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        검색결과 9,282

        221.
        2023.11 구독 인증기관·개인회원 무료
        Dry storage of nuclear fuel is compromised by threats to the cladding integrity, such as creep and hydride reorientation. To predict these phenomena, spent fuel simulation codes have been developed. In spent fuel simulation, temperature information is the most influential factor for creep and hydride formation. Traditional fuel simulation codes required a user-defined temperature history input which is given by separate thermal analysis. Moreover, geometric changes in nuclear fuel, such as creep, can alter the cask’s internal subchannels, thereby changing the thermal analysis. This necessitates the development of a coupled thermal and nuclear fuel analysis code. In this study, we integrated the 2D FDM nuclear fuel code GIFT developed at SNU with COBRA -SFS. Using this, we analyzed spent nuclear stored in TN-24P dry storage cask over several decades and identified conditions posing threats due to phenomena like creep and hydrogen reorientation, represented by the burnup and peak cladding temperature at the start of dry storage. We also investigated the safety zone of spent nuclear fuel based on burnup and wet storage duration using decay heat.
        222.
        2023.11 구독 인증기관·개인회원 무료
        Post Irradiation Examination Facility (PIEF) is a test facility for nuclear fuel research and development and performance evaluation. From the past to the present, assemblies and fuel rods have been transported from nuclear power plants (NPP) several times, and various destructive and non-destructive tests have been performed. Among these, in the case of the 14×14 Westinghouse STD assemblies that are transported as a whole assembly, the top nozzle is connected to the guide tube by welding. Therefore, the fuel rods could not be removed from the assembly at the NPP, so the assemblies were transported to PIEF as is. Then, after cutting between the top nozzle and the guide tube in the pool, and the fuel rods were extracted and tested. In order to transport the assembly in the future, it is necessary to maintain stability by inserting the dummy rod into the unit cell from which the fuel rod is extracted. However, since the length of the dummy rod is almost 4 m and the diameter is about 10 mm, the dummy rod often bends while passing through the dimple spring of the grid. Additionally, when dummy rods are inserted into unit cells that are continuously empty after the fuel rods are extracted, there may be cases where the dummy rods are not inserted into the desired unit cell but are bent and incorrectly inserted into the next unit cell. The moment the dummy rods are inserted into the dimple spring of grid, a load is applied to the dummy rod due to the tension of the spring. If it can be inserted while offsetting the load, the work can be performed more smoothly. Accordingly, an underwater handling tool was developed that can be inserted while offsetting the tension of the spring. Using this handling tool applies a load to the dummy rod and rotates the dummy rod itself, offsetting the tension of the spring and allowing the dummy rod to be inserted without bending. This handling tool is equipped with a shock absorbing device to protect the dummy rod and spring, and a module to rotate the dummy rod. As a result of inserting the dummy rod using the developed handling tool, it was possible to easily insert the dummy rod into unit cells that were previously impossible to insert.
        223.
