Recently, measuring instruments for SHM of structures had being developed. In general, the wireless transmission of sensor signals, compared to its wired counterpart, is preferable due to its absence of triboelectric noise and elimination of the requirement for cumbersome cable. However, the research on the tall buildings with relatively small vibration levels is insufficient. Therefore, in this paper, we used the wireless MEMS sensor and iPad to compare and analyze the vibration measurements of three tall buildings and two towers.