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        검색결과 1,288

        61.
        2023.11 구독 인증기관·개인회원 무료
        The saturation of wet storage facilities constructed and operated within nuclear power plant sites has magnified the significance of research concerning the dry storage of spent nuclear fuel. Not only do wet storage facilities incur higher operational and maintenance costs compared to dry storage facilities, but long-term storage of metal-clad fuel assemblies submerged in aqueous tanks is deemed unsuitable. Consequently, dry storage is anticipated to gain prominence in the future. Nevertheless, it is widely acknowledged that quantitatively assessing the residual water content remains elusive even when employing the apparatus and procedures utilized in the existing dry storage processes. The presence of residual water can only be inferred from damage or structural alterations to the spent nuclear fuel during its dry storage, making precise prediction of this element crucial, as it can be a significant contributor to potential deformations and deterioration. The aforementioned challenges compound the issue of retrievability, as substantial complexities emerge when attempting to retrieve spent nuclear fuel for permanent disposal in the future. Consequently, our research team has established a laboratory-scale vacuum drying facility to investigate the sensitivity of various parameters, including canister volume, pump capacity, water surface area, and water temperature, which can exert thermohydraulic influences on residual water content. Moreover, we have conducted dimensional analysis to quantify the thermohydraulic effects of these parameters and express them as dimensionless numbers. These analytical approaches will subsequently be integrated into predictive models for residual water content, which will be further developed and validated at pilot or full-scale levels. Furthermore, our research team is actively engaged in experimental investigations aimed at fine-tuning the duration of the pressure-holding phase while optimizing the evaporation process under conditions designed to avert the formation of ice caused by abrupt temperature fluctuations. Given that the canister is constructed from acrylic material, we are able to identify, from a phenomenological perspective, the specific juncture at which the boiling phenomenon becomes manifest during the vacuum drying process.
        62.
        2023.11 구독 인증기관·개인회원 무료
        International Atomic Energy Agency defines the term “Poison” as a substance used to reduce reactivity, by virtue of its high neutron absorption cross-section, in IAEA glossary. Poison material is generally used in the reactor core, but it is also used in dry storage systems to maintain the subcriticality of spent fuel. Most neutron poison materials for dry storage systems are boron-based materials such as Al-B Carbide Cermet (e.g., Boral®), Al-B Carbide MMC (e.g., METAMIC), Borated Stainless Steel, Borated Al alloy. These materials help maintain subcriticality as a part of the basket. U.S.NRC report NUREG-2214 provides a general assessment of aging mechanisms that may impair the ability of SSCs of dry storage systems to perform their safety functions during longterm storage periods. Boron depletion is an aging mechanism of neutron poison evaluated in that report. Although that report concludes that boron depletion is not considered to be a credible aging mechanism, the report says analysis of boron depletion is needed in original design bases for providing long-term safety of DSS. Therefore, this study aimed to simulate the composition change of neutron poison material in the KORAD-21 system during cooling time considering spent fuel that can be stored. The neutron source term of spent fuel was calculated by ORIGEN-ARP. Using that source term, neutron transport calculation for counting neutrons that reach neutron poison material was carried out by MCNP®-6.2. Then, the composition change of neutron poison material by neutron-induced reaction was simulated by FISPACT-II. The boron-10 concentration change of neutron poison material was analyzed at the end. This study is expected to be the preliminary study for the aging analysis of neutron poison material about boron depletion.
        63.
        2023.11 구독 인증기관·개인회원 무료
        After the Fukushima disaster, overseas nuclear power plants have established conditions for issuing a red alert in the event of fuel damage within the spent fuel pool and they have already implemented conditions for issuing a blue alert when fuel is exposed above the water surface. In South Korean nuclear power plants, a real-time monitoring system is in place to oversee the exposure of spent fuel to the surface within the spent fuel pool. To achieve this, a water level indicator gauge is installed within the spent fuel pool, allowing for continuous real-time monitoring. This paper conducted a comparative assessment of radiation levels from water level monitoring system in two units’ spent fuel pools based on the low water levels (1 feet from the storage rack), utilizing the radiation analysis code (MCNP).