        2023.11 구독 인증기관·개인회원 무료
        In general, systems are developed by repeatedly performing the processes of design, analysis, manufacturing, and performance testing. In particular, systems with temperature, pressure, and flow rate often utilize computational fluid dynamics tools at the design stage. In this paper, we aim to verify the reliability of the analysis results of Solidworks Flow Simulation, which is widely used in heat flow analysis at the design stage. A tube furnace was manufactured, various experiments were performed, and a study was conducted to compare the analysis results. The details of the experiment are as follows. First, an experiment was conducted in which the heater was heated to 900°C without insulating the exposed part of the tube. The detailed contents of the experiment are as follows; - Heating heater and measuring temperature without supplying flow inside the tube, - Tube flow supply (25°C, 15 lpm air) and heater heating/temperature measurement. Second, an experiment was performed in which the exposed part of the tube was insulated (thickness 50 mm) and the heater was heated to 900°C. The detailed contents of the experiment are as follows; - Insulate the outside of the tube except for the flanges at both ends of the tube, and heat the heater and measure the temperature without supplying flow inside the tube. - Insulate the outside of the tube except for the flanges at both ends of the tube, supply flow rate inside the tube (25°C, 15 lpm air) and measure heater heating/temperature. - Insulate the flange of the flow supply section, heat the heater and measure temperature without supplying flow inside the tube. - Insulate the flange of the flow supply section, heat the supply air (277°C, 15 lpm) and measure the temperature using a heating gun without heating the heater. - Insulate the flange of the flow supply section, supply heated air (277°C, 15 lpm) and measure heater heating/temperature. - Insulate the flange of the flow supply section and measure temperature according to heater heating (900°C) and supply temperature (25°C, 277°C 15 lpm). The following results were derived from the experimental and analysis results. - When the exposed part of the tube is insulated, the temperature inside the tube increases and the steady-state power decreases compared to non-insulated. - In areas with insulation, the temperature error between experiment and analysis results is not large. - When flow rate is supplied, there is a large temperature error in experiment and analysis results. - The temperature change after the center of the heater is not large for a temperature change of 15 lpm flow rate. From these results, it can be seen that Solidworks Flow Simulation has a significant difference from the experimental results when there is a flow rate in the tube. This was thought to be because the flow rate acts as a disturbance, and this cannot be sufficiently accounted for in the analysis. In the future, we plan to check whether there is a way to solve this problem.
        224.
        2023.11 구독 인증기관·개인회원 무료
        Considering the domestic situation where all nuclear power plants are located on seaside, the interim storage site is also likely to be located on coastal site. Maritime transportation is inevitable and the its risk assessment is very important for safety. Currently, there is no independently developed maritime transportation risk assessment code in Korea, and no research has been conducted to evaluate the release of radioactive waste due to the immersion of transport cask. Previous studies show that the release rate of radionuclides contained in a submerged transport cask is significantly affected by the area of flow path generated at the breached containment boundary. Due to the robustness of a cask, the breach is the most likely generated between the lid and body of cask. CRIEPI investigated the effect of cask containment on the release rate of radioactive contents into the ocean and proposed a procedure to calculate the release rate considering the socalled barrier effect. However, the contribution of O-ring on the release rate was not considered in the work. In this study, test and analysis is performed to determine the equivalent flow path gap considering the influence of O-rings. These results will be implemented in the computational model to assess sea water flow through a breached containment boundary using CFD techniques to assess radionuclide release rates. To evaluate the release rate as a function of lid displacement, a small containment vessel is engineered and a metal O-ring of the Helicoflex HN type is installed, which is the most commonly used one in transport and storage casks. The lid of containment vessel is displaced in vertical and horizontal direction and the release rate of the vessel was quantified using the helium leak test and the pressure drop test. Through this work, the relationship between the vertical opening displacement and horizontal sliding displacement of the cask lid and the actual flow path area created is established. This will be implemented in the CFD model for flow rate calculation from a submerged transport cask in the deep sea. In addition, the compression of the O-ring causes very small gaps, such as capillaries. In these cases, Poiseuille’s law is used to calculate the capillary flow rate.
        225.
