Undeclared nuclear activities are challenging given the lack of information from the sites involved in such activities. Wide-area environmental sampling (WAES) can be an effective method to detect undeclared nuclear activities. However, it is crucial to address the potential risks during the WAES, including sample tampering or extortions. Therefore, tracking and monitoring of various on-site data is imperative to accurately interpret the status of samples and workers throughout the WAES process. ‘Environmental and Geographical Data Transfer (EGDT)’ was developed for the real-time monitoring of integrated on-site data. EGDT module is equipped with various sensors and can be attached to a worker’s uniform or a sample storage box. This study demonstrated the technical effectiveness of EGDT by exploring three experimental methodologies for feasibility assessment. Compared to the Normal Operation case, the inference of the Sample Extortion case was predominantly based on changes in lux and dose rate. The inference of the Out-of-Work-Area case primarily relied on changes in dose rate and acceleration. Finally, the preliminary evaluation of the performance of the developed prototype was conducted, and a foundation was established for enhancing the application in the WAES process.

Recently, the status of North Korea’s denuclearization has become an international issue, and there are also indications of potential nuclear proliferation among neighboring countries. So, the need for establishment of nuclear activity verification technology and strategy is growing. In terms of ensuring verification completeness, sample collection-based analysis is essential. The concepts of Chain of Custody (CoC) and Continuity of Knowledge (CoK) can be defined in the process of sample extraction as follows: CoC is interpreted as the ‘system for managing the flow of information subjected by the examinee’, and CoK is interpreted as the ‘Continuity of information collection through CoC subjected by the inspector’. In the case of sample collection process in unreported areas for nuclear activity verification, there are additional risks such as worker exposure/kidnapping or sample theft/tampering. Therefore, the introduction of additional devices might be required to maintain CoC and CoK in the unreported area. In this study, an Environmental Geometrical Data Transfer (EGDT) was developed to ensure the safety of workers and the CoC/CoK of the samples during the collection process. This device was designed for achieving both mobility and rechargeability. It is categorized into two modes based on its intended users: sample mode and worker mode. Through the sensors, which is positioned in the rear part of device, such as radiation, gyroscope, light, temperature, humidity and proximity sensors, it can be easily achievable various environmental information in real-time. Additionally, GPS information can also be received, allowing for responsiveness to various hazardous scenarios. Moreover, the OLED display positioned on the front gives us for checking device information such as the current status of the device such as the battery level, the connectivity of wifi, and etc. Finally, an alarm function was integrated to enable rapid awareness during emergency situations. These functions can be updated and modified through Arduino-based firmware, and both the device and the information collected through it can be remotely controlled via custom software. Based on the presented design conditions, a prototype was developed and field assessments were conducted, yielding results within an acceptable margin of error for various scenarios. Through the application of the EGDT developed in this study to the sample collection process for nuclear activity verification purposes, it is expected to achieve a stable maintenance of CoC/CoK through more accurate information transmission and reception.

Our research team has developed a gamma ray detector which can be distributed over large area through air transport. Multiple detectors (9 devices per 1 set) are distributed to measure environmental radiation, and information such as the activity and location of the radiation source can be inferred using the measured data. Generally, radiation is usually measured by pointing the detector towards the radioactive sources for efficient measurement. However, the detector developed in this study is placed on the ground by dropping from the drone. Thus, it does not always face toward the radiation source. Also, since it is a remote measurement system, the user cannot know the angle information between the source and detector. Without the angle information, it is impossible to correct the measured value. The most problematic feature is when the backside of the detector (opposite of the scintillator) faces the radiation source. It was confirmed that the measurement value decreased by approximately 50% when the backside of the detector was facing towards the radiation source. To calibrate the measured value, we need the information that can indicate which part of the detector (front, side, back) faces the source. Therefore, in this study, we installed a small gamma sensor on the backside of the detector to find the direction of the detector. Since this sensor has different measurement specifications from the main sensor in terms of the area, type, efficiency and measurement method, the measured values between the two sensors are different. Therefore, we only extract approximate direction using the variation in the measured value ratio of the two sensors. In this study, to verify the applicability of the detector structure and measurement method, the ratio of measured values that change according to the direction of the source was investigated through MCNP simulation. The radioactive source was Cs-137, and the simulation was performed while moving in a semicircular shape with 15 degree steps from 0 degree to 180 degrees at a distance of 20 cm from the center point of the main sensor. Since the MCNP result indicates the probability of generating a pulse for one photon, this value was calculated based on 88.6 μCi to obtain an actual count. Through the ratio of the count values of the two sensors, it was determined whether the radioactive source was located in the front, side, or back of the probe.

