Vortex-induced vibration and instability vibration of tall buildings are very important fluid-structure interaction phenomenon, and many fundamental questions concerning the influence of body movement on the unsteady aerodynamic force remain unanswered. For tall buildings, there are two experimental methods to investigate the characteristics of unsteady aerodynamic forces, one is forced vibration method and the other is free vibration method. In the present paper, a free vibration method was used to investigate the unsteady aerodynamic force on tall building whose aspect ratio is 9 under boundary layer simulating city area. Wind pressures on surfaces and tip displacements were measured simultaneously, and the characteristics of tip displacements and generalized forces were discussed. It was found that variation of across-wind displacements showed different trend between the case when wind speed increases and wind speed decreases, and the fluctuating generalize forces in across-wind direction of vibrating model are larger than that of static model near the resonant wind speed and approach to the static value. And for higher wind speed range, there were two peaks in across-wind power spectra of generalize forces of vibrating model, which means that two frequency components are predominant in unsteady aerodynamic forces.