        2023.11 구독 인증기관·개인회원 무료
        The solid-state chemistry of uranium is essential to the nuclear fuel cycle. Uranyl nitrate is a key compound that is produced at various stages of the nuclear fuel cycle, both in front-end and backend cycles. It is typically formed by dissolving spent nuclear fuel in nitric acid or through a wet conversion process for the preparation of UF6. Additionally, uranium oxides are a primary consideration in the nuclear fuel cycle because they are the most commonly used nuclear fuel in commercial nuclear reactors. Therefore, it is crucial to understand the oxidation and thermal behavior of uranium oxides and uranyl nitrates. Under the ‘2023 Nuclear Global Researcher Training Program for the Back-end Nuclear Fuel Cycle,’ supported by KONICOF, several experiments were conducted at IMRAM (Institute of Multidisciplinary Research for Advanced Materials) at Tohoku University. First, the recovery ratio of uranium was analyzed during the synthesis of uranyl nitrate by dissolving the actual radioisotope, U3O8, in a nitric acid solution. Second, thermogravimetric-differential thermal analysis (TG-DTA) of uranyl nitrate (UO2(NO3)2) and hyper-stoichiometric uranium dioxide (UO2+X) was performed. The enthalpy change was discussed to confirm the mechanism of thermal decomposition of uranyl nitrate under heating conditions and to determine the chemical hydrate form of uranyl nitrate. In the case of UO2+X, the value of ‘x’ was determined through the calculation of weight change data, and the initial form was verified using the phase diagram for the U-O system. Finally, the formation of a few UO2+X compounds was observed with heat treatment of uranyl nitrate and uranium dioxide at different temperature intervals (450°C-600°C). As a result of these studies, a deeper understanding of the thermal and chemical behavior of uranium compounds was achieved. This knowledge is vital for improving the efficiency and safety of nuclear fuel cycle processes and contributes to advancements in nuclear science and technology.
        226.
        2023.11 구독 인증기관·개인회원 무료
        To address the pressing societal concern in Korea, characterized by the imminent saturation of spent nuclear fuel storage, this study was undertaken to validate the fundamental reprocessing process capable of substantially mitigating the accumulation of spent nuclear fuel. Reprocessing is divided into dry processing (pyro-processing) and wet reprocessing (PUREX). Within this context, the primary focus of this research is to elucidate the foundational principles of PUREX (Plutonium Uranium Redox Extraction). Specifically, the central objective is to elucidate the interaction between uranium (U) and plutonium (Pu) utilizing an organic phase consisting of tributyl phosphate (TBP) and dodecane. The objective was to comprehensively understand the role of HNO3 in the PUREX (Plutonium Uranium Redox Extraction) process by subjecting organic phases mixed with TBPdodecane to various HNO3 concentrations (0.1 M, 1.0 M, 5.0 M). Subsequently, the introduction of Strontium (Sr-85) and Europium (Eu-152) stock solutions was carried out to simulate the presence of fission products typically contented in the spent nuclear fuel. When the operation proceeds, the complex structure takes the following form. 􀜷􀜱􀬶 􀬶􀬾(􀜽􀝍) + 2􀜰􀜱􀬷 􀬿(􀜽􀝍) + 2􀜶􀜤􀜲(􀝋􀝎􀝃) ↔ 􀜷􀜱􀬶(􀜰􀜱􀬷)􀬶 ∙ 2􀜶􀜤􀜲(􀝋􀝎􀝃) Subsequently, separate samples were gathered from both the organic and aqueous phases for the quantification of gamma-rays and alpha particles. Alpha particle measurements were conducted utilizing the Liquid Scintillation Counter (LSC) system, while gamma-ray measurements were carried out using the High-Purity Germanium Detector (HPGe). The distribution ratio for U, Eu (Eu-152), and Sr (Sr-84) was ascertained by quantifying their activity through LSC and HPGe. Through the experiments conducted within this program, we have gained a comprehensive understanding of the selective solvent extraction of actinides. Specifically, uranium has been effectively separated from the aqueous phase into the organic phase using a combination of tributyl phosphate (TBP) and dodecane. Subsequently, samples containing U(VI), Eu(III), and Sr(II) underwent thorough analysis utilizing LSC and HPGe detectors. Our radiation measurements have firmly established that the concentration of nitric acid enhances the selective separation of uranium within the process.
        227.
