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Estimation of Hydrogen Gas Production Rate According to the Material of the Disposal Canister and the Disposal Environment in the Deep Disposal System

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한국방사성폐기물학회 학술논문요약집 (Abstracts of Proceedings of the Korean Radioactive Wasts Society)
한국방사성폐기물학회 (Korean Radioactive Waste Society)
초록

The International Atomic Energy Agency recommends the deep geological disposal system as one of the disposal methods for high-level radioactive waste (HLW), such as spent nuclear fuel. The deep geological disposal system disposes of HLW in a deep and stable geological formation to isolate the HLW from the human biosphere and restrict the inflow of radionuclides into the ecosystem. It mainly consists of an engineered barrier and a natural barrier. Safety evaluation using a numerical model has been performed primarily to evaluate the buffer’s long-term stability. However, although the gas generation rate input for long-term stability evaluation is the critical factor that has the most significant influence on the long-term hydraulic-mechanical behavior of the buffer, in-depth research and experimental data are lacking. In this study, the gas generation rate on the interface between the disposal canister and the buffer material, a component of the engineered barrier, was mainly studied. Gas can be generated between the disposal canister and the buffer material due to various causes such as anaerobic corrosion of the disposal canister metal, organic matter decomposition, radiation decomposition, and steam generation due to high temperature. The generation of gas in such a disposal environment increases the pore gas pressure in the buffer and causes internal cracks. The occurred cracks increase the intrinsic permeability of the buffer, which leads to a decrease in the primary performance of the buffer. For this reason, it is essential to apply the appropriate gas generation rate according to the disposal condition and buffer material for accurate long-term stability analysis. Therefore, the theoretical models regarding the estimation of gas generation were summarized through a literature study. The amount of gas generated was estimated according to the disposal environment and material of the disposal canister. It is expected that estimated values might be used to estimate the long-term stability analysis of buffer performance according to the disposal condition.

저자
  • Jung-Tae Kim(Korea Atomic Energy Research Institute, 111, Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon)
  • Changsoo Lee(Korea Atomic Energy Research Institute, 111, Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon) Corresponding author
  • Jin-Seop Kim(Korea Atomic Energy Research Institute, 111, Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon)
  • Sinhang Kang(Korea Atomic Energy Research Institute, 111, Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon)