Nuclear weapon generates huge amount of radioactive fallout which is extremely dangerous. The fallout gradually falls to the ground and then covers every surface in city and nature. A hydrogel decontamination medium has been developed to clean the surface polluted by the fallout. The hydrogel is soluble in water so the used hydrogel can be simply removed from the surface by washing. However, significant amount of waste water, containing the radioactive fallout, is generated with this process. In this respect, it is necessary to secure alternative technical options for the used hydrogel recovery. In this study, a steam-suction process was suggested for the used hydrogel recovery. Contaminated stainless steel surface, with fixed simulated fallout particles, was prepared for test. The simulated fallout particles were obtained by high-temperature treatment of a mixture of natural soil, used concrete, and Fe2O3. The hydrogel, composed of poly-vinyl alcohol and borax, was spread onto the contaminated stainless steel surface. The hydrogel was soft at first and it gradually becomes rigid with time. The used hydrogel was recovered by suction with a simultaneous steam spraying to soften the rigid gel. As a result, the clean surface of the stainless steel without the simulated fallout particles was obtained, showing the feasibility of this technique for the used hydrogel recovery.