비록 산화 그래핀의 비표면적은 환원된 산화 그래핀에 비해 낮지만, 산화 그래핀의 이산화탄소 흡착량은 기존 그 래핀 또는 환원된 산화 그래핀에 비해 많다. Lerf-Klinowski 모델에 따르면, 산화 그래핀은 가장 자리와 면 내부에 수산화기, 에폭시드, 카보닐, 카복실기 등이 있으며, 이러한 작용기가 이산화탄소 분자와 강하게 결합하여 화학 흡착을 유도한다. 본 연 구에서는 산소 플라즈마/UV 오존 및 열처리를 통해 그래핀 산화물의 산소 함량과 이산화탄소 흡착 친화도 사이의 상관관계 를 탐구하였다. 산소 함량의 변화는 XPS와 FT-IR 분석을 통해 확인하였다. 흥미롭게도 산화 그래핀의 이산화탄소 흡착 경향 은 전체 산소 함량과 정비례하지 않았다. 반면, XPS 분석 결과 산화 그래핀의 카보닐 작용기가 이산화탄소 흡착에 중요한 기 여를 하는 것으로 나타났다. 이러한 연구 결과는 산화 그래핀의 특성 및 이를 활용한 탄소 포집 및 가스 저장 응용 가능성에 대한 통찰을 제공한다.

본 연구는 인접하게 식재된 서어나무, 갈참나무, 졸참나무, 스트로브잣나무 조림지를 대상으로 2023년 3월부터 2024년 3월까지 낙엽·낙지 부위별 탄소 유입량을 1개월 단위로 조사하였다. 월별 낙엽·낙지에 의한 탄소 유입량의 경우 잎은 모든 수종에서 10월~11월 가장 높았으나 수종 간 최대 유입시기가 다르게 나타났다. 생식기관의 경우 스트로브잣나무는 6월 수꽃(웅화수, male flowers)에 의해, 졸참나무와 갈참나무는 4월과 5월 꽃뿐만 아니라 8월과 9월 도토리 등 종자에 의한 탄소 유입량이 높게 나타났다. 기타 물질에 의한 탄소 유입량은 11월 서어나무와 스트로브잣나무 조림지에서 높게 나타났으며 가지의 경우 불규칙한 월 변동을 보여 월별, 수종별 상호작용 모두 유의성이 없었다(P>0.05). 본 연구에 따르면 낙엽·낙지에 의한 부위별 탄소 유입량은 월별 또는 조림지 간 유의적인 차이(P<0.05)를 나타냈음에도 불구하고 연간 총 탄소 유입량은 조림지 간 유의적인 차이가 없었다(P>0.05).

탄소흡수원으로서 천연활엽수림의 역할이 강조되고 있으나, 다양한 수종과 다양한 입지 환경으로 인하여 정확한 탄소저장량을 추정하는 것은 어려운 과제 중 하나로 인식되고 있다. 본 연구는 강원도 평창군 가리왕산의 천연활엽수림의 주요 수종인 신갈나무(Quercus mongolica), 고로쇠나무 (Acer pictum subsp. mono), 물푸레나무(Fraxinus rhynchophylla)를 대상으로 임목 바이오매스, 낙엽 탄소저장량, 토양 탄소저장량을 비교하고, 임분의 다양한 특성과 탄소저장량과의 관계를 파악하기 위하여 수행되었다. 총 43개 조사구를 구획하였으며, 임목 바이오매스, 낙엽 탄소저장량, 토양 탄소저장량을 측정하였다. 임목 바이오매스의 탄소저장량은 신갈나무 우점 임분에서 172.64tC/ha로 가장 높게 나타났으며, 고로쇠나무 임분 (170.98tC/ha), 물푸레나무 임분(170.49tC/ha)순으로 나타났다. 토양 탄소저장량은 신갈나무 우점 임분에서 78.07tC/ha으로 다른 임분에 비해 유의적으로 높게 나타났으며, 낙엽의 탄소저장량은 임분 간 유의한 차이를 보이지 않았다. 총 탄소저장량은 신갈나무 임분에서 258.79tC/ha으로 가장 높게 나타났으며, 고로쇠나무 임분(257.65tC/ha), 물푸레나무 임분(241.65tC/ha) 순으로 나타났다. 총 탄소저장량은 임목 바이오매스의 탄소저 장량(r = 0.88**)과 토양 탄소저장량(r = 0.79**)의 영향을 모두 받는 것으로 나타났다. 본 연구는 천연활엽수림의 최적의 탄소 관리를 위해서는 임령, 임목 생장, 토양 특성 등에 대한 이해와 장기적 모니터링이 매우 중요함을 시사한다.