        64.
        2023.11 구독 인증기관·개인회원 무료
        Due to the saturation of spent fuel pool of nuclear power plant in Korea, temporary storage for spent fuel will be installed, and spent fuel will be stored and managed in dry cask for a considerable period of time. Since spent nuclear fuel must withstand continuous decay heat, radiation and high internal pressure of the fuel rod in the cask, behavior of spent nuclear fuel is needed to be reviewed. Spent nuclear fuel used in Pressurized Water Reactor (PWR) in Korea is stored in a wet storage currently, but it is going to store a temporary dry-storage facility on Kori site. Therefore, it is very important and meaningful to evaluate the behavior of nuclear fuel with realistic modeling. Also, domestic PWR nuclear fuel has various burn-up. In the past, the burn-up of nuclear fuel in light water reactors was low, but in order to increase power generation efficiency, the concentration of uranium was increased and the number of new fuel was increased. Therefore, a large amount of nuclear fuel with burn-up of 45,000 MWD/MTU or higher, generally called high burn-up, is also stored in the spent fuel pool (SFP). Therefore, it is necessary to evaluate by dividing three different burn-up such as, low, medium, and high burn-up. Thus, this study will review the behavior of nuclear fuel at different burn-up during the temporary storage period with FALCON (EPRI), computational code and analyze the factors affecting the integrity of nuclear fuel, including when the temporary storage is extended its additional lifetime. And this evaluation will contribute developing the spent fuel management plan in Korea.
        65.
        2023.11 구독 인증기관·개인회원 무료
        After the decision of the Wolsong unit 1 permanent shutdown (2019), spent fuel stored in the spent fuel bay (hereafter, SFB) should be transported to a dry storage facility (MACSTOR or Canister) in order to decommission Wolsong unit 1. Accordingly, KHNP has established a shipment schedule for damaged fuel of Wolsong Unit 1 and is trying to complete the shipment according to the schedule. Wolsong is equipped with transportation casks and dry storage facilities, but baskets need to be manufactured separately. In addition, license approval is required for baskets, transport cask, and dry storage facilities for legal grounds to contain, transport, and store damaged fuels. In this paper, the initial model, upgrade model, and automation model of encapsulation equipment planned to be introduced in Canada to handle PHWR’s damaged fuel were compared, and the optimal model was selected in consideration of KHNP’s planned spent fuel shipment schedule. The PHWR’s damaged fuel encapsulation system is a system developed the PHWR’s damaged spent fuel to be handled in the same way as the existing PHWR when storing it in the dry storage facility and loading a basket for capsulation into transport cask. At the Gentilly-2 nuclear power plant in Canada, a manually operated encapsulation system was used due to the low quantity of damaged fuel, which can be encapsulated two bundles a day, and this model is an initial model. In the case of Wolsong Unit 1, it has about 300 damaged fuels, so it takes about nine months to work when using the initial model. The upgrade model developed to improve work efficiency and reliability has increased work efficiency through some automation, but it would take about eight months to process the damaged spent fuels of Wolsong Unit 1, and this model has not yet been manufactured and applied. Lastly, the automation model changed the work location outside the SFB and automated drainage/drying operations. It is easy to maintain and replace consumables because the work is carried out by lifting the damaged fuel to a shuttle outside the SFB surrounded by a shielding chimney. Considering the reduction of drainage/drying time, it is possible to save about four times as much time as the initial model. That is, if the automation model is used, it is judged that the supply of Wolsong Unit 1 can be processed in about two months. However, in terms of license, initial model and upgrade model are expected to be easier and the period is expected to be shortened. However, if licensing is carried out as soon as equipment design is completed, it is believed that the period can be shortened by parallel equipment manufacturing and licensing. It is judged that the best way to comply with the target schedule is to select an automation model with excellent work performance, develop equipment, and proceed with licensing at the same time. Accordingly, KHNP is in the process of designing equipment with the aim of using the automation model to take out damaged fuel for Wolsong Unit 1.
