Backfill is one of the main components of engineered barrier in a high-level waste repository. The material selection of the backfill determines the barrier performance of the backfill. Overseas, its related research has been carried out mainly in Sweden, Finland, Canada, and Japan. However, Korea has recently started backfill research, and it is urgent to select a potential material for establishing the concept of backfill material and conducting backfill research. This study reviews NEA report, potential materials for overseas backfill research, advantages and disadvantages of single and mixed backfill materials, cases of license applications in Finland and Sweden for the selection of potential materials for backfill in Korea’s high-level waste repository. The review results indicated that it is reasonable to carry out backfill research according to the following plan: Both single and mixed materials are considered as potential materials for backfill research; experiments and performance studies are conducted with these materials; and, based on the results, a potential material or candidate material for the backfill suitable for the HLW repository in Korea is determined. For this plan, the single material is tentatively selected, as in Sweden, as bentonite with a montmorillonite content of about 40-50%. Then, if the selection criteria for montmorillonite content are determined through experiments and performance studies, we determine the final potential backfill material. As for the mixed backfill material, the bentonite/crushed rock mixture seems to be more advantageous than the bentonite/sand mixture considering the disposing problem of crushed rock generated from tunnel excavation and economic feasibility through its recycling. It is thought that the bentonite used in the bentonite/crushed rock mixture should have a higher montmorillonite content than bentonite used as a single backfill material since the crushed rock acts as an inert material in the mixture. The results of this study can be used as basic data for selecting the backfill material to be applied to the high-level waste repository in Korea, and can be used as a guideline for selecting the potential material required for backfill experiments and performance studies to be carried out in the future.