지속저인 산업발전은 화석 연료사용과 에너지 사용을 증가시켰으며, 각 국가별 온실가스 배출은 증가하고 있는 실정이다. 국제사회는 지구 온난화 방지를 위해 1997년 교토 의정서를 채택하였고, 이산화탄소(CO2) 순 배출량 0을 목표로 하여 자체적으로 온실가스 배출 목표를 정하고 실천하고자 2015년 '파리기후변화협정'을 채택하였다. 우리나라는 2015년 '파리기후변화협정' 체결 후 2030년까지 2017년 총 배출량 대비 24.4 % 감축을 목표로 설정하였다.(외교부, 2020) 국내 사회 각 분야에서는 온실가스 감축을 위해 노력하고 있으며, 도로분야에서는 온실가스 저감을 위한 환경친화형 도로 설계와 시 공기술 개발을 위한 연구들이 검토되고 있다. 그 중 가열 아스팔트 혼합물 제조 시 사용되는 기존의 연료(중유, 벙커씨유, 정제유 등) 를 상대적으로 탄소배출량이 적은 연료(LPG, LNG)로 전환하거나, 플랜트 생산온도를 낮추어 사용되는 연료를 저감하는 방법 등 다양 한 연구를 진행하고 있다. 따라서 본 연구에서는 일반 가열 아스팔트 혼합물보다 약 50℃ 낮은 상태에서 생산할 수 있게 도와주는 탄소저감형 첨가제를 적용 한 저가열 아스팔트의 특성을 파악하고자 하였다. 기본 물성시험으로는 연화점, 신도, 회전점도를 시험하였으며, 공용성 등급 시험을 통하여 PG 등급을 확인하였다. 또한 기존에 상용화된 제품과 차이를 보기 위해, 첨가제가 투입되지 않은 일반 아스팔트와 중온 첨가 제 2종(고상형, 액상형)이 적용된 중온 아스팔트도 동일한 시험을 진행하였고, 저가열 아스팔트와 비교·분석 하였다.

To analyse the relationship between above-ground carbon stocks, species diversity and broadleaved forests structural diversity of South Korean forests, we collected vegetation inventories from environmental impact assessment projects over the past 10 years. The available data were selected and organised including tree species, DBH and area each projects. The data was classified by forest type, aboveground carbon stocks were calculated and compared, and the correlation between aboveground carbon stocks and biodiversity and structural diversity was analysed. The results showed that above-ground carbon stocks were higher in mixed forests and broadleaved forests and lower in needleleaved forests, similar to previous studies. However aboveground carbon stocks of mixed forests were higher in natural forests than in plantations. Aboveground carbon stocks in broadleaved forests were higher in plantations than natural forests, and there was no statistical different of between natural and plantations in needleleaved forest. This could be the result of a variety influences including biological and environmental factors in the study area, and further research is needed to analyse the effects on carbon sequestration. Correlation analysis showed no correlation between biodiversity and above-ground carbon stocks, but a positive correlation between structural diversity and above-ground carbon stocks. This indicates that above-ground carbon stocks in forests are associated with unevenness diameters and the proportion and evenness of tree species by diameter. In addition, it has been analysed that the high succession stages in forest have higher species diversity and structural diversity, and greater efficiency in the utilization of resources required for plant growth, leading to increased plant productivity and storage. Considering that the study sites were young forests with an average DBH of 14.8~23.7 cm, it is expected that carbon stocks will increase as biodiversity and structural diversity increase. Further research is needed to develop techniques to quantitatively assess the relationship of diversity to carbon stocks for policy use in assessing and increasing carbon stocks in forests.