        66.
        2023.11 구독 인증기관·개인회원 무료
        On a global scale, the storage of spent nuclear fuel (SNF) within nuclear power plants (NPP) has become an important research topic due to limited space caused by approaching capacity saturation. SNF have e been collected over decades of NPP operation, coming up to capacity limitation. In case of Korea, every reactor except Saeul 1 and 2 has reached a SNF storage saturation rate of over 75%. One of the most studied methods for enhancing storage capacity efficiency involves increasing storage density using racks with neutron absorbers. Neutron absorbers like borated stainless steel (BSS) are utilized to manage the reactivity of densely stored SNF. However, major challenges of applying BSS are manufacturing hardness from heterogenous microstructure and mechanical property degradation from helium bubble formation. This study suggests that innovative fabrication methods of 3D printing can be good candidate for easier fabrication and better structural integrity of BSS. Directed energy deposition (DED), one of the 3D printing methods have become major candidate method for various alloys. It deposits alloy powder on base melt surface by high intensity laser, similar with welding process. Powder manufacturing is already demonstrated superior performance compared to casting in ASTM-A887, such as increased mechanical properties, owing to its well distributed chemistry of alloy. Moreover, as its original microstructural property, the formation of micro-pores through DED could lead to long-term performance improvements by capturing helium generated from the neutron absorption of boron. The potential for fabricating complex structure is also among the advantages of DED-produced neutron absorbers. Expected challenge on DED application on BSS is lack of printing condition data, because the 3D printing process have to be kept very careful variables of thermal intensity, powder flux and etc. These processes may get through much of trial & error for initial condition approaching. Nonetheless, as a recommendation of improved neutron absorber for efficient SNF pool storage, the concept of 3D printed BSS stands out as an intriguing avenue for research.
        67.
        2023.11 구독 인증기관·개인회원 무료
        More than 20,000 bundles of spent nuclear fuel are stored in the spent nuclear fuel storage pool of domestic nuclear power plants, and the dry storage facility project in the nuclear power plant site is being promoted as the saturation of the wet storage pool is imminent. Since bending or twisting of spent nuclear fuel is an important item in order to load spent nuclear fuel into a dry storage cask, PSE (Pool Side Examination) was performed to verify this. This paper describes whether it can be safely loaded into a dry storage cask based on the measurement results of bending or twisting of spent nuclear fuel. The nuclear fuel assembly is designed to prevent excessive assembly bending and twisting because it can cause interference during dry storage and handling due to factors such as differences in depletion of nuclear fuel rods, irradiation growth, and coolant flow during reactor operation. The bending of the nuclear fuel assembly is measured by establishing a Plumb Line to photograph the nuclear fuel assembly based on it, and calculating a pixel that images the distance between the support grid and the Plumb Line. The twisting of the nuclear fuel assembly is measured by forming a virtual vertical plane with two Plumb Lines, and based on this, the twisting angle of the lower fixed compared to the upper fixed. As a result of the measurement, the bending of spent nuclear fuel was about 0.0-10.2 mm, much lower than the reactor loading criteria of 15.0 mm, and in the case of twisting, about 0.0~2.2° much lower than the reactor loading criteria of 5.0°. Therefore, it was confirmed that spent nuclear fuel at domestic nuclear power plants was not affected by bending and twisting when loading into dry storage cask.
        68.
        2023.11 구독 인증기관·개인회원 무료
        In Korea, most temporary storage facilities for spent nuclear fuel are nearing saturation. As an alternative to this, the 2nd basic plan for high-level radioactive waste management specified the operation plan of dry interim storage facility. Meanwhile, the NSSC No. 2021-19 stipulates that it is necessary to evaluate the possibility and potential effect of accident before operating interim storage facility. Therefore, this study analyzed the categories of accident scenarios that may occur in dry storage facility as part of prior research on this. We investigated the case of categorization of dry storage facility accident scenarios of IAEA, NRC, KAREI, and KINS. The IAEA presented accident scenarios that could occur in on-site dry storage facility operated with silo and cask method. NRC has classified accident scenarios in dry storage facility and estimated the probability of accidents for each. KAERI and KINS selected major accident scenarios and analyzed the processes for each, in preparation for the introduction of dry storage facility in Korea in the future. Overall, a total of 10 accident scenarios were considered, and the scenarios considered by each institution were different. Among 10 scenarios, cask drop and aircraft collision were included in the categorization of most institutions. The results of this study can be used as basic data for cataloging accidents subject to safety evaluation when introducing dry interim storage facility in Korea in the future.
