Interim dry cask storage systems comprising AISI 304 or 316 stainless steel canisters have become critical for the storage of spent nuclear fuel from light water reactors in the Republic of Korea. However, the combination of microstructural sensitization, residual tensile stress, and corrosive environments can induce chloride-induced stress corrosion cracking (CISCC) for stainless steel canisters. Suppressing one or more of these three variables can effectively mitigate CISCC initiation or propagation. Surface-modification technologies, such as surface peening and burnishing, focus on relieving residual tensile stress by introducing compressive stress to near-surface regions of materials. Overlay coating methods such as cold spray can serve as a barrier between the environment and the canister, while also inducing compressive stress similar to surface peening. This approach can both mitigate CISCC initiation and facilitate CISCC repair. Surface-painting methods can also be used to isolate materials from external corrosive environments. However, environmental variables, such as relative humidity, composition of surface deposits, and pH can affect the CISCC behavior. Therefore, in addition to research on surface modification and coating technologies, site-specific environmental investigations of various nuclear power plants are required.

Because most spent nuclear fuel storage casks have been designed for low burnup fuel, a safety-significant high burnup dry storage cask must be developed for nuclear facilities in Korea to store the increasing high burnup and damaged fuels. More than 20% of fuels generated by PWRs comprise high burnup fuels. This study conducted a structural safety evaluation of the preliminary designs for a high burnup storage cask with 21 spent nuclear fuels and evaluated feasible loading conditions under normal, off-normal, and accident conditions. Two types of metal and concrete storage casks were used in the evaluation. Structural integrity was assessed by comparing load combinations and stress intensity limits under each condition. Evaluation results showed that the storage cask had secured structural integrity as it satisfied the stress intensity limit under normal, off-normal, and accident conditions. These results can be used as baseline data for the detailed design of high burnup storage casks.

A transfer cask serves as the container for transporting and handling canisters loaded with spent nuclear fuels from light water reactors. This study focuses on a cylindrical transfer cask, standing at 5,300 mm with an external diameter of 2,170 mm, featuring impact limiters on the top and bottom sides. The base of the cask body has an openable/closable lid for loading canisters with storage modules. The transfer cask houses a canister containing spent nuclear fuels from lightweight reactors, serving as the confinement boundary while the cask itself lacks the confinement structure. The objective of this study was to conduct a structural analysis evaluation of the transfer cask, currently under development in Korea, ensuring its safety. This evaluation encompasses analyses of loads under normal, off-normal, and accident conditions, adhering to NUREG-2215. Structural integrity was assessed by comparing combined results for each load against stress limits. The results confirm that the transfer cask meets stress limits across normal, off-normal, and accident conditions, establishing its structural safety.

For the sake of future generations, the management of radioactive waste is essential. The disposal of spent nuclear fuel (SNF) is considered an urgent challenge to ensure human safety by storing it until its radioactivity drops to a negligible level. Evaluating the safety of disposal facilities is crucial to guarantee their durability for more than 100,000 years, a period sufficient for SNF radioactivity to become ignored. Past studies have proposed various parameters for forecasting the safety of SNF disposal. Among these, radiochemistry and electrochemistry play pivotal roles in predicting the corrosion-related chemical reactions occurring within the SNF and the structural materials of disposal facilities. Our study considers an extreme scenario where the SNF canister becomes compromised, allowing underground water to infiltrate and contact the SNF. We aim to improve the corrosion mechanism and mass-balance equation compared with what Shoesmith et al. proved under the same circumstances. To enhance the comprehensibility of the chemical reactions occurring within the breached SNF canister, we have organized these reactions into eight categories: mass diffusion, alpha radiolysis, adsorption, hydrate formation, solidification, decomposition, ionization, and oxidation. After categorization, we define how each species interacts with others and calculate the rate of change in species’ concentrations resulting from these reactions. By summing up the concentration change rates of each species due to these reactions, we redefine the mass-balance equations for each species. These newly categorized equations, which have not been explained in detail previously, offer a detailed description of corrosion reactions. This comprehensive understanding allows us to evaluate the safety implications of a compromised SNF canister and the associated disposal facilities by numerically solving the mass-balance equations.