        2023.11 구독 인증기관·개인회원 무료
        The hydride reorientation (HR) of used nuclear fuel cladding after operation affects the integrity during intermediate and disposal storage, as well as the handling processes associated with transportation and storage. In particular, during dry storage, which is an intermediate storage method, the radial hydrogen redistributes into circumferential hydrogen, increasing the embrittlement of used nuclear fuel cladding. This hydride reorientation is influenced by various key factors such as circumferential stress (hoop stress) due to internal rod pressure, maximum temperature reached, cooling rate during storage, and the concentration of precipitated hydrogen during irradiation. To simulate long-term dry storage of used nuclear fuel, hydrogenated Zircaloy-4 cladding (CWSRA) specimens were used in hydride reorientation tests under various hoop stress conditions (70, 80, 90, and 110 MPa) for extended cooling periods (3 months, 6 months, and 12 months). After the hydride reorientation tests, the cladding’s offset strain (%) was evaluated through a ring compression test, a mechanical property test encompassing both ductility and brittleness. In this study, the offset deformation of the hydride reorientation specimens was compared and evaluated through ring tensile tests. In this study, the offset deformation values were compared and evaluated through ring tensile tests of the hydride reorientation test specimens. Hydrogen in zirconium cladding reduces ductility from a physical perspective and induces rapid plastic deformation. Generally, even in hydrogenated unirradiated cladding, it maintains a tensile strength of around 800 MPa at room temperature. However, high hydrogen content accelerates plastic deformation. In contrast, samples with radial hydrogen distribution exhibit fracture behavior in the elastic region below 500 MPa. This is attributed to the directional of radial hydrogen distribution. Specimens with a hydrogen concentration of 200 ppm fracture faster than those with hydrogen concentrations exceeding 400 ppm. This is believed to be due to the ease of reorientation of radial hydrogen in cladding with relatively low hydrogen content. Although the consistency of the test results is not ideal, ongoing research is needed to identify trends in hydride reorientation from a cladding perspective.
        228.
        2023.11 구독 인증기관·개인회원 무료
        Currently, the Korea Atomic Energy Research Institute is conducting research on the development of technology to reduce the disposal area for SF (Spent nuclear Fuel). If the main radionuclides contained in SF can be separated and recovered according to their characteristics (long half-life, high mobility and high heat load) and uranium oxide which is expected to be the final residue, can be made into solids, the burden of the permanent disposal area of the SF will be greatly reduced. The waste form that end up in the repository must be verified for ease of manufacture and stability of the block. And, in order to increase the loading efficiency, a large block manufacturing technology is needed. This study describes the background of introducing PSA (Particle Size Analyzer) which is one of the necessary equipment for manufacturing UO2 blocks using slip casting, the method of using the equipment and performance verification of the equipment using standard samples. The particle size affects the sintering quality by the way the particles rearrange themselves during sintering. Powders of small particles are generally less free flowing and more difficult to compress, they form thin pores between the particles and sinter to higher density. In contrast, larger particle has a lower sintered density. Therefore, accurate particle size measurement and the selection of a suitable particle size are important. For this purpose, a PSA was installed in nuclear cycle experiment research center. To verify the performance of the equipment, a standard sample of 1.025 μm was analyzed. We got an average particle size of 1.0293 μm and standard deviation of 0.0668 μm. This value was within the uncertainty(±0.018 μm) of the sample’s certificate. In the future, this equipment will measure the size of UO2 (depleted uranium) powder and to produce large scale uranium oxide blocks.
        229.
        2023.11 구독 인증기관·개인회원 무료
        Pyroprocessing technology has emerged as a viable alternative for the treatment of metal/oxide used fuel within the nuclear fuel cycle. This innovative approach involves an oxide reduction process wherein spent fuel in oxide form is placed within a cathode basket immersed in a molten LiCl-Li2O salt operating at 923 K. The chemical reduction of these oxide materials into their metallic counterparts occurs through a reaction with Li metal, which is electrochemically deposited onto the cathode. However, during process, the generation of Li2O within the fuel basket is inevitable, and due to the limited reduction efficiency, a significant portion of rare earth oxides (REOx) remains in their oxide state. The presence of these impurities, specifically Li2O and REOx, necessitates their transfer into the electrorefining system, leading to several challenges. Both Li2O and REOx exhibit reactivity with UCl3, the primary electrolyte within the electrorefining system, causing a continuous reduction in UCl3 concentration throughout the process. Furthermore, the formation of fine UO2 powder within the salt system, resulting from chemical reactions, poses a potential long-term operational and safety concern within the electrorefining process.Various techniques have been developed to address the issue of UO2 fine particle removal from the salt, utilizing both chemical and mechanical methods. However, it is crucial that these methods do not interfere with the core pyroprocessing procedure. This study aims to investigate the impact of Li2O and REOx introduced from the electrolytic reduction process on the electrorefining system. Additionally, we propose a method to effectively eliminate the generated UO2 fine powder, thereby enhancing the long-term operational stability of the electrorefining process. The efficiency of this proposed solution in removing oxidized powder has been confirmed through laboratory-scale testing, and we will provide a comprehensive discussion of the detailed results.