        69.
        2023.11 구독 인증기관·개인회원 무료
        In KNF, fuel performance analysis modules were developed to predict the overall behavior of a fuel rod under normal operating conditions. Their main focus is to provide information on initial conditions prior to dry storage. Potential degradation mechanisms that may affect sheath integrity of spent CANDU fuel during dry storage are: creep rupture under internal gas pressure, sheath oxidation in air environment, stress corrosion cracking, delayed hydride cracking, and sheath splitting due to UO2 oxidation for a defective fuel. To upgrade the developed modules that address all the damage mechanisms, the first step was a review of the available technical information on phenomena relevant to fuel integrity. The second step was an examination of the technical bases of all modules, identify and extend the ranges of all modules to required operating ranges. The 300°C spent CANDU fuel sheath temperature metric for dry storage ensures spent CANDU fuel element integrity from the failure mechanisms of creep rupture, oxidation and stress corrosion cracking at a failure probability of 2×10-5 for a dry storage time of 100 years. The 300°C sheath temperature metric for dry storage has relatively a lower failure rate than the target criteria for dry storage of spent LWR fuel. Although different modes of failure were treated separately for simplicity, ignoring possible synergistic effects, these results are conservative because of the conservative assumptions that have been made for evaluating spent fuel element conditions, and because of the inherent conservatism of the applied models. Additional conservatism of the model comes from the fact that isothermal conditions do not prevail in actual storage conditions. Further R&D being considered includes acquisition of new functional models to implement overall fuel behavior evaluation and cover spent CANDU fuel in dry storage, and upgrades of the analysis module to achieve sufficient accuracy in key output parameters. The developed modules provide a platform for research and industrial applications, including the design of fuel behavior experiments and prediction of safe operating margins for spent CANDU fuel.
        70.
        2023.11 구독 인증기관·개인회원 무료
        This study investigated the effectiveness of various chlorinating agents in partitioning light water reactor spent fuel, with the aim of optimizing the chlorination process. Through thermodynamic equilibrium calculations, the effects of using MgCl2, NH4Cl, and Cl2 as a single chlorinating agent or applying MgCl2, NH4Cl, and Cl2 sequentially for spent fuel chlorination were evaluated Furthermore, in this study, assuming the actual process operation situation, where only a part of the semi-volatile nuclides is removed during the heat treatment process, and including the process of precipitating the molten salt from the chlorination process with K3PO4 and K2CO3 precipitants, the percentage distribution of 50 nuclides in the light water reactor spent fuel into each process stream was quantitatively calculated using the simulation function of the HSC program and tabulated for intuitive viewing. Compared to a single chlorinator, sequential chlorination more effectively separated the heat and radioactivity of the spent fuel from the uranium-dominated product solids. Specifically, the sequential application of the chlorinating agents following heat treatment led to a final solid separation characterized by 93.1% mass retention, 5.1% radioactivity, and 15.4% decay heat, relative to the original spent fuel. The findings underscore that sequential chlorination can be an effective method for spent fuel partitioning, either as a standalone approach or in combination with other partitioning processes such as pyroprocessing.
        71.