In emergency situations such as nuclear accidents or terrorism, radioactive and nuclear materials can be released by some environmental reasons such as the atmosphere and underground water. To secure the safety of human beings and to respond appropriately emergency situation, it is required to designate high and low dose rate regions in the early stages by analyzing the location and radioactivity of sources through environmental radiation measurement. This research team has developed a small gamma probe which is featured by its geometrical accessibility and higher radiation sensitivity than other drone detectors. A plastic scintillator and Silicon Photomultiplier (SiPM) were applied to the probe to optimize the wireless measurement condition. SiPM has a higher gain (higher than 106) and lower operating voltage (less than 30 V) compared to a general photodiode. However, the electronic components in the SiPM are sensitively affected by temperature, which causes the performance degradation of the SiPM. As the SiPM temperature increases, the breakdown voltage (VBD) of the SiPM also increases, so the gain must be maintained by applying the appropriate VBD. Therefore, when the SiPM temperature increases while the VBD is fixed, the gain decreases. Thus, the signal does not exceed the threshold voltage (VTH) and the overall count is reduced. In general, the optimal gain is maintained by cooling the SiPM or through a temperature compensation circuit. However, in the developed system, the hardware correction method such as cooling or temperature compensation circuit cannot be applied. In this study, it was confirmed that the count decreased by up to 20% according to the increase in the temperature of the SiPM when the probe was operated at room temperature (26°C). We propose methods to calibrate the total count without cooling device or compensation circuit. After operating the probe at room temperature, the first measured count is set as the reference value, and the correction factor is derived using the tendency of the count to decrease as the temperature increases. In addition, since this probe is used for environmental radiation monitoring, periodic measurements are more suitable than continuous measurements. Therefore, the temperature of the probe can be maintained by adding a power saving interval to the operation sequence of the probe. These two methods use the operation sequence and measurement data, respectively. Thus, it is expected to be the most effective method for the current system where the temperature compensation through hardware is not possible.

When the nuclear accident like the Fukushima is occurred, it is required to immediately determine the location of radioactive materials and their activities. Various studies related the unmanned technique to detect and characterize the contaminated area have been conducted. The Korea Institute of Nuclear Nonproliferation and Control (KINAC) has developed a new gamma detection system which consists of nine probes using a silicon photomultiplier (SiPM) and plastic scintillator. The probe is the small gamma detector designed to be carried and dropped near the accident area by the unmanned aerial vehicle. In this paper, we developed the improved design related to the angular dependence of the radioactive contamination detection system with the purpose of increasing the detection efficiency. The detection efficiency, radiation shielding and back-scattering varies depending on the direction of incidence of radiation because the probe has vertical structure of consisting scintillator, photomultiplier, and electric circuits. That is, when the experimental conditions are same except the direction of gamma probe, the result of measurements is different. It causes errors in measuring the radioactivity and location of the radioactive source. Since the direction of the probe is arbitrarily determined during the deployment of the probe through the unmanned aerial vehicle, it is considered changing the design of the scintillator from a conventional 1.0" × 1.0" Φ cylindrical shape to a 1.0" Φ spherical shape. In case of using the spherical scintillator, it is confirmed that angular dependence was reduced through MCNP simulation. The difference in the measurement depending on the direction of the probe could be reduced through additional structure design. Finally, we hope that the developed detection system which has the probes with spherical shape of scintillator can measure the radioactivity and location of the radioactive source in a range of about 100 × 100 m2 by measuring for at least 5 minutes. The field test at Fukushima area will be carried out with JAEA members in order to prove the feasibility of the new system.

The Republic of Korea is expected to participate in the denuclearization verification activities by the International Atomic Energy Agency (IAEA) in case any neighboring countries declared denuclearization. In this study, samples for the verification of nuclear activities in undeclared areas were selected for the denuclearization of neighboring countries, and the appropriateness of the procedures was considered. If a country with nuclear weapons declares denuclearization, it must be accompanied by the IAEA’s verification regarding nuclear materials and weapons in the declared and undeclared areas. The analysis of the process samples or on-site environmental samples and the verification of undeclared nuclear facilities and materials aid in uncovering any evidence of concealment of nuclear activity in undeclared areas. Therefore, a methodology was established for effective sampling and analysis in accordance with proper procedures. Preparations for sampling in undeclared areas were undertaken for various potential scenarios, such as, the establishment of zones according to radiation dose, methods of supplying electricity, wireless communication networks, targets of sampling according to characteristics of nuclides, manned sampling method, and unmanned sampling method. Through this, procedures were established for pre- and post-site settings in preparation for hazards and limiting factors at nuclear inspection sites.

다양한 수질 오염원 중 페놀과 같은 유기화합물은 배출조건이 비정상적인 경우 기존의 처리방법으로 제거하거나 파괴하기 어렵다. 수용액으로부터 페놀을 분리하기 위한 최근의 연구들은 활성탄에 의한 흡착, 용매 추출 등에 의해 수행되어져 왔으며, 물-기름 유화에 기초를 둔 액막법이 기존의 기술들을 대체하기 위한 방법으로 시험되어져 왔다. 본 연구에서는 tri-n-butyl phosphate(TBP)와 액상 고분자를 지지액막의 액막용액으로 선정하여 수용액상의 페놀을 분리하였다. 공급측 페놀 농도를 변화시키고 다양한 액막용액을 사용하여 이들이 페놀분리에 미치는 효과를 연구하였다. TBP를 운반체로 사용한 경우의 실험결과들은 용매추출에서 주로 사용되고 있는 methyl isobutyl ketone(MIBK)보다 높은 물질전달속도를 보여주었으며, 선택한 액상고분자 중 polypropylene glycol 4000(PPG-4000), polybutylene glycol 500(PBG 500)의 경우 MIBK와 유사하거나 조금 높은 값을 나타내었다.