With South Korea increasingly focusing on nuclear energy, the management of spent nuclear fuel has attracted considerable attention in South Korea. This study established a novel procedure for selecting safety-relevant radionuclides for long-term safety assessments of a deep geological repository in South Korea. Statistical evaluations were performed to identify the design basis reference spent nuclear fuels and evaluate the source term for up to one million years. Safety-relevant radionuclides were determined based on the half-life criteria, the projected activities for the design basis reference spent nuclear fuel, and the annual limit of ingestion set by the Nuclear Safety and Security Commission Notification No. 2019-10 without considering their chemical and hydrogeological properties. The proposed process was used to select 56 radionuclides, comprising 27 fission and activation products and 29 actinide nuclides. This study explains first the determination of the design basis reference spent nuclear fuels, followed by a comprehensive discussion on the selection criteria and methodology for safety-relevant radionuclides.

The timescale for the post-closure safety assessment of a deep geological repository ranges from ten thousand to a million year. In such a long period of time, the biosphere inevitably undergoes changes. Therefore, the long-term evolution of a biosphere is recognized as an important issue in the post-closure safety assessment of a deep geological repository for spent fuels. In this study, we reviewed the approaches to address the long-term evolution of a biosphere. The major drivers of longterm evolution of a biosphere are the climate change and the resulting landscape development. They can affect the hydrogeological and hydrogeochemical characteristics of a biosphere, and then the radionuclide migration through the biosphere followed by the exposure doses for the critical groups. In addition, human activities and the social developments can affect the climate change resulting in the long-term evolution of a biosphere. To make a biosphere assessment, the long-term evolution scenarios for the biosphere should be formulated considering these climate change, landscape development, and human activities. In addition, features, events, and processes (FEPs) that affect the long-term evolution of a biosphere should be used. According to the Safety Case reports of Finland, the major long-term evolution scenario drivers of a biosphere are local sea-level change due to climate change and land use related to crop type, irrigation procedures, livestock, forest management, construction of a well, and demographics. The climate change causing the local sea-level change can be simulated using various earth system models such as CLIMBER-2, MPI/UW, and UVic and an icesheet model such as SICOPOLIS. The review results of this study and FEPs related to the climate change, the landscape development, and human activities will be used to formulate long-term evolution scenarios for the safety assessment of a deep geological repository for spent fuels.

The Korea Atomic Energy Research Institute (KAERI) has developed geological repository systems for the disposal of high-level wastes and spent nuclear fuels (SNFs) in South Korea. The purpose of the most recently developed system, the improved KAERI Reference Disposal System Plus (KRS+), is to dispose of all SNFs in Korea with improved disposal area efficiency. In this paper, a system-level safety assessment model for the KRS+ is presented with long-term assessment results. A system-level model is used to evaluate the overall performance of the disposal system rather than simulating a single component. Because a repository site in Korea has yet to be selected, a conceptual model is used to describe the proposed disposal system. Some uncertain parameters are incorporated into the model for the future site selection process. These parameters include options for a fractured pathway in a geosphere, parameters for radionuclide migration, and repository design dimensions. Two types of SNF, PULS7 from a pressurized water reactor and Canada Deuterium Uranium from a heavy water reactor, were selected as a reference inventory considering the future cumulative stock of SNFs in Korea. The highest peak radiological dose to a representative public was estimated to be 8.19×10-4 mSv‧yr-1, primarily from 129I. The proposed KRS+ design is expected to have a high safety margin that is on the order of two times lower than the dose limit criterion of 0.1 mSv‧yr-1.