For safe and economical spent fuel management, assessing the integrity of the cladding, which is the first barrier to the escape of radioactive material, is very important. For the sake of risk assessment, it is essential to calculate the probability of failure of the spent fuel rods loaded inside the cask during the transportation or storage. However, due to the large amounts of calculations required, it is not practical to analyze every detail of the spent fuel rods and assemblies. This study presents a methodology to perform a cask-level analysis by sequentially simplifying the fuel rods and spent fuel assemblies for the calculation of fuel rod failure probability. A simplified single fuel rod model was generated by considering the material properties of a high burnup fuel rod stored in dry storage for approximately 5 years and the interfacial bonding conditions of the cladding tube. The simplified model produces the same deflection as the detailed model at the critical moment that produces a fracture plastic strain of 1%. The developed single fuel rod simplified model is assembled in a CE 16×16 configuration, and a methodology is presented in which the CE 16×16 assembly model is once again replaced by a simplified model with a cuboidal shape. Compression analyses were performed on each part of the CE 16×16 model to obtain isotropic property data, and a simplified model was created based on those data and the cross-sectional second moment values of the parts. A cask drop analysis was performed to validate the similarity of the CE 16×16 model and the simplified model by comparing important structural responses such as impact acceleration. The 20 simplified fuel assembly models and one detailed model were loaded into a cask to perform the drop analysis. For the detailed model, the impact acceleration was extracted for different loading positions and the corresponding impact load and pinch load were derived. The spring force and contact force corresponding to the pinch load were extracted by applying a Python script technique to extract the maximum value of them exerted on each fuel rod. The vulnerability of spent fuel rods to bending loads and the failure criteria were considered during the simplification process of a single fuel rod. From the extracted impact and pinch loads, the probability of failure of the spent fuel rods as a function of impact acceleration can be calculated.

Considering the domestic situation where all nuclear power plants are located on seaside, the interim storage site is also likely to be located on coastal site. Maritime transportation is inevitable and the its risk assessment is very important for safety. Currently, there is no independently developed maritime transportation risk assessment code in Korea, and no research has been conducted to evaluate the release of radioactive waste due to the immersion of transport cask. Previous studies show that the release rate of radionuclides contained in a submerged transport cask is significantly affected by the area of flow path generated at the breached containment boundary. Due to the robustness of a cask, the breach is the most likely generated between the lid and body of cask. CRIEPI investigated the effect of cask containment on the release rate of radioactive contents into the ocean and proposed a procedure to calculate the release rate considering the socalled barrier effect. However, the contribution of O-ring on the release rate was not considered in the work. In this study, test and analysis is performed to determine the equivalent flow path gap considering the influence of O-rings. These results will be implemented in the computational model to assess sea water flow through a breached containment boundary using CFD techniques to assess radionuclide release rates. To evaluate the release rate as a function of lid displacement, a small containment vessel is engineered and a metal O-ring of the Helicoflex HN type is installed, which is the most commonly used one in transport and storage casks. The lid of containment vessel is displaced in vertical and horizontal direction and the release rate of the vessel was quantified using the helium leak test and the pressure drop test. Through this work, the relationship between the vertical opening displacement and horizontal sliding displacement of the cask lid and the actual flow path area created is established. This will be implemented in the CFD model for flow rate calculation from a submerged transport cask in the deep sea. In addition, the compression of the O-ring causes very small gaps, such as capillaries. In these cases, Poiseuille’s law is used to calculate the capillary flow rate.

