Tubes
    3.2 In-situ Raman Spectroscopic Analysis forZr-Nb-Sn Alloy
    3.3 Ex-situ Analysis for Zirconium Oxide UsingTEM
    3.4 Relationship Between Zirconium OxidePhase and Mechanical Property
4. Conclusion
Acknowledgements
REFERENCES
저자
  • Taeho Kim(Korea Atomic Energy Research Institute, 111, Daedeok‑daero 989beon‑gil, Yuseong‑gu, Daejeon 34057, Republic of Korea)
  • Kyoung Joon Choi(Korea Railroad Research Institute, 176, Cheoldobangmulgwan-ro, Uiwang-si, Gyeonggi-do 16105, Republic of Korea)
  • Seung Chang Yoo(Ulsan National Institute of Science and Technology, 50, UNIST-gil, Eonyang-eup, Ulju-gun, Ulsan 44919, Republic of Korea)
  • Yunju Lee(Ulsan National Institute of Science and Technology, 50, UNIST-gil, Eonyang-eup, Ulju-gun, Ulsan 44919, Republic of Korea)
  • Ji Hyun Kim(Ulsan National Institute of Science and Technology, 50, UNIST-gil, Eonyang-eup, Ulju-gun, Ulsan 44919, Republic of Korea) Corresponding author