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Characterization of Fine and Ultrafine Particles Generated During the Dismantling of a Mock-up Reactor Pressure Vessel

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한국방사성폐기물학회 학술논문요약집 (Abstracts of Proceedings of the Korean Radioactive Wasts Society)
한국방사성폐기물학회 (Korean Radioactive Waste Society)
초록

Cutting reactor pressure vessels (RPV) into acceptable sizes for waste disposal is a key process in dismantling nuclear power plants. In the case of Kori-1, a remote oxyfuel cutting method has been developed by Doosan Heavy Industry & Construction to dismantle RPVs. Cutting radioactive material, such as RPV, generates a large number of fine and ultrafine particles incorporating radioactive isotopes. To minimize radiological exposure of dismantling workers and workplace surface contamination, understanding the characteristics of radioactive aerosols from the cutting process is crucial. However, there is a paucity of knowledge of the by-products of the cutting process. To overcome the limitations, a mock-up RPV cutting experiment was designed and established to investigate the characteristics of fine and ultrafine particles from the remote cutting process of the RPV at the Nuclear Decommissioning Center of Doosan Heavy Industry & Construction. The aerosol measurement system was composed of a cutting system, purification system, sampling system, and measurement device. The cutting system has a shielding tent and oxyfuel cutting torch and remote cutting robot arm. It was designed to prevent fine particle leakage. The shielding tent acts as a cutting chamber and is connected to the purification system. The purification system operates a pressure difference by generating an airflow which delivers aerosols from the cutting system to the purification system. The sampling system was installed at the center of the pipe which connects the shielding tent and purification system and was carefully designed to achieve isokinetic sampling for unbiased sampling. Sampled aerosols were delivered to the measurement device. A high-resolution electrical low-pressure impactor (HR-ELPI+, Dekati) is used to measure the size distribution of inhalable aerosols (Aerodynamic diameter: 6 nm to 10 μm) and to collect size classified aerosols. In this work, the mock-up reactor vessel was cut 3 times to measure the number distribution of fine and ultrafine particles and mass distribution of iron, chromium, nickel, and manganese. The number distribution of aerosols showed the bi-modal distribution; two peaks were positioned at 0.01−0.02 μm and 0.04–0.07 μm respectively. The mass distribution of metal elements showed bi-modal and trimodal distribution. Such results could be criteria for filter selection to be used in the filtration system for the cutting process and fundamental data for internal dose assessment for accidents. Future work includes the investigations relationships between the characteristics of the generated aerosols and physicochemical properties of metal elements.

저자
  • Wonseok Yang(Korea Advanced Institute of Science and Technology, 291, Daehak-ro, Yuseong-gu, Daejeon)
  • Minho Lee(FNC Technology, 46, Tapsil-ro, Giheung-gu, Yongin-si, Gyeonggi-do)
  • Samuel Park(Seoul National University, 1, Gwanak-ro, Gwanak-gu, Seoul)
  • Nakkyu Chae(Seoul National University, 1, Gwanak-ro, Gwanak-gu, Seoul)
  • HaeWoong Kim(Doosan Enerbility Co., Ltd., 22, Doosan volvo-ro, Seongsan-gu, Changwon-si, Gyeongsangnam-do)
  • Kwangsoo Park(Doosan Enerbility Co., Ltd., 22, Doosan volvo-ro, Seongsan-gu, Changwon-si, Gyeongsangnam-do)
  • Sungyeol Choi(Seoul National University, 1, Gwanak-ro, Gwanak-gu, Seoul) Corresponding author