Spent nuclear fuels should be safely stored until being disposed and dry storage system is predominantly used to retain the fuels. Thermal analysis to estimate temperatures of spent nuclear fuel and the storage system should be performed to evaluate whether the temperatures exceed safety limit. Recently, thermal hydraulic analysis with CFD codes is widely used to investigate the temperature of spent nuclear fuel in dry storage. COBRA-SFS is a legacy code based on subchannel analysis code, and its fidelity is verified for evaluating the thermal analysis for licensing a dry cask system. Herein, thermal analysis result based on CFD and COBRA-SFS codes is compared and the Dry Cask Simulator (DCS) is assessed as a benchmark experiment in this study. Extended Storage Collaborating Program (ESCP) led by the Electric Power Research Institute (EPRI) is organized to address the degradation effects of spent nuclear fuel during long-term dry storage, and DCS is the first phase of the program. The dry storage system, containing a single BWR assembly in a canister, was designed to produce validation-quality data for thermal analysis model. ANSYS FLUENT was used to simulate DCS. Simulations were conducted in various decay heat and helium pressure inside the canister. In realistic conditions of decay heat and helium pressure of actual dry cask system, CFD and COBRA-SFS analysis results gave good agreement with experimental measurement. Peak temperatures of channel can, basket, canister and shell predicted by CFD simulation also showed good prediction and the discrepancies were less than 7 K while measurements uncertainty was 7 K. In high decay heat and high pressure condition, however, CFD and COBRA-SFS underestimated peak cladding temperature than experimental results.

In the case of dry storage facilities, slipping of the cask or tip-over are dangerous phenomena. For this reason, in dry storage facilities, measures against slipping and tip-over or related safety evaluations are important. Accidental conditions that can cause cask slippage and tip-over in dry storage facilities include natural phenomena such as floods, tornadoes, tsunamis, typhoons, earthquakes, and artificial phenomena such as airplane crashes. However, among natural phenomena, earthquakes are the most important natural phenomenon that causes tip-over. Also, many people had the stereotype that Korea is an earthquake-safe zone before 2016. However, earthquakes become a major disaster in Korea due to the 2016 Gyeongju earthquake and the 2017 Pohang earthquake, followed by the Goesan earthquake in October 2022. In this paper, seismic analysis was performed based on dry storage facilities including multiple casks. Design variables for the construction of an analysis model for dry storage facilities were investigated, and seismic analysis was performed. To evaluate tip-over accident during earthquake, seismic load was used from 0.2 g PGA to 0.8 g PGA and these earthquakes were followed Design Response Spectrum (DRS) in RG 1.60. The friction coefficient of concrete pad was used from 0.2 to 1.0. As a result of the analysis, tip-over accident could not find in the analysis from 0.2 g to 0.6 g. However, tip-over was appeared at friction coefficients of 0.8 and 1.0 at 0.8 g PGA. Tip-over angular velocity of cask was derived by seismic analysis and was compared with formula and tip-over analysis results. As a result, a generalized dry storage facility analysis model was proposed, and dry storage facility safety evaluation was conducted through seismic analysis. Also, tip-over angular velocity was derived using seismic analysis for tip-over analysis.

Given the situation in the Republic of Korea that all nuclear power plants are located at the seaside, the interim storage facility is also likely to be located at seaside and the maritime transportation of Spent Nuclear Fuel is considered inevitable. The Republic of Korea does not have an independently developed maritime transportation risk assessment code, and no research has been conducted to evaluate the release rate of radionuclides from a submerged transportation cask in the sea. Therefore, there is a need to develop a technology that can assess the impact of immersion accidents and establish a regulatory framework for maritime transportation accidents. The release rate of radionuclides should be calculated from the flow rate through a flow path in the breached containment boundary. According to the cask design criteria, it is anticipated that even under severe accident conditions, the flow path size will be very small. Previous studies have evaluated fluid flow passing through micro-scale channel by integrating internal and external flows within and around a transport cask. As part of the evaluation, a comprehensive “Full-Field Model” incorporating external flow fields and a localized “Local-Field Model” with micro-scale flow paths were constructed. Sub-modeling techniques were employed to couple the flow field calculated by the two models. The aforementioned approach is utilized to conduct the evaluation of fluid flow passing through micro-scale flow paths. This study aims to evaluate fluid flow passing through micro-scale flow paths using the aforementioned CFD (Computational Fluid Dynamics) method and aims to code the findings. The Gaussian Process Regression technique, a machine learning model, is utilized for developing a mathematical metamodel. The selected input parameters for coding are organized and their respective impacts are analyzed. The range of these selected parameters is tailored to suit domestic environments, and computational experiments are planned through Design of Experiments. The flow path size is included as an input parameter in the coded model. In cases where the flow path size becomes extremely small, making it impractical to use CFD techniques for calculations, Poiseuille’s law is employed to calculate the release rate. In this study, a model is developed to evaluate the release rate of radionuclides using CFD and mathematical equations covering the whole possible range of flow path size in a lost cask in the deep sea. The model will be used in the development of a maritime transportation risk assessment code suitable for the situation and environment in Korea.