        2023.11 구독 인증기관·개인회원 무료
        A lot of CANDU Spent Fuels (CSFs) have been stored in spent nuclear fuel pools and dry storage facilities. In accordance with the enhanced nuclear regulations, the initial characteristics of CSF should be inspected to ensure the integrity of CSF and the reliable operation of storage system before loading it into a cask for long-term dry storage. For the inspections, an initial characteristics measurement equipment was designed, which is used for Pool-Side Examination (PSE) in the spent fuel pool of the pressurized heavy water reactor nuclear power plant. Measurements using the equipment consist of non-contact inspections and contact inspections. The non-contact inspections do not affect CSF integrity, whereas the integrity of CSF can be reduced during the contact inspections under abnormal operating conditions because the probe of equipment may apply specific loads to the CSF. Therefore, the structural integrity evaluations of equipment and CSF are performed using Finite Element (FE) analyses for four combinations based on two abnormal conditions and two probe positions. The used abnormal conditions are the pressing load condition and the scratching load condition, and two probe positions are the center and bottom of the fuel rod in the longitudinal direction, respectively. In this evaluation, the bottoms of the fuel rod or CSF are defined as the regions facing the bottom surface of equipment. The analysis of the pressing load condition is performed by pressing the probe of the equipment in radial direction of the CSF fuel rod. That of the scratching load condition is carried out by applying a specific radial load to the CSF fuel rod using the probe and then applying the load to the surface of the fuel rod while moving axially along the surface. All combinations are analyzed considering geometric, boundary and material non-linearity under the dynamic load, which is dependent on the equipment operating velocity. The stresses of CSF and equipment components were obtained from these analyses. The maximum stress of each component was generated at the combination on the scratching load condition for the bottom position among the four combinations. The obtained maximum stresses are lower than the yield stress for each component material. Also, the CSF is not overturned due to the support plate of the equipment in all analyses. Therefore, the structural integrity and safety of the equipment and the CSF are maintained under abnormal operating conditions during the inspection using the initial characteristic measurement equipment.
        72.
        2023.11 구독 인증기관·개인회원 무료
        In the case of dry storage facilities, slipping of the cask or tip-over are dangerous phenomena. For this reason, in dry storage facilities, measures against slipping and tip-over or related safety evaluations are important. Accidental conditions that can cause cask slippage and tip-over in dry storage facilities include natural phenomena such as floods, tornadoes, tsunamis, typhoons, earthquakes, and artificial phenomena such as airplane crashes. However, among natural phenomena, earthquakes are the most important natural phenomenon that causes tip-over. Also, many people had the stereotype that Korea is an earthquake-safe zone before 2016. However, earthquakes become a major disaster in Korea due to the 2016 Gyeongju earthquake and the 2017 Pohang earthquake, followed by the Goesan earthquake in October 2022. In this paper, seismic analysis was performed based on dry storage facilities including multiple casks. Design variables for the construction of an analysis model for dry storage facilities were investigated, and seismic analysis was performed. To evaluate tip-over accident during earthquake, seismic load was used from 0.2 g PGA to 0.8 g PGA and these earthquakes were followed Design Response Spectrum (DRS) in RG 1.60. The friction coefficient of concrete pad was used from 0.2 to 1.0. As a result of the analysis, tip-over accident could not find in the analysis from 0.2 g to 0.6 g. However, tip-over was appeared at friction coefficients of 0.8 and 1.0 at 0.8 g PGA. Tip-over angular velocity of cask was derived by seismic analysis and was compared with formula and tip-over analysis results. As a result, a generalized dry storage facility analysis model was proposed, and dry storage facility safety evaluation was conducted through seismic analysis. Also, tip-over angular velocity was derived using seismic analysis for tip-over analysis.
        73.
