Among the twenty six nuclear power plants in Korea, twenty four plants are currently in operation excluding the two permanently shut-down Kori #1 and Wolsung #1 plants. The decommissioning process includes many tasks such as cutting, decontamination, disposal and treatment. Among the tasks, because cutting is one of the tasks performed close to the target structure, there is a possibility for the workers to be exposed excessively to the radiation. There are representative large structures such as steam generators, nuclear reactors, reactor coolant pump, and pressurizer, made of metals, and radioactive concrete, made of concrete. Especially, compared to the trend of research to manage the radiation exposure of steam generators that are directly connected to pressurizers, the trend of research to manage the radiation exposure of pressurizers to workers is not satisfactory. Moreover, although there have been many studies on radioactive concrete, the studies to manage the radiation exposure to workers with a systematic cutting scenario are insufficient. In this study, radioactive concrete, a representative large structure made of concrete, was selected as the target for evaluation. The conditions for evaluation were cutting speed (1~10 m2/hr) and the time for cutting (permanent shutdown~30 years after the shutdown). A cutting scenario was developed by applying the situation for abrasive decontamination beforehand and Hot-to-Cold and Cold-to-Hot, and effort was made to derive a reasonable plan. The evaluation result derived were hourly radiation dose distribution of 1.19~0.103 mSv/hour and 1.29~0.0113 mSv/hour for a scenario without abrasive decontamination (in the order of Hot to Cold, Cold to Hot), and hourly radiation dose distribution of 0.547~0.0479 mSv/hour and 0.608~0.0522 mSv/hour for a scenario with abrasive decontamination. The maximum value of collective dose derived was 1.54E+04 mSv at the cutting time of permanent shutdown with cutting speed of 1 m2/hour in the Cold to Hot scenario before abrasive decontamination, and the minimum value derived was 5.15E+01 mSv at the cutting time of 30-year after the permanent shutdown with cutting speed of 10 m2/hour in the Hot to Cold scenario after abrasive decontamination.

When decommissioning and operating nuclear power plants, a lot of radioactive waste in concentrated waste powder, slurry, sludge, and powder is generated. The radioactive waste, non-conformity for disposal, cannot be treated or disposed of, but is currently being stored instead. To dispose of the waste, the waste can be solidified by mixing with an appropriate solidification agent. However, when the solidification agent and powder particles are mixed as in the conventional method, the final volume of the waste form to be disposed of increases. In order to solve this problem, in this study, volume reduction was achieved, compared to the existing powder, by applying the roll compaction technology to mold the radioactive waste into compressed pellets. Soil, concrete, concentrate waste, and contaminated soil powder were used as test materials, and pellets were prepared under different operating conditions. Subsequently, a compressive strength test was performed to confirm the integrity and optimal process conditions of the manufactured pellets. However, in order to perform the compressive strength test, the upper and lower surfaces of the pellets must be horizontal, but the pellet has the shape of two tetrahedrons joined together. Hence, test specimens for measuring compressive strength were prepared by making a surface treatment jig. The compressive strength test showed a high strength of 5.20~28.20 MPa. The process conditions showing high compressive strengths were selected as the optimal process conditions. Finally, the volume reduction ratios were calculated by measuring the weight, density and volume of the manufactured pellets. The degrees of volume reduction of the manufactured pellets compared to the existing powder were checked. When the roll gap was 0 mm, the average reduction ratios of the test materials were 3.7 for the soil, 4.0 for the concrete, 4.6 for the concentrate waste, and 3.8 for the contaminated soil. When roll gap was 1 mm, the ratios were 2.7 for the soil, 2.9 for the concrete, 3.4 for the concentrate waste, and 2.8 for the contaminated soil. Therefore, from a conservative point of view (Roll gap = 1 mm), when powdered waste is formed into pellets, it means that the volume is reduced by 1/2.7 for soil, 1/2.9 for concrete, 1/3.4 for concentrated waste, and 1/2.8 for contaminated soil.

Radioactive materials emitted from nuclear accident or decommissioning cause soil contamination over wide areas. In the event of such a wide area of contaminated soil, decontamination is inevitable for residents to reside and reuse as industrial land. There are many ways to decontaminate these contaminated soils, but in urgent situations, the soil washing, which has a short process period and relatively high decontamination efficiency, is considered the most suitable. However, the soil washing process of removing fine soil and cesium by using washing liquid as water and adding a flocculating agent (J-AF) generates slurry/sludge-type secondary waste (Cs-contaminated soil + flocculating agent). Since this form of sludge contaminants cannot be disposed, solidification is needed using an appropriate solidification agent to treat wastes for disposal. Therefore, this study devised a treatment method of contaminated fine soils occurring after the soil washing process. This investigation prepared the simulated wastes of contaminated fine soils generated after the soil washing, and pelletized the samples using a roll compactor under the optimum operating conditions. The optimum conditions of the device were determined in the pre-test. Roll speed, feeding rate, and hydraulic pressure were 1.5 rpm, 25 rpm, and 28.44 MPa, respectively. The waste forms were manufactured by incorporating created pellets (H 6.5 × W 9.4 mm) using polymers as solidification agents. Used polymers were main ingredient (YD-128), hardener (G-1034), and diluent (LGE). The optimum mixing ratio was YD-128 : G-1034 = 65 : 35 phr, and LGE was added in an amount of 10wt% of the total mixture. To confirm the disposal suitability of the manufactured waste forms, characterization evaluation was carried out (compressive strength, thermal cycling, immersion, and leaching test). Characterization evaluation revealed a minimum compressive strength of 23.1 MPa, far exceeding 3.44 MPa of the disposal facility waste acceptance criteria. Compressive strength increased to the highest value of 31.90 MPa after immersion test. To examine leaching characteristics, the pH, Electrical Conductivity (EC) and leachability index (􀜮􀯜) of leachates were identified. As results, pH and EC consistently increased or remained constant with leaching time. The average of Co, Cs and Sr nuclides was 17.76, 17.38 and 14.04, respectively, exceeding the value of 6 in the waste acceptance criteria. Effective waste treatment/ disposal can be achieved without increasing volumes of sludge/slurry by enhancing the technique of this research by performing additional studies in the future.

처분 부적합 폐기물이란 원전운영이나 해체 시 처리, 고화 및 포장이 요구되는 방사성폐기물 등을 일컬으며, 대표적으로 분산 특성을 갖는 입자성 방사성폐기물을 예로 들 수가 있다. 이들 폐기물에는 원전 운영과정에서 발생되는 농축폐액의 건조 분말, 슬러리 및 슬러지, 향후 원전 해체과정에서 발생되는 온갖 분말 상태의 폐기물(콘크리트 파쇄물, 제염 슬러지 등), 그리고 제염이 용이치 못한 미세 크기의 방사능오염 토양 등이 있다. 입자성 폐기물을 기존의 고화방식으로 처리할 경우에는 최종 폐기물의 부피가 증가하는 단점을 갖게 되어 처분 비용의 증가 및 처분장의 수용성을 감소하는 결과를 야기할 수가 있 다. 따라서 이들 문제를 해결하고자 본 연구에서는 최종 폐기물 부피의 감용화를 위해 롤 압축 기술을 이용하여 분말의 펠렛화 연구를 수행하였다.