As regulations on carbon emissions increase, the interest in renewable energy is also increasing. However, the efficiency of renewable energy generation is highly low and has limitations in replacing existing energy consumption. In terms of this view, nuclear power generation is highlighted because it has the advantage of not emitting carbon. And accordingly, the amount of spent nuclear fuel is going to increase naturally in the future. Therefore, it will be important to obtain the reliability of containers for transporting safely and storing spent nuclear fuel. In this study, a method for verifying the integrity and airtightness of a metal cask for the safe transportation and storage of spent nuclear fuel was studied. Non-destructive testing, thermal stability, leakage stability, and neutron shielding were demonstrated, and as a result, suitable quality for loading spent nuclear fuel could be obtained. Furthermore, it is meaningful in that it has secured manufacturing technology that can be directly applied to industrial field by verifying actual products.

This study investigates the behavior of the thermal conductivity among material properties in order to develop a thermal evaluation methodology of spent fuel assembles in a transport cask. It is inefficient to model each element of the spent fuel assembly in detail, and it is generally calculated by modeling the effective thermal conductivity (ETC). The ETC model was developed to allow a much simpler representation of a spent fuel assembly within a fuel compartment by treating the entire spent fuel rod array and the surrounding fill gas within the confines of the compartment as a homogenous solid material. The fuel rod assembly and surrounding gas are modeled with an effective conductivity that is designed to yield an overall conduction heat transfer rate that is equivalent to the combined effect of local conduction and radiation heat transfer in a plane through the assembly. When this model is applied to the transport cask, it tends to predict the cladding peak temperature lower than the results of detailed model in which the fuel rod arrangement and shape of the fuel assembly are simulated. As for the tendency of the error, the model tended to under-predict when basket temperature was lower than a certain temperature, and over-predict when it was higher. The purpose of this study is to investigate the attenuation effect of the cladding peak temperature on the related variables when the ETC model is applied to the transport cask. In addition, based on the thermal characteristics of this model, a correction factor that can compensate for this attenuation effect is presented. This correction factor is obtained by finding the difference between a separate ETC homogeneous model and a separate detailed fuel model, rather than directly applying the ETC calculated from the detailed fuel model to the transport cask.

Concrete structures of spent nuclear fuel interim storage facility should maintain their ability to shield and structural integrity during normal, off-normal and accident conditions. The concrete structures may deteriorate if the interim storage facility operates for more than several decades. Even if deterioration occurs, the concrete structures must maintain their own functions such as radiation shielding protection and structural integrity. Therefore, it is necessary to establish an analysis methodology that can evaluate whether the deteriorated concrete structure maintains its integrity under not only normal or off-normal condition but also accident condition. In accident conditions such as tip over and aircraft collision, both static material properties and dynamic properties are needed to evaluate the structural integrity of the concrete structures. Especially, it has been known to be difficult to estimate the resulted damage precisely where an aircraft collides with the degraded concrete structures at a high strain rate. In this study, damage evaluation of concrete overpack due to aircraft collisions was conducted. First, in order to verify the impact analysis methodology, the aircraft impact analysis of plane concrete overpack was performed and compared with the test results previously conducted by our research team. Then, the impact analysis for the overpack of KORAD21C was performed. In the future, the radiation shielding analysis will be performed under the conditions to evaluate whether or not the radiation shielding ability is maintained.