As global climate change impacts become more apparent, countries are implementing various policies to achieve carbon neutrality that can be categorized into direct regulations and market-based indirect regulations. The latter, utilizing economic incentives, is considered more efficient in transforming corporate behavior and promoting voluntary efforts for carbon reduction. In alignment with international trends, South Korea has introduced the Emission Trading System (ETS) in 2015. Despite this, the domestic carbon market remains underdeveloped, with low ETS participation, particularly in the aquaculture sector. In order to activate external projects under the ETS, this study proposes short-term strategies including linking ETS with popular eco-friendly energy distribution projects, developing standardized monitoring techniques, and integrating carbon reduction initiatives with other support mechanisms such as direct payment programs. Long-term strategies focus on developing new methodologies for external projects, promoting the use of renewable energy, and enhancing technologies to reduce energy consumption in aquaculture operations. By implementing these strategies, the study aims to enhance the participation of the aquaculture sector in carbon reduction efforts, contributing to the overall goal of carbon neutrality.

본 연구는 한국에서 시행 중인 탄소배출권 거래제도가 탄소중립을 달 성하는데 효과적으로 기여하고 효율적으로 작동할 수 있도록 정책적 시 사점을 제공하고자 한다. 이를 위해서, 탄소배출권 가격과 전산업생산지 수의 관계를 분석하였다. 즉, 탄소배출권 가격과 전산업생산지수의 선형 및 비선형 관계를 고려하여 경제학적 모형을 통해 추정 및 분석을 진행 하였다. 분석 방식은 구조변화를 반영한 방식과 임계값(문턱값)을 반영하 는 방식으로 나누어 모형을 구축하고 추정하였다. 그 결과, 한국의 탄소 배출권 가격과 전산업생산지수는 추정한 모형에서 비선형적 관계가 포착 되었다. 이러한 결과는 한국에서 시행 중인 탄소배출권 거래제도가 효율 적으로 작동할 수 있도록 추가적인 정책이 필요함을 시사한다. 예를 들 어, 산업 분야에서 저탄소 공정으로의 전환(또는 저탄소 경제로의 전환) 이 완전히 이루어지지 않은 현실을 고려할 때, 여전히 경제가 성장하는 상황에서 비선형 관계가 포착된다는 것은 탄소배출권 가격이 적정한 수 준을 유지하지 못하고 지속적으로 하락하는 추세를 나타낸다는 것이기 때문이다. 따라서, 탄소배출권 거래제도의 본래 취지인 탄소배출량의 감 축에 기여할 수 있도록 적정한 탄소배출권 가격이 배출권 거래제도하에 서 유지되도록 하는 정책을 고려해야 한다.

In this paper, the adsorption removal characteristic for 10 species of perfluoroalkyl and polyfluoroalkyl substances (PFAS) was investigated using GAC and modified GAC (GAC-Cu). After modification with Cu(II), the amount of copper was to 1.93 and 4.73 mg/g for GAC and GAC-Cu, respectively. The total amount of 10 species of PFAS per specific area was obtained to 0.548 and 0.612 ng/m2 for GAC and GAC-Cu, respectively. A series of batch test confirmed lower efficiency was observed with a smaller number of carbon chain length and the removal efficiency of PFCA (perfluoroalkyl carboxylic acids) was lower than that of PFSA (perfluoroalkyl sulfonic acids) with the same carbon chain length. Regarding the pH effect, the adsorption capacity was decreased with increase of pH due to the increase of electrostatic repulsion. According to pseudo first and second order (PFO and PSO) kinetic models, while the values of equilibrium uptake and time did not show significant difference, a difference in uptake was observed between 24-48h. Furthermore, based on correlation analysis, Log Kow and uptake have a high correlation with molecular weight (M.W.) and initial concentration, respectively. These results show that long-chain PFAS have higher removal efficiency due to their increased hydrophobicity.

PURPOSES : This study aimed to evaluate the performance of carbon-reduced asphalt mixtures based on asphalt binder and asphalt mixture tests. METHODS : A carbon-reducing asphalt additive was developed, and samples were prepared by mixing the additive(0.85%, 1.35%, and 1.85%) with virgin asphalt binder to measure changes in the asphalt’s physical properties based on the content of the developed additive. The basic physical properties the penetration, softening point, ductility, and rotational viscosity and performance grade of the samples were measured, and the optimal content of the additive was determined to be 1.35%. An asphalt mixture was produced using the optimal additive content of 1.35%, and stability, indirect tensile strength, tensile strength ratio(TSR), and dynamic stability tests were conducted to compare its performance with that of hot mixed asphalt(HMA). Additionally, a dynamic modulus test that could simulate various loading conditions was conducted. Fuel consumption and CO2 emission were measured at the plant. RESULTS : The developed additive had the effect of reducing the viscosity of the binder while maintaining properties similar to those of the base binder when used at the selected content. The mixture test confirmed that the physical properties related to strength tended to decrease slightly when the additive were applied; however, all specifications were satisfied. In the dynamic modulus test, the results were confirmed to be similar to those of HMA. The fuel consumption and CO2 emission were reduced by 25-30%. CONCLUSIONS : Evidently, asphalt mixtures with carbon-reducing additives can perform at a level equivalent to that of HMA. To bolster this conclusion, it is necessary to track the long-term performance of low-carbon asphalt mixtures on pilot roads.

