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Graphene-based derivatives such as graphene oxide(GO) have great potential as membrane material due to their controllable d-spacing, extremely large surface area and tunability of multifunctional groups. GO, highly oxidized graphene, has especially good affinity to CO2 arose from its oxide functional groups(e.g. carboxylic acid, hydroxyl groups) on 2-D nanosheet plane. Here, we synthesized GO/polymer composite materials and fabricated large-area thin film composite(TFC) membrane for CO2 separation using polymeric porous support. Further, we have produced flat-sheet membrane modules with the TFC membranes and tested the performance of the module under CO2/N2 mixed gas and flue gas conditions. The membrane module exhibited high CO2 separation performance as 74% of purity and 22% of recovery under flue gas condition including CO2, O2 and N2.
