This study aims to prepare bamboo-based activated carbons with surface modifications, focusing on carbon dioxide (CO2) capture in public indoor spaces. The surface of the activated carbon adsorbents was chemically modified through three steps: carbonization, steam activation, and chemical treatment using potassium hydroxide (KOH) and potassium sulfamate (KSO3NH2). The specific surface area and pore volume of the obtained adsorbent (BSAC-KN) were 1,246 m2/g and 0.74 cm3/g, respectively. The surface modification resulted in an adsorption capacity of up to 3.79 mmol-CO2/ g-AC for carbon dioxide. In addition, the expansion of the specific surface area and the enhanced physico-chemical interaction between the weak acidic CO2 molecules and the basic AC surface improved adsorption capacity.