In the present study, a coal-based pitch containing 12.1% quinoline insoluble (QI) underwent isothermal heat treatment, and changes in the mesophase microstructure were analyzed for the heat treatment duration. The nuclei creation and growth rate of mesophase were affected by the distribution of QI particles in the pitch. The growth process could be explained in four regions through the mesophase area fraction. During the carbonization of carbon blocks, mesophase formation was induced in the binder phase. The physical properties of carbon blocks were measured as a function of residence time. As residence time increased, bulk density decreased and porosity increased, but electrical conductivity increased. It was determined that forming a mesophase in the binder phase during carbonization reduced the size of large pores in carbon block and improved the connectivity between particles, thereby increasing electrical conductivity. These results are expected to show greater improvement in electrical properties after graphitization.

One of the key challenges for the commercialization of carbon nanotube fibers (CNTFs) is their large-scale economic production. Among CNTF spinning methods, surfactant-based wet spinning is one of the promising techniques for mass producing CNTFs. Here, we investigated how the coagulation bath composition affects the spinnability and the properties of CNTFs in surfactant-based wet spinning. We used acetone, DMAc, ethanol, and IPA as coagulants and analyzed the relationship between coagulation bath composition and the properties of CNTFs in terms of kinetic and thermodynamic coagulation parameters. From a kinetic perspective, we found that a low mass transfer rate difference (MTRD) is favorable for wet spinning. Based on this finding, we mixed the coagulant bath with solvent in a proper ratio to reduce the MTRD, which generally improved the wet spinning. We also showed that the coagulation strength, a thermodynamic parameter, should be considered. We believe that our research can contribute to establishment of surfactant-based wet spinning of CNTFs.

Electrochemical water splitting presents an optimal approach for generating hydrogen ( H2), a highly promising alternative energy source. Nevertheless, the slow kinetics of the electrochemical oxygen evolution reaction (OER) and the exorbitant cost, limited availability, and susceptibility to oxidation of noble metal-based electrocatalysts have compelled scientists to investigate cost-effective and efficient electrocatalysts. Bimetallic nanostructured materials have been demonstrated to exhibit improved catalytic performances for the oxygen evolution reaction (OER). Herein, we report carbon aerogel (CA) decorated with different molar ratios of Fe and Ni with enhanced OER activity. Microwave irradiation was involved as a novel strategy during the synthesis process. Inductively coupled plasma mass spectrometry (ICP-MS), X-ray diffraction (XRD), X-ray Photoelectron Spectroscopy (XPS), Scanning Electron Microscope (SEM), Energy dispersive X-ray spectroscopy (EDAX spectra and EDAX mapping), Transmission Electron Microscope (TEM), High-Resolution Transmission Electron Microscope (HR-TEM), and Selected Area Electron Diffraction (SAED) were used for physical characterizations of as-prepared material. Electrochemical potential towards OER was examined through cyclic voltammetry (CV), chronoamperometry, and electrochemical impedance spectroscopy (EIS). The FeNi/CA with optimized molar ratios exhibits low overpotential 377 mV at 10 mAcm− 2, smaller Tafel slope (94.5 mV dec− 1), and high turnover frequency (1.09 s− 1 at 300 mV). Other electrocatalytic parameters were also calculated and compared with previously reported OER catalysts. Additionally, chronoamperometric studies confirmed excellent electrochemical stability, as the OER activity shows minimal change even after a stability test lasting 3600 s. Moreover, the bimetallic (Fe and Ni) carbon aerogel exhibits faster catalytic kinetics and higher conductivity than the monometallic (Fe), which was observed through EIS investigation. This research opens up possibilities for utilizing bi- or multi-metallic anchored carbon aerogel with high conductivities and exceptional electrocatalytic performances in electrochemical energy conversion.

