Currently, Japan is undertaking a nationwide project to measure and map radioactive contamination around Fukushima, as part of the efforts to restore normalcy following the nuclear accident. The Japan Atomic Energy Agency (JAEA) manages the Fukushima Environmental Safety Center, located approximately 20 km north of the Fukushima Daiichi nuclear power plant in Minamisōma City, Fukushima Prefecture. In collaboration with the JAEA, this study involved conducting comparison experiments and analyses with radiation detectors in high radiation environments, a challenging task in Korean environments. Environmental radiation surveys were conducted using three types of detectors: CZT, NaI(Tl), and LaBr3(Ce), across two contaminated areas. Dose rate values were converted using dose rate conversion factors for each detector type, and dose rate maps were subsequently created and compared. The detectors yielded similar results, demonstrating their feasibility and reliability in high radiation environments. The findings of this study are expected to be a crucial reference for enhancing the verification and supplementation of procedures and methods in future radiation measurements and mobile surveys in high-radiation environments, using these three types of radiation instruments.

In-situ gamma spectrometer with mobile equipment can be used for rapid determination of radioactivity in the environment within a very short interval. 2”×2” NaI(Tl) scintillator are used to build a mobile radiation measurement system (called as Monitoring of Ambient Radiations of KAERI for Backpack, MARK-B3) with a signal processing unit, and GPS and interface units to a PC for wireless controlling system. Development of the survey system is to measure ambient gamma-ray spectrometry for estimating ground radioactivity and radiation dose in the environment. The ambient dose rate is estimated using G-factor method. For determination of G-factor, we conducted MCNP simulations in assumptions of various incident photons into the detector system. And the scintillator was exposed to Cs-137 source in the range of 1- 300 mGy/hr. Calculated dose rates for different simulation results were compared to the irradiated dose rate to derive correction factor of G-factor. To evaluate performance of the MARK-B3, in-situ gamma spectrometry was conducted in Jeju island.

Airborne surveys are an essential analysis method for rapid response and contamination identification in the early event of a radiation emergency. On the other hand, airborne surveys are far from the ground, so it is necessary to convert the dose rate at a height of 1 m above the ground. In order to improve the accuracy of the analysis value, a lot of analysis of the measurement data is required. In our previous research, we developed MARK-A1, an instrument for rapid radiation aerial survey in high radiation environment, and MARK-M1, a multipurpose instrument for radiation detection. In this study, a large unmanned aerial vehicle (UAV) was used to conduct airborne surveys using three types of detectors in the Jeju Island environment. The NaI(Tl) detector uses one 3-inch scintillator (38 mm φ × 38 mm H), and the LaBr3 detector uses two 2-inch scintillators (25 mm φ × 25 mm H). The CZT detector uses a detector with dimensions of (15 mm × 15 mm × 7.5 mm). The UAV has a payload of 15 kg (J10, JCH systems Inc. Seoul, Korea). Three different detectors were operated at a constant height of 20 m, 30 m, and 50 m. The flight experiments were performed in the west near Jeju City. Dose rate conversion factors were used to convert the dose rate from the measured spectra, and hovering flights were conducted between 1 and 50 meters to derive altitude correction factors. In this paper, the data measured with each detector in the same area were compared and the differences were derived.

This study was performed to assess the cosmic-ray effect caused by altitude in the aerial gammaray measurement. For the gamma-ray measurement experiment by altitude, the aerial survey system composed of four 4×4×16 inches large volume NaI (Tl) detectors was used. The aerial survey system was installed in a rotor-craft to stably keep its flight altitude and position. In addition, in order to avoid to time-dependent shielding effects with the amount of fuel, a rotor-craft of which the fuel tank is not located beneath the cabin floor was selected. In this study, the ROI (Region Of Interest) was set to the 3~6 MeV range to assess the cosmic-ray contribution to the gamma-ray spectrum that could ignore the contribution of the dominant natural radionuclides. The gamma-ray spectra measured inside and outside of the rotor-craft on the ground were compared to evaluate the shielding effects of the aircraft body. As a result, the count rate of the 40K photo peak was decreased by about 10% when measuring the inside compared to the outside. On the other hand, the total count rate of the 3~6 MeV region was decreased by about 0.7% under the same condition. Therefore, the aircraft body effect was insignificant in 3~6 MeV region considering the relative uncertainty of 0.04~0.78% (1σ). In addition, the count rate in the 3~6 MeV range according to altitude was evaluated to assess the cosmic-ray effect. In order to evaluate the change in the ROI count rate according to the altitude, the gamma-ray spectrum was measured in the range of 300~2,000 m above the sea to avoid the effect of terrestrial radiation. As a result, the relationship between altitude and count rate in the 3~6 MeV range showed a high correlation with the R2 value of 0.99, when the approximate equation was derived in the form of a quadratic polynomial. Also, the count rate of 3~6 MeV at 50~500 m above the ground was estimated using the correlation equation, and this value was compared with the measured count rate. As a result of comparing the average value of estimated count rate and measured count rate, the relative difference is less than 2%. Considering the relative uncertainty of 0.78~4.11% (1σ), it was possible to evaluate the count rate of the 3~6 MeV region relatively accurately. The results of this study could be used for further study on background dose corrections in aerial survey.