In concrete structures exposed to chloride environments such as seashore structures, chloride ions penetrate into the concrete. Chlorine ions in concrete react with cement hydrates to form Friedel’s salt and change the microstructure. Changes in the microstructure of concrete affect the mechanical performance, and the effect varies depending on the concentration of chloride ions that have penetrated. However, research on the mechanical performance of concrete by chloride ion penetration is lacking. In this study, the effect of chloride ion penetration on the mechanical performance of dry cask concrete exposed to the marine environment was investigated. The mixture proportion of self-compacting concrete is used to produce concrete specimens. CaCl2 was used to add chlorine ions, and 0, 1, 2, and 4% of the binder in weight were added. To evaluate the mechanical performance of concrete, a compressive strength test, and a splitting tensile strength test were performed. The compressive strength test was conducted through displacement control to obtain a stress-strain curve, and the loading speed was set to 10 με/sec, which is the speed of the quasi-static level. The splitting tensile strength test was performed according to KS F 2423. As a result of the experiment, the compressive strength increased when the chloride ion concentration was 1%, and the compressive strength decreased when the chlorine ion concentration was 4%. The effect of the chloride ion concentration on the peak strain was not shown. In order to present a stress-strain curve model according to the chloride ion concentration, the existing concrete compressive stress-strain models were reviewed, and it was confirmed that the experimental results could be simulated through the Popovics model.

Spent nuclear fuels should be safely stored until being disposed and dry storage system is predominantly used to retain the fuels. During long-term storage, there are several mechanisms that could result in the degradation of spent nuclear fuels, and the temperature is the most important parameter to predict and estimate the degradation behaviors. Therefore, thermal analysis to estimate temperatures of spent nuclear fuel and the storage system should be performed to evaluate whether the temperatures exceed safety limit. Recently, thermal hydraulic analysis with CFD codes is widely used to investigate the temperature of spent nuclear fuel in dry storage. Herein, Explicit CFD analysis model is introduced and validated by estimating the thermal hydraulic response of the dry storage system that is Dry Cask Simulator (DCS). Extended Storage Collaborating Program (ESCP) led by the Electric Power Research Institute (EPRI) is organized to assess degradation effects of spent nuclear fuel during long-term dry storage, and DCS is the first phase of the program. The dry storage system, containing a single BWR assembly in a canister, was designed to produce validation-quality data for thermal analysis model. ANSYS FLUENT is used to simulate DCS, and the test condition of 0.5 kW decay heat and 100 kPa helium pressure was investigated in this study. In case of peak cladding temperature (PCT), PCT from the experiment was 376 K while that of CFD was 374 K. It implies CFD simulation gives good agreement with experimental measurement. Peak temperatures of channel can, basket, canister and shell predicted by CFD simulation also show good prediction and the discrepancies were less than 7 K while measurements uncertainty was 7 K.

A radiation shielding resin with thermal stability and high radiation shielding effect has been developed for the neutron shielding resin filled in the shielding shell of dry storage/transport cask for spent nuclear fuel. Among the most commercially available neutron shielding resins, epoxy and aluminum hydroxide boron carbide are used. But in case of the resin, hydrogen content enhances the neutron shielding effect through optimization of aluminum hydroxide, zinc borate, boron carbide, and flame retardant. We developed a radiation shielding material that can increase the boron content and have thermal stability. Flame retardancy was evaluated for thermal stability, and neutron shielding evaluation was conducted in a research reactor to prove the shielding effect. As a result of the UL94 vertical burning test, a grade of V-0 was received. Therefore, it was confirmed that it had flame retardancy. According to an experiment to measure the shielding rate of the resin against neutron rays using NRF (Neutron Radiography Facility), a shielding rate of 91.54% was confirmed for the existing resin composition and a shielding rate of 96.30% for the developed resin composition. A 40 M SANS (40 M Small Angle Neutron Scattering Instrument) neutron shielding rate test was performed. Assuming aging conditions (6 hours, 180 degrees), the shielding rate was analyzed after heating. As a result of the experiment, the developed products with 99.8740% and 99.9644% showed the same or higher performance.