Carbon foam composites containing hollow microspheres, reinforced by carbon nanotubes (CNTs) and montmorillonite (MMT), have been developed as the thermal insulation and EMI shielding layer. The effects of additive amounts of CNTs/ MMT on microstructure and properties of the carbon foam composites were investigated. Results showed that carbon foam composites had hierarchical porous structure, with CNTs and MMT being relatively uniformly dispersed in the composites. The addition of multiscale additives improved the mechanical, electromagnetic shielding effectiveness and thermal insulation properties of carbon foam composites. The composites containing 0.2 wt.% CNTs and 5 wt.% MMT, showed outstanding compressive strength, up to 8.54 MPa, increased by 116% to pure carbon foam. Their electromagnetic shielding effectiveness was as high as 65 dB, increased by 75%. Due to the hierarchical porous structure and MMT’s heat barrier effect, carbon foam composites presented remarkable thermal insulation properties. The minimum thermal conductivity was 0.45 W·m−1·K−1 at 800 °C. Their exceptional thermal protection can also be evidenced by ablation resistance under flame at 1000 °C. Therefore, such multifunctional carbon-based composites are ideal for use in thermal protection.

This study pioneers a transformative approach of discarded orange peels (Citrus sinensis) into highly porous carbon, demonstrating its potential application in energy storage devices. The porous carbon structure offers a substantial surface area, making it conducive for effective ion adsorption and storage, thereby enhancing capacitance. The comprehensive characterization, including X-ray diffraction, Fourier transform infrared, Raman spectroscopy, field emission scanning electron microscopy, and XPS verifies the material’s suitability for energy storage applications by confirming its nature, functional groups, graphitic structure, porous morphology and surface elemental compositions. Moreover, the introduced plasma treatment not only improves the material’s intensity, bending vibrations, and morphology but also increases capacitance, as evidenced by galvanostatic charge–discharge tests. The air plasma-treated carbon exhibits a noteworthy capacitance of 1916F/g at 0.05A/g in 2 M KOH electrolyte. long term cyclic stability has been conducted up to 10,000 cycles, the calculated capacitance retention and columbic efficiency is 92.7% and 97.6%. These advancements underscore the potential of utilizing activated carbon from agricultural waste in capacitors and supercapatteries, offering a sustainable solution for energy storage with enhanced performance characteristics.

Moso bamboo, as a kind of renewable functional material, exhibits outstanding development potential. It is promising to prepare activated carbon with good mechanical strength and high specific surface area using moso bamboo as raw material. In this work, we employed a hydraulic extruder to extrude the bamboo charcoal and the adhesive to obtain the moso bamboo activated carbon, and improved the specific surface area of the columnar activated carbon through high-temperature water vapor activation. Through the catalytic role of the water vapor activation process, the formation and expansion of the pores were promoted and the internal pores were greatly increased. The obtained columnar activated carbon shows excellent mechanical strength (93%) and high specific surface area (791.54 m2/ g). Polyacrylamide@asphalt is one of the most effective adhesives in the high-temperature water vapor activation. The average pore size (22.99 nm) and pore volume (0.36 cm3/ g) of the prepared columnar activated carbon showed a high mesoporous ratio (83%). Based on the excellent pore structure brought by the activation process, the adsorption capacity of iodine (1135.75 mg/g), methylene blue (230 mg/g) and carbon tetrachloride (64.03 mg/g) were greatly improved. The resultant moso bamboo columnar activated carbon with high specific surface area, excellent mechanical properties, and outstanding adsorption capacity possesses a wide range of industrial applications and environmental protection potential.

This study comprehensively investigates three types of graphite materials as potential anodes for potassium-ion batteries. Natural graphite, artificial carbon-coated graphite, and mesocarbon microbeads (MCMB) are examined for their structural characteristics and electrochemical performances. Structural analyses, including HRTEM, XRD, Raman spectroscopy, and laser particle size measurements, reveal distinct features in each graphite type. XRD spectra confirm that all graphites are composed of pure carbon, with high crystallinity and varying crystal sizes. Raman spectroscopy indicates differences in disorder levels, with artificial carbon-coated graphite exhibiting the highest disorder, attributed to its outer carbon coating. Ex-situ Raman and HRTEM techniques on the electrodes reveal their distinct electrochemical behaviors. MCMB stands out with superior stability and capacity retention during prolonged cycling, attributed to its unique spherical particle structure facilitating potassium-ion diffusion. The study suggests that MCMB holds promise for potassium-ion full batteries. In addition, artificial carbon-coated graphite, despite challenges in hindering potassium-ion diffusion, may find applications in commercial potassium-ion battery anodes with suitable coatings. The research contributes valuable insights into potassiumion battery anode materials, offering a significant extension to the current understanding of graphite-based electrode performance.