본 연구에서는 원자력 사고 또는 방사선 비상 시 지표면에 침적될 수 있는 감마선방출 핵종의 방사능을 신속하게 평가하기 위해 이용될 수 있는 NaI(Tl), LaBr3(Ce) 및 CeBr3 섬광검출기의 성능을 비교 평가하였다. 검출성능은 최소검출가능방사능 (MDA, Minimum Detectable Activity)을 통해 평가하였으며, 각 검출기의 지표면 침적 감마선방출 핵종에 대한 검출효율은 수학적 모델링과 점선원을 이용하여 반실험적으로 산출하였다. MDA 평가를 위한 백그라운드 감마선에너지스펙트럼은 비교적 넓고 평탄한 초지에서 측정되었으며, 원자력 사고 시 방출될 수 있는 주요 핵종에 대한 각 검출기의 MDA를 산출하였다. 그 결과 일반 환경방사능 준위에서 지표면 침적 감마핵종에 대한 각 검출기의 MDA 크기는 대체로“NaI(Tl)> LaBr3(Ce)> CeBr3”로 평가되었으며, 백그라운드 준위가 유사한 에너지 영역에서는 분해능이 가장 우수한 LaBr3(Ce)에서 최소 값을 보였다. 이는 관심 핵종의 감마선에너지 영역에 대한 각 검출기의 자체 및 측정 환경 백그라운드, 측정 효율, 그리고 에너지 분해능 특성을 바탕으로 비교 분석되었다.

일반적으로 방사선 선원의 강도는 거리의 역자승 법칙을 따른다. 그러나 방사선 선원과 검출기와의 거리가 가까울수록 거리의 역자승 법칙 실험은 이론과 실험의 일치하지 못하는 오류를 가져오게 된다. 본 연구에서는 방사선 선원과검출기와의 거리에 따른 거리의 역자승 법칙이 실제 실험에서는 정확하게 성립하지 않는 이유를 실험적으로 확인하였다. 그리고 이 문제를 해결하기 위하여 측정된 방사능을 보정하기 위하여 보정계수를 실험적으로 얻었다. 측정에 사용한 검출기는 2˝×2˝ø NaI(Tl) 신틸레이션 검출기를 사용하였고, 방사선에너지의 변화에 따른 효과를 확인하기 위하여감마선 선원 60Co(1.174 MeV, 1.333 MeV)와 137Cs(0.662 MeV)에 대한 실험도 병행하였다. 측정에서 얻어진 거리의역자승 법칙의 결과들을 보정계수를 이용하여 측정값들을 보정한 결과 거리의 역자승 법칙과 매우 일치하는 경향을 보였고, 오류에 대한 원인을 실험적으로 확인하였다. 이러한 결과는 유한한 체적을 가진 검출기를 사용하여 방사선의 강도가 거리의 역자승에 반비례하는 실험을 할 경우 모두 해당되는 문제이므로 본 연구의 결과는 방사선계측 분야에 매우 유용하게 사용되어질 것으로 사료된다.

The neutron capture spectrum for the light nuclide was very useful to study the nuclear structure. In the present study, the capture gamma-ray from the 27-keV resonance of 19F(n,g)20F reaction were measured with an anti-Compton NaI(Tl) spectrometer and the 3-MV Pelletron accelerator of the Research Laboratory for Nuclear Reactors at the Tokyo institute of technology. A neutron Time-of-Flight method was adopted with a 1.5 ns pulsed neutron source by the 7Li(p,n)7Be reaction. In the present experiment, a Teflon((CF2)n) sample was used The sample was disk with a diameter of 90mm. The thickness of sample was determined so that reasonable counting rates could be obtained and the correction was not so large for the self-shielding and multiple scattering of neutrons in the sample, and was 5mm. The primary gamma-ray transitions were compared with previous measurement of Kenny.