        230.
        2023.11 구독 인증기관·개인회원 무료
        Once discharged, spent nuclear fuel undergoes an initial cooling process within deactivation pools situated at the reactor site. This cooling step is crucial for reducing the fuel’s temperature. Once the heat has sufficiently diminished, two viable options emerge: reprocessing or interim storage. A method known as PUREX, for aqueous nuclear reprocessing, involves a chemical procedure aimed at separating uranium and plutonium from the spent nuclear fuel. This separation not only minimizes waste volume but also facilitates the reuse of the extracted materials as fuel for nuclear reactors. The transformation of uranium oxides through dissolution in nitric acid followed by drying results in uranium taking the form of UO2(NO3)2 + 6H2O, which can then be converted into various solid-state configurations through different heat treatments. This study specifically focuses on investigating the phase transitions of artificially synthesized UO2(NO3)2 + 6H2O subjected to heat treatment at various temperatures (450, 500, 550, 600°C) using X-ray Diffraction (XRD) analysis. Heat treatments were also conducted on UO2 to analyze its phase transformations. Additionally, the study utilized XRD analysis on an unidentified oxidized uranium oxide, UO2+X, and employed lattice parameters and Bragg’s law to ascertain the oxidation state of the unknown sample. To synthesize UO2(NO3)2 + 6H2O, U3O8 powder is first dissolved in a 20% HNO3 solution. The solid UO2(NO3)2 + 6H2O is obtained after drying on a hotplate and is subsequently subjected to heat treatment at temperatures of 450, 500, 550, and 600°C. As the heat treatment temperature increases, the color of the samples transitions from orange to dark green, indicating the formation of different phases at different temperatures. XRD analysis confirms that uranyl nitrate, when heattreated at 500 and 550°C, oxidizes to UO3, while the sample subjected to 600°C heat treatment transforms into U3O8 due to the higher temperature. All samples exhibit sharp crystal peaks in their XRD spectra, except for the one heat-treated at 450°C. In the second experiment, the XRD spectra of the heat-treated UO2 consistently indicate the presence of U3O8 rather than UO3, regardless of the temperature. Under an oxidizing atmosphere within a temperature range of 300 to 700°C, UO2 can be oxidized to form U3O8. In the final experiment, the oxidation state of the unknown UO2+X was determined using Bragg’s law and lattice parameters, revealing that it was a material in which UO2 had been oxidized, resulting in an oxidation state of UO2.24.
        231.
        2023.11 구독 인증기관·개인회원 무료
        Molten salt reactor (MSR) uses fluoride or chloride based molten salt as a coolant of the system, and fuel materials are dissolved in the molten salt, therefore it can be act as both coolant and nuclear fuel. A few issues have arisen from early-stage research and development program of MSR from Oak Ridge National Laboratory, including corrosion of structural materials and fission product management. For investigating the effect of additives on corrosion of structural materials, Mg(OH)2 and MgCl2*6H2O are added into the NaCl-MgCl2 eutectic salt. Prepared chloride salt is injected into the autoclave in the glove box, as well as corrosion coupons for candidate structural materials for molten chloride salt reactor, SS316, Alloy 600, and C-276 are also prepared. The temperature is set as 700°C. After 500 h corrosion experiment, the samples are taken out from the autoclave, and they are analyzed with scanning electron microscopy (SEM) and energy-dispersive X-ray spectroscopy (EDS). SS316 samples show weight loss with all salt conditions, while Alloy 600 and C-276 show weight gain after the corrosion experiment.
