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Predicting the Distribution Coefficients of Radionuclides Using Machine Learning

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한국방사성폐기물학회 학술논문요약집 (Abstracts of Proceedings of the Korean Radioactive Wasts Society)
한국방사성폐기물학회 (Korean Radioactive Waste Society)
초록

Nuclear facilities present the important task related to the migration and retention of radioactive contaminants such as cesium (Cs), strontium (Sr), and cobalt (Co) for unexpected events in various environmental conditions. The distribution coefficient (Kd) is important factor for understanding these contaminants mobility, influenced by environmental variables. This study focusses the prediction of Kd values for radionuclides within solid phase groups through the application of machine-learning models trained on experimental data and open source data from Japan atomic energy agency. Three machine-learning models, such as the convolutional neural network, artificial neural network, and random forest, were trained for prediction model of the distribution coefficient (Kd). Fourteen input variables drawn from the database and experimental data, including parameters such as initial concentration, solid-phase characteristics, and solution conditions, served as the basis for model training. To enhance model performance, these variables underwent preprocessing steps involving normalization and log transformation. The performances of the models were evaluated using the coefficient of determination. These results showed that the environmental media, initial radionuclide concentration, solid phase properties, and solution conditions were significant variables for Kd prediction. These models accurately predict Kd values for different environmental conditions and can assess the environmental risk by analyzing the behavior of radionuclides in solid phase groups. The results of this study can improve safety analyses and longterm risk assessments related to waste disposal and prevent potential hazards and sources of contamination in the surrounding environment.

저자
  • In-Ho Yoon(Korea Atomic Energy Research Institute (KAERI)) Corresponding author
  • Seongyeon Na(Ulsan National Institute of Science and Technology (UNIST))
  • Seok Min Hong(Ulsan National Institute of Science and Technology (UNIST))
  • Ilgook Kim(Korea Atomic Energy Research Institute (KAERI))
  • Ikjune Kim(Korea Atomic Energy Research Institute (KAERI))
  • KwanSeong Jeong(Korea Atomic Energy Research Institute (KAERI))
  • Kyung Hwa Cho(Korea University)