        2023.11 구독 인증기관·개인회원 무료
        In nuclear facilities, a graded approach is applied to achieve safety effectively and efficiently. It means that the structures, systems, and components (SSCs) that are important to safety should be assured to be high quality. Accordingly, SSCs that consist of nuclear facilities should be classified with respect to their safety importance as several classes, so that the requirements of quality assurance relevant to the designing, manufacturing, testing, maintenance, etc. can be applied. Guidance for the safety classification of SSCs consisting of nuclear power plants and radioactive waste management facilities was developed by U.S.NRC and IAEA. Especially, in guidance for nuclear power plants, safety significance can be evaluated as following details. The single SSC that mitigates or/and prevents the radiological consequence or hazard was assumed to be failure or malfunction as the initiating event/accident occurred and the following radiological consequence was evaluated. Considering both the consequence and frequency of the occurrence of the initiating event/accident, the safety significance of each SSC can be evaluated. Based on the evaluated safety significance, a safety class can be assigned. The guidance for the safety classification of the spent nuclear fuel dry storage systems (DSS) was also developed in the United States (NUREG/CR-6407) and the U.S.NRC acknowledges the application of it to the safety classification of DSS in the United States. Also, worldwide including the KOREA, that guidance has been applied to several DSSs. However, the guidance does not include the methodology for classifying the safety or the evaluated safety significance of each SSC, and the classification criteria are not based on quantitative safety significance but are expressed somewhat qualitatively. Vendors of DSS may have difficulties to apply this guidance appropriately due to the different design characteristics of DSSs. Therefore, the purpose of this study is to evaluate the safety significance of representative SSCs in DSS. A framework was established to evaluate the safety significance of SSCs performing safety functions related to radiation shielding and confinement of radioactive materials. Furthermore, the framework was applied to the test case.
        74.
        2023.11 구독 인증기관·개인회원 무료
        In the establishment of procedures for managing spent fuel, the development of an information system for data management is an indispensable prerequisite. Given the prolonged period of spent nuclear fuel management, marked by numerous personnel changes and the anticipation of vast data retention, addressing this matter appropriately is imperative, particularly in the specialized field of spent nuclear fuel operations. Recognizing the need for a method to mitigate these challenges, we endeavored to apply semantic technology to the information system. To achieve this, we constructed the ontology of spent nuclear fuel and conducted research to transform it into a relational database. As a result, the information system, developed by the application of semantic technology, has attained the capability to comprehend and perceive relationships among information itself. Through this research, the system not only addresses previously identified concerns but also enhances its versatility, enabling it to perform functions previously unattainable within existing information systems.
        75.
        2023.11 구독 인증기관·개인회원 무료
        In Korea, Kori Unit 1 and Wolsong Unit 1, have been permanently shut down in 2017 and 2019, and more nuclear power plants are expected to be permanently shut down after continued operation successively. Spent fuel has been generated during operation and stored in spent fuel pools. Due to the expected saturation of spent fuel pools within the next several decades, transportation of a huge amount of spent fuel is anticipated to interim storage facilities or final disposal facilities, even though the specific location is not decided. The U.S. Nuclear Regulatory Commission (NRC) states that every environmental report prepared for the licensing stage of a Pressurized Water Reactor shall contain a statement concerning risk during the transportation of fuel and radioactive wastes to and from the reactor. Thus, the licensee should ensure that the radiological effects in accidents, as well as normal conditions in transport, do not exceed certain criteria or be small if cannot be numerically quantified. Specific conditions that a full description and detailed analysis of the environmental effects of transportation of fuel and wastes to and from the reactor are exempted are specified in 10 CFR Part 51. Since there are no official requirements for radiological dose assessment for workers and public during the transportation of spent fuel in Korea, the margin when applying the U.S. regulatory criteria to the environmental impact assessment during the transport of spent fuel generated from domestic nuclear power plants is evaluated. A different approach would be needed due to the difference in the characteristics of spent fuel and geographical features.
        76.