        232.
        2023.11 구독 인증기관·개인회원 무료
        This study investigated the effectiveness of various chlorinating agents in partitioning light water reactor spent fuel, with the aim of optimizing the chlorination process. Through thermodynamic equilibrium calculations, the effects of using MgCl2, NH4Cl, and Cl2 as a single chlorinating agent or applying MgCl2, NH4Cl, and Cl2 sequentially for spent fuel chlorination were evaluated Furthermore, in this study, assuming the actual process operation situation, where only a part of the semi-volatile nuclides is removed during the heat treatment process, and including the process of precipitating the molten salt from the chlorination process with K3PO4 and K2CO3 precipitants, the percentage distribution of 50 nuclides in the light water reactor spent fuel into each process stream was quantitatively calculated using the simulation function of the HSC program and tabulated for intuitive viewing. Compared to a single chlorinator, sequential chlorination more effectively separated the heat and radioactivity of the spent fuel from the uranium-dominated product solids. Specifically, the sequential application of the chlorinating agents following heat treatment led to a final solid separation characterized by 93.1% mass retention, 5.1% radioactivity, and 15.4% decay heat, relative to the original spent fuel. The findings underscore that sequential chlorination can be an effective method for spent fuel partitioning, either as a standalone approach or in combination with other partitioning processes such as pyroprocessing.
        233.
        2023.11 구독 인증기관·개인회원 무료
        In the establishment of procedures for managing spent fuel, the development of an information system for data management is an indispensable prerequisite. Given the prolonged period of spent nuclear fuel management, marked by numerous personnel changes and the anticipation of vast data retention, addressing this matter appropriately is imperative, particularly in the specialized field of spent nuclear fuel operations. Recognizing the need for a method to mitigate these challenges, we endeavored to apply semantic technology to the information system. To achieve this, we constructed the ontology of spent nuclear fuel and conducted research to transform it into a relational database. As a result, the information system, developed by the application of semantic technology, has attained the capability to comprehend and perceive relationships among information itself. Through this research, the system not only addresses previously identified concerns but also enhances its versatility, enabling it to perform functions previously unattainable within existing information systems.
        234.
        2023.11 구독 인증기관·개인회원 무료
        In Korea, Kori Unit 1 and Wolsong Unit 1, have been permanently shut down in 2017 and 2019, and more nuclear power plants are expected to be permanently shut down after continued operation successively. Spent fuel has been generated during operation and stored in spent fuel pools. Due to the expected saturation of spent fuel pools within the next several decades, transportation of a huge amount of spent fuel is anticipated to interim storage facilities or final disposal facilities, even though the specific location is not decided. The U.S. Nuclear Regulatory Commission (NRC) states that every environmental report prepared for the licensing stage of a Pressurized Water Reactor shall contain a statement concerning risk during the transportation of fuel and radioactive wastes to and from the reactor. Thus, the licensee should ensure that the radiological effects in accidents, as well as normal conditions in transport, do not exceed certain criteria or be small if cannot be numerically quantified. Specific conditions that a full description and detailed analysis of the environmental effects of transportation of fuel and wastes to and from the reactor are exempted are specified in 10 CFR Part 51. Since there are no official requirements for radiological dose assessment for workers and public during the transportation of spent fuel in Korea, the margin when applying the U.S. regulatory criteria to the environmental impact assessment during the transport of spent fuel generated from domestic nuclear power plants is evaluated. A different approach would be needed due to the difference in the characteristics of spent fuel and geographical features.
        235.