In this study, polyimide (PI)-based activated carbon fibers (ACFs) were prepared for application as electrode materials in electric double-layer capacitors by varying the steam activation time for the PI fiber prepared under identical cross-linking conditions. The surface morphology and microcrystal structural characteristics of the prepared PI-ACFs were observed by field-emission scanning electron microscopy and X-ray diffractometry, respectively. The textural properties (specific surface area, pore volume, and pore size distribution) of the ACFs were calculated using the Brunauer–Emmett–Teller, Barrett–Joyner–Halenda, and non-local density functional theory equations based on N2/ 77 K adsorption isotherm curve measurements. From the results, the specific surface area and total pore volume of PI-ACFs were determined to be 760–1550 m2/ g and 0.36–1.03 cm3/ g, respectively. It was confirmed that the specific surface area and total pore volume tended to continuously increase with the activation time. As for the electrochemical properties of PI-ACFs, the specific capacitance increased from 9.96 to 78.64 F/g owing to the developed specific surface area as the activation time increased.

We successfully synthesized a porous carbon material with abundant hexagonal boron nitride (h-BN) dispersed on a carbon matrix (p-BN-C) as efficient electrocatalysts for two-electron oxygen reduction reaction ( 2e− ORR) to produce hydrogen peroxide ( H2O2). This catalyst was fabricated via ball-milling-assisted h-BN exfoliation and subsequent growth of carbon structure. In alkaline solutions, the h-BN/carbon heterostructure exhibited superior electrocatalytic activity for H2O2 generation measured by a rotating ring-disk electrode (RRDE), with a remarkable selectivity of up to 90–97% in the potential range of 0.3–0.6 V vs reversible hydrogen electrode (RHE), superior to most of the reported carbon-based electrocatalysts. Density functional theory (DFT) simulations indicated that the B atoms at the h-BN heterostructure interface were crucial active sites. These results underscore the remarkable catalytic activity of heterostructure and provide a novel approach for tailoring carbon-based catalysts, enhancing the selectivity and activity in the production of H2O2 through heterostructure engineering.

In this paper, the formation and characterization of Pt2, Pt3 as well as Pt4 atomic clusters in cup-stacked carbon nanotubes (CSCNTs) are evaluated by DFT to examine the adsorption capacity under the clusters. The results show that the Pt clusters move toward the bottom edge or form rings in the optimized stable structure. Pt far from the carbon substrate possesses more active electrons and adsorption advantages. The three clusters can adsorb up to 17, 18, and 16 hydrogen molecules. Loading metal clusters at the bottom edge maintains a relatively good adsorption property despite the low binding energy through comparative studies. The adsorption capacity does not increase with the number of Pt for metal aggregation reducing the hydrogen adsorption area thus impacting the hydrogen storage ability and the aggregation phenomenon limiting the action of Pt metal. During adsorption, chemisorption occurs only in the Pt2 cluster, while multiple hydrogen molecules achieve physiochemical adsorption in the Pt3 and Pt4 clusters. Compared with the atomic loading of the dispersion system in equal quantities, the dispersion system features higher molecular stability and can significantly reduce the energy of the carbon substrates, providing more sites for hydrogen adsorption in space.

The electrochemical properties of a CFX cathode were improved by defluorination of the surface with a N2 plasma and using a silica wafer. Compared to the N2 plasma treatment alone, when the CFX and silica were reacted together, the C-F bonds were modified and the surface was etched efficiently, so defluorination was enhanced. An electrochemical analysis confirmed that Half-cells prepared by treating CFx and silica with nitrogen plasma exhibited a capacity of about 400 mAh/g at 5C. In addition, it was confirmed that the loss of charge transfer was reduced by up to 71% compared to that for pristine CFX. As shown by a GITT analysis, when the CFx and silica were treated with N2 plasma together, the ion conductivity gradually increased due to a decrease in the ion diffusion barriers and the formation of a carbon layer. Therefore, this is a simple and effective way to improve the conductivities of CFX cathode materials with the energy of a N2 plasma and the silica-fluorine reaction.