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Characterization of Groundwater Colloids From the Granitic KURT Site and Their Roles in Radionuclide Migration KCI 등재 SCOPUS

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방사성폐기물학회지 (Journal of the Korean Radioactive Waste Society)
한국방사성폐기물학회 (Korean Radioactive Waste Society)
초록

The fundamental characteristics of groundwater colloids, such as composition, concentration, size, and stability, were analyzed using granitic groundwater samples taken from the KAERI Underground Research Tunnel (KURT) site by such analytical methods as inductively coupled plasma-mass spectrometry, field emission-transmission electron microscopy, a liquid chromatography-organic carbon detector, and dynamic light scattering technique. The results show that the KURT groundwater colloids are mainly composed of clay minerals, calcite, metal (Fe) oxide, and organic matter. The size and concentration of the groundwater colloids were 10–250 nm and 33–64 μg·L−1, respectively. These values are similar to those from other studies performed in granitic groundwater. The groundwater colloids were found to be moderately stable under the groundwater conditions of the KURT site. Consequently, the groundwater colloids in the fractured granite system of the KURT site can form stable radiocolloids and increase the mobility of radionuclides if they associate with radionuclides released from a radioactive waste repository. The results provide basic data for evaluating the effects of groundwater colloids on radionuclide migration in fractured granite rock, which is necessary for the safety assessment of a high-level radioactive waste repository.

목차
1. Introduction
2. Experiment and Analyses
    2.1 Groundwater Sampling
    2.2 Separation and Concentration of GroundwaterColloids
    2.3 Analytical Methods
3. Results and Discussion
    3.1 Composition and Concentration ofGroundwater Colloids
    3.2 Size of Groundwater Colloids
    3.3 Organic Colloids
    3.4 Stability of Groundwater Colloids
    3.5 Comparison of Properties for GraniticGroundwater Colloids
    3.6 Roles of Groundwater Colloids in theMobility of Radionuclides
4. Conclusions
Acknowledgements
REFERENCES
저자
  • Min-Hoon Baik(Korea Atomic Energy Research Institute, 111, Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon 34057, Republic of Korea) Corresponding Author
  • Tae-Jin Park(Korea Atomic Energy Research Institute, 111, Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon 34057, Republic of Korea)
  • Hye-Ryun Cho(Korea Atomic Energy Research Institute, 111, Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon 34057, Republic of Korea)
  • Euo Chang Jung(Korea Atomic Energy Research Institute, 111, Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon 34057, Republic of Korea)