        2023.11 구독 인증기관·개인회원 무료
        Korea has an agreement for cooperation with 31 countries, including the United States, Canada, Australia, and Japan. Under the agreement, the obligated items must be used for peaceful purposes, comply with nuclear non-proliferation and international safeguards, and obtain prior consent of shipment in case of enrichment, reprocessing, retransfer. Among them, the United States, Canada, and Australia have signed Administrative Arrangements of Cooperation Agreements (Supplementary Arrangements in Canada) for the international transfer and annual reports of obligated items. When operators submit an annual report, the government compiles and make the annual report based on the data. Ideally, the final report is submitted by the operator should be the national annual report, but in practice, discrepancies occur between sum of the operator’s and goverment’s. In order to resolve these problems and strengthen the linkage between exports contrpol and safeguards, our institute has begun the project to develop an ‘Obligation Tracking System for internationally controlled items (OTS)’. It is believed that obligated items which are unnecessarily included or omitted in annual report could be managed properly by developing OTS for life cycle of the items such as import, disposal/ termination or transfer to other countries. In case of nuclear material, especially, the characteristics of the facilities (e.g., bulk-handling facilities) must be considered and principles of fungibility, equivalence, and proportionality should be applied to materials. In order to computerize these procedures, we would like to propose to adopt the format of Code 10 for obligated item management. Code 10 is the form of the annex to the Korea-IAEA safeguards agreement which includes all records of inventory changes, import/export, and domestic movement of nuclear materials. It is expected to minimize discrepancies between operators’ annual reporting data and national annual reporting and further contribute to enhancing national trust and nuclear transparency.
        236.
        2023.11 구독 인증기관·개인회원 무료
        Nuclear Forensics is recognized as a essential component in the nuclear non-proliferation verification sector by the international community. It is being advanced under the leadership of the IAEA, the U.S., and the EU. Both the U.S.’s Lawrence Livermore National Laboratory (LLNL) and the international collaborative organization, the Nuclear Forensics International Technical Working Group (ITWG), have proposed to establish a relationship between the production timing and radiochronometry of nuclear materials or samples to utilize in the field of nuclear forensics. Radiochronometry of nuclear materials is calculated based on the Bateman equation, incorporating factors with uncertainties derived from tests, experiments, and analyses. The results from the nuclear activity radiochronometry also encompass uncertainties, affecting their reliability. This study examined the mathematical uncertainty calculations related to the results of nuclear activity radiochronometry, focusing on calculation methods, contribution rates per factor, and sensitivities. Uncertainty factors for the Bateman equation-based radiochronometry were observed in the decay constants for each nuclide type and the uncertainty in the radioactive ratio of the tracer nuclide. The sensitivity for each factor revealed that the uncertainty in the radioactive ratio of the signature nuclide contributed more significantly than the uncertainty in decay constants for each nuclide type. Each factor displayed a distinct sensitivity curve relative to the radioactive ratio. As it approaches a radioactive equilibrium, the sensitivity tends to increase infinitely, indicating a corresponding trend of infinite increase in uncertainty. Because the time and curve shape to reach radioactive equilibrium vary depending on the signature nuclide, it’s essential to choose an appropriate signature nuclide based on the anticipated period and analysis requirements for nuclear activity radiochronometry. However, radiochronometry using mathematical methods is limited to the relationship between parent and daughter nuclides, presenting the potential for underestimation of uncertainty factors like decay constants. Future research will need to focus on uncertainty calculation methods through computational simulations, especially using the Monte Carlo method, to overcome the limitations of mathematical approaches and potential underestimations.
        237.
