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Study on the Quench Curve for Low-Level Tritium Measurement Using a Liquid Scintillation Counter KCI 등재 SCOPUS

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방사성폐기물학회지 (Journal of the Korean Radioactive Waste Society)
한국방사성폐기물학회 (Korean Radioactive Waste Society)
초록

The recent release of contaminated water from the Fukushima Daiichi Nuclear Power Plant highlights the need for accurate tritium measurement, particularly near the minimum detectable activity (MDA) of 5 Bq·L−1 set by South Korea’s Nuclear Safety and Security Commission. This study aims to improve low-level tritium measurement accuracy by optimizing the region of interest (ROI) for quench curve determination. These adjustments are crucial for separating tritium signals from background noise. Quench standards were prepared and measured using a liquid scintillation counter (LSC). Three ROIs were analyzed to assess the impact of channel selection on measurement precision: A 20-148 channel range optimized via figure of merit (FOM) analysis, a 20-250 channel range covering tritium’s full beta spectrum, and a broad 1-1024 channel range. Quench curves were obtained by fitting the counting efficiency of each ROI to the quench standards. Tritium samples with six different activity levels were prepared, and their radioactivity was calculated using the quench curves. Selecting appropriate ROIs for quench curve determination is critical for measuring low-concentration tritium accurately. This approach reduces uncertainty and emphasizes reliable methods to improve the precision and consistency of tritium measurements.

목차
1. Introduction
2. Materials and Methods
    2.1 Preparation of Quench Standards
    2.2 Quench Curve
    2.3 Measurement of Tritium Samples
    2.4 Uncertainty
    2.5 Figure of Merit
3. Results and Discussion
    3.1 Optimizing ROI Ranges
    3.2 Determination of the Quench Curve
    3.3 Difference From Massic Activity
4. Conclusion
Conflict of Interest
Acknowledgements
REFERENCES
저자
  • Seongkyeong Cho(University of Science and Technology, 217, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea, Korea Research Institute of Standards and Science, 267, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea)
  • Kyoung Beom Lee(University of Science and Technology, 217, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea, Korea Research Institute of Standards and Science, 267, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea)
  • Jong-Man Lee(University of Science and Technology, 217, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea, Korea Research Institute of Standards and Science, 267, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea) Corresponding author
  • Byoung-Chul Kim(Korea Research Institute of Standards and Science, 267, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea)
  • Yeong Jae Park(Korea Research Institute of Standards and Science, 267, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea)
  • Dong Hye Heo(Korea Research Institute of Standards and Science, 267, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea)
  • Tae Hee Kim(Korea Research Institute of Standards and Science, 267, Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea)
  • Myoung Jung Kim(Korea Atomic Energy Research Institute, 111, Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon 34057, Republic of Korea)