        2023.11 구독 인증기관·개인회원 무료
        The types of fuel loaded and burned in domestic nuclear power plants are WH-type and OPR/ APR-type nuclear power plants, with a total of 19 types. In the case of spent nuclear fuel released in Korea, the low combustion level of 45,000 MWD/MTU or less accounts for about 75%. In terms of fuel type, WH 17×17 and CE 16×16 fuels account for about 85% of all spent nuclear fuels. The thickness of the oxide film of the fuel cladding can make the fuel rod vulnerable during reactor operation, directly affecting the integrity of the fuel rods. so, it is a very important design factor in design. Therefore, the fuel rod design code that predicts and evaluates this has also been developed to accurately predict fuel rod corrosion. And it’s being applied to the design. In this study, the ECT probe measured by inserting it between fuel rods. The thickness of the fuel cladding oxide film was measured for spent nuclear fuel. When reloading operational nuclear fuel, the IAEA recommends an oxide film thickness of up to 100 micrometers. In this study, it was confirmed that spent nuclear fuels keeping integrity burned for 2-3 cycles were sufficiently maintained within the limit. However, the difference could be confirmed according to the characteristics of the coating material, the combustion cycle, and the use of poison rods. For the reliability of the data, symmetrical to the quadrant fuels were selected, and the fuel burned at the same period was measured. The method of selecting the target fuel can produce meaningful results.
        77.
        2023.11 구독 인증기관·개인회원 무료
        In pyroprocessing, the residual salts (LiCl containing Li and Li2O) in the metallic fuel produced by the oxide reduction (OR) process are removed by salt distillation and fed into electrorefining. This study undertook an investigation into the potential viability of employing a separate LiCl salt rinsing process as an innovative alternative to conventional salt distillation techniques. The primary objective of this novel approach was to mitigate the presence of Li and Li2O within the residual OR salt of metallic fuel, subsequently facilitating its suitability for electrorefining processes. The process of rinsing the metallic fuel involved immersing it in a LiCl salt environment at a temperature of 650°C. During this immersion process, the residual OR salt contained within the fuel underwent dissolution, thereby reducing the concentrations of Li2O and Li generated during the OR process. Furthermore, the Li and Li2O dissolved within the LiCl salt were effectively consumed through chemical reactions with ZrO2 particles present within the salt. Importantly, even after the metallic fuel had been subjected to rinsing in a conventional LiCl salt solution, the concentration of Li and Li2O within the salt remained consistent with its initial levels, due to the utilization of ZrO2. Moreover, it was observed that the Li- Li2O content within the metallic fuel was significantly diluted as a result of the rinsing process.
        78.
        2023.11 구독 인증기관·개인회원 무료
        The Fukushima-Daiichi accident in 2011 revealed the limitations of Zr-alloys in accident scenarios where severe steam oxidation led to the liberation of heat and hydrogen and the destruction of the reactor core. In response to this accident, there has been a concerted effort by industry, national laboratories, and universities to develop cladding and fuel materials for lightwater reactors (LWRs) that are more accident tolerant. The near-term approach has been to develop coatings for Zr-alloys that would provide additional safety and operational margin by virtue of its excellent corrosion/oxidation resistance at both normal and accident conditions. The designs being considered for implementation by major nuclear fuel suppliers include a thin Cr or a ceramic coating on the conventional LWR fuel cladding. For improved economics, the industries are also considering ATF coated cladding with high enrichment fuel (up to 8%) to achieve high burnup (> 75 GWd/MTU). While the development of ATF concepts (i.e., the front end of the fuel cycle), including coated claddings and doped fuels have progressed at an accelerated pace, relatively less attention has been devoted to the used fuel disposition of ATF fuels (i.e., the backend of the fuel cycle). For accelerated deployment of the ATF designs in the current LWR fleet, it is necessary to investigate technical aspects of the ATF used nuclear fuel (UNF) management in transportation, storage, and disposal. This presentation will provide a brief overview of state-of-the-art ATF developments and list out potential considerations to apply the fuels into back-end fuel cycle. New test plan should be planned to compare the characteristics of current LWR used nuclear fuels with those of the new fuel designs. For example, research focus can be understanding of ATF used fuel particulate size and quantity (at high burnup condition) and mechanical integrity of coated cladding under normal and off-normal conditions during transportation and long-term storage. Finally, the impacts of CRUD on the new fuel cladding, increased container weight, temperature, and radiation level to the back-end fuel cycle activities need to be investigated.
        79.