        2023.11 구독 인증기관·개인회원 무료
        Strategic item export control aims to maintain international peace and safety and serves as a significant nuclear non-proliferation regime that directly impacts a nation’s security. Therefore, establishing an autonomous export control system at the state level is crucial, and one of the most efficient methods to achieve this is by enhancing an export company’s management system. Accordingly, many advanced countries, such as the United States, Europe, and Japan, have operated their own internal compliance programs (CP or ICP) to manage and screen the export of strategic items as a corporate social responsibility and risk mitigation measure. In Korea, which has a high dependence on trade, the need for CP was continuously confirmed, but the system was introduced in 2004, relatively late compared to other advanced countries. So far, the Korean government has made steady efforts to develop and establish the system and is actively encouraging businesses to obtain Compliance Program certification to autonomously manage strategic items. Major technologically advanced countries utilize technology transfer as a tool for economic sanctions, trade security, and strategic technology management, and they continue to strengthen their control regimes. In these countries, CP certification is considered a standard practice for export control among mid-sized and large enterprises. It serves as a vital risk management system that protects companies from unforeseen incidents. However, in Korea, the application of CP under the Foreign Trade Act is limited to dual-use items and does not extend to the nuclear export control system. Therefore, this paper analyzes international cases and CP requirements in countries like the United States, Japan, Europe, and Singapore. As a result of the review, the application of CP into Korea’s nuclear export control could be a coexistence means that can strengthen supply chain control as well as provide benefits not to impede technical research, international trade, and exchanges.
        238.
        2023.11 구독 인증기관·개인회원 무료
        The Republic of Korea (ROK), as a member state of the IAEA, is operating the State’s System of Accounting for and Control (SSAC) and conducting independent national inspections. Furthermore, an evaluation methodology for the material unaccounted for (MUF) is being developed in ROK to enhance capabilities of national inspection. Generally, physical and chemical changes of nuclear material are unavoidable due to the operating system and structure of facilities, an accumulation of material unaccounted for (MUF) has been issued. IAEA developed statistical MUF evaluation method that can be applied to all facilities around the world and it mainly focuses on the diversion detection of nuclear materials in facilities. However, in terms of the national safeguard inspection, an evaluation of accountancy in facilities is additionally needed. Therefore, in this research, a new approach to MUF evaluation is suggested, based on the Guide to the Expression of Uncertainty in Measurement (GUM) that an evaluation of measurement uncertainty factors is straightforward. A hypothetical list of inventory items (LII) which has 6,118 items at the beginning and end of the material balance period, along with 360 inflow and outflow nuclear material items at a virtual fuel fabrication plant was employed for both the conventional IAEA MUF evaluation method and the proposed GUM-based method. To calculate the measurement uncertainty, it was assumed that an electronic balance, gravimetry, and a thermal ionization mass spectrometer were used for a measurement of the mass, concentration, and enrichment of 235U, respectively. Additionally, it was considered that independent and correlated uncertainty factors were defined as random factors and systematic factors for the ease of uncertainty propagation by the GUM. The total MUF uncertainties of IAEA (σMUF) and GUM (uMUF) method were 37.951 and 36.692 kg, respectively, under the aforementioned assumptions. The difference is low, it was demonstrated that the GUM method is applicable to the MUF evaluation. The IAEA method demonstrated its applicability to all nuclear facilities, but its calculated errors exhibited low traceability due to its simplification. In contrast, the calculated uncertainty based on the GUM method exhibited high reliability and traceability, as it allows for individual management of measurement uncertainty based on the facility’s accounting information. Consequently, the application of the GUM approach could offer more benefits than the conventional IAEA method in cases of national safeguard inspections where factor analysis is required for MUF assessment.
        239.
        2023.11 구독 인증기관·개인회원 무료
        SMR, which has recently been in the spotlight, has several advantages. However, it poses additional challenges in the areas of new design, digitalization, security, safety and safeguards. Among them, security refers to measures to protect nuclear materials and facilities from unauthorized access, theft, or destruction. Safeguards refer to measures to prevent the spread of nuclear weapons. The relationship between security and safeguards is complex and constantly evolving. In general, security measures are designed to protect nuclear materials and facilities from physical attack, while safeguards are designed to track and monitor the movement of nuclear materials and prevent them from being used to create nuclear weapons. In some areas security and safeguards work in complementary ways, and in other areas they conflict. But ultimately, finding a balance is what is effective and efficient. In conclusion, although the security and safeguards of SMRs have different key objectives, they are closely related and must be implemented comprehensively and consistently to ensure the safety of nuclear facilities, the public, and the environment. In this paper, we investigate how the safety and safeguards of SMR are currently being researched and analyze what difficulties there are when assuming that they are operated as a single interface.