At the late 20th century, many problems surfaced from the environmental destruction, which raised the importance of natural environments; technology and ecology started collaborating, the boundary between architecture and landscape destroyed, and developed into a hybrid-oriented form. This study has focused on the use of green architecture materials as a way to furnish natural expression & mood and dealt with water, plants, trees, sand, rocks, light, wind, mist, cloud and their applications on basic compositional elements such as floor, ceiling, walls, openings and other elements. The discoveries revealed that application of green architecture materials is visible in raw material aspect, architectural forming media aspect, technical aspect, and natural image aspect; furthermore, the use of green architecture materials can make the expression of natural design trend possible. Study of green architecture materials should continue to advance through collaborations and co-studies among interior design, architecture, landscape, and horticulture related design fields for the years to come.