        2023.11 구독 인증기관·개인회원 무료
        Spent nuclear fuel continues to be generated domestically and abroad, and various studies are actively being conducted for interim dry storage and disposal of spent nuclear fuel. The characteristics vary depending on the type of spent nuclear fuel and the initial specifications, and based on these characteristics, it is essential to estimate the burnup and enrichment of spent nuclear fuel as a nondestructive assay. In particular, it is important to estimate the characteristics of spent nuclear fuel with non-destructive tests because destructive tests cannot be performed on all encapsulated spent nuclear fuel in case of intrusion traces in safeguards. Data is made by measuring spent nuclear fuel directly to evaluate burnup of spent nuclear fuel, but computer simulation research is also important to understand its characteristics because past burnup history is not accurately written, and destructive testing is difficult. In Sweden, the dependency of the burnup history in source strength and mass of light-water reactor-type spent nuclear fuel was evaluated, and this part was also applied to MAGNOX in consideration of the possibility of being used to verify DPRK’s denuclearization. SCALE 6.2 TRITON modeling was performed based on public information on DPRK’s 5 MWe Yongbyon reactor, and the source strength of Nb-95, Zr-95, Ru-106, Cs-134, Cs-137, Ce-141, Ce- 144, Eu-154 nuclides were evaluated. Since the burnup of MAGNOX is lower than that of lightwater reactors, major nuclides in decay heat were not considered. The cooling period was evaluated based on 0, 5, 10, and 20 years. In case the discharge timing was different, the total period of discharge and reloading was the same, and the end-cycle burnup was the same, calculations showed that the source strength emitted from major nuclides was evaluated within 2-3% except for Ru-106 and Ce-144 nuclides. Even the burnup step of nuclear fuel is the same, and the reloaded length after discharge is different, i.e., the cooling period between is different at 5, 10, and 20, the source strength of Nb-95, Zr-95, Ce-144, and Cs-137 was evaluated as an error of 1%. Except for Ru-106 and Ce-144, nuclides are highly dependent on burnup. Compared to the case of light-water reactors, the possibility of a decrease in error needs to be considered later because the specific power is low. As a result, radionuclides in released fuel depend on the effects of burnup, discharged and reloaded period, and a cooling period after release, and research is needed to correct the cooling period within the future burnup history. In addition, in this study, it is necessary to select a scenario -based burnup because the standard burnup due to the statistical treatment of discharged fuels was not considered as conducted in previous studies.
        80.
        2023.11 구독 인증기관·개인회원 무료
        As the demand for nuclear power increases as a means to achieve carbon neutrality, concerns about nuclear proliferation have also grown. Consequently, significant researches have conducted to enhance nuclear non-proliferation resistance. Among these research, nuclear material attractiveness is a methodology used to evaluate how appealing a particular material is for potential use in nuclear weapons, based on the characteristics of that material. Existing nuclear material attractiveness assessments focused on materials like U, Pu, and TRU, which could be directly used in the production of nuclear weapons. However, these assessments did not consider how the properties of nuclear materials change throughout the nuclear fuel cycle, with each facility process. This study assumed a scenario of the nuclear fuel cycle of graphite reduction reactors and analyzed including enrichment facilities and PUREX. This study used the FOM (Figure-Of-Merit) method developed by LANL (Los Alamos National Laboratory) for evaluating the nuclear material attractiveness. The FOM formula consists of three parameters such as critical mass, heat content, and dose The critical mass of targe materials and the dose evaluation were conducted using the Monte Carlo N-Particle code. The heat content was calculated using the ORIGEN code embedded in the Scale code. In particular, if U-238 is dominant in the facility’s materials, such as mining and refining facilities, and critical mass evaluation is unpractical. Therefore, 1SQ (Significant Quantity) of that uranium was assumed as the critical mass value for the FOM evaluation, even though 1SQ is not identical to the critical mass As a result of this study, the attractiveness of Pu produced by PUREX among all nuclear fuel cycle facilities was 2.7616, which was the most attractive to be diverted to nuclear weapons. Through this study, it was shown that the proliferation risk of the nuclear facilities in the nuclear fuel cycle and risk of diversion among those facilities.
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