검색결과

검색조건
좁혀보기
검색필터
결과 내 재검색

간행물

    분야

      발행연도

      -

        검색결과 5,398

        122.
        2023.11 구독 인증기관·개인회원 무료
        Molten Salt Reactor, which employs molten salt mixture as fuel, has many advantages in reactor size and operation compared to conventional nuclear reactor. In developing Molten Salt Reactor, the behavior of fission product in operation should be preliminary evaluated for the correct design of reactor and its associated system including off-gas treatment. In this study, for 100 Mw 46 KCl- 54 UCl3 based Molten Salt Reactor with operating life time of 20 year, the fission product behavior was estimated by thermodynamic modeling employing FactSage 8.2. Total inventory of all fission product were firstly calculated using OpenMC code allowing depletion during neutronic calculation. Then, among all inventory, 46 element species from Uranium to Holmium were chosen and given to the input for equilibrium module of Factsage with its mass. In phase equilibrium calculation, for the correct description of solution phase, KCl-UCl3 solution database based on modified quasichemical model in the quadruplet approximation (ANL/CFCT-21/04) was employed and the coexisting solid phase was assumed to pure state. With the assumption of no oxygen and moisture ingress into reactor system, equilibrium calculation showed that 1% of solid phase and of gas phase were newly formed and, in gas phase, major species were identified : ZrCl4 (47%), Xe (33%), UCl4 (14%), Kr (5%), Ar (1%) and others. This result reveals that off-gas treatment of system should account for the appropriate treatment of ZrCl4 and UCl4 besides treatment of noble gas such as Xe and Kr.
        123.
        2023.11 구독 인증기관·개인회원 무료
        Most of the C-14 produced is in the organic form, generated as methane (14CH4), methanol (14CH3OH), formaldehyde (14CH2O), and formic acid (14CO2H2). When analyzing C-14, it is transformed into the form of 14CO2, and its concentration is determined using LSC. Typical examples include the wet oxidation method, the combustion or Pyrolysis. The wet oxidation method uses strong acids and involves repeated operations, which generates large amounts of acid waste and secondary radioactive waste. The combustion method uses high temperatures, which requires an oxygen device. Pyrolysis also requires high temperature in a vacuum and catalysts. Catalysts are expensive because they are platinum-based. To compensate for these shortcomings, a C-14 analysis method using UV irradiation was developed. In this study, 100 mL of distilled water mixed with formic acid (CO2H2), potassium persulfate (K2S2O8), and silver nitrate (AgNO3) was irradiated with a 320-390 nm UV lamp to conduct a CO2 production reaction experiment. The UV range was measured using a photometer (UV Power puck II). The beaker was made of quartz in 150 mL size with three inlets : a temperature measurement, a sample inlet, and a collection tube connector. We changed the UV lamp used from a 450 W halogen lamp to a 100 W LED, which has a lower temperature and is safer. As a result of the experiment, CO2 bubbles were generated in the collection tube, due to the UV irradiation react, which uses oxidizer and catalysts. The maximum temperature of the solution irradiated with the LED UV lamp was less than 56°C. It confirmed the rate of bubble generation changed depending on the lamp distance, the amount of sample, oxidizer, and catalyst. In an experiment to confirm the reaction caused by heat, it was found that although a reaction occurred due to heat, the reaction was significantly lower than when using a UV lamp. The reproducibility experiment was conducted three times in total under the same conditions. It showed the same pattern. In the future, we plan to select mock samples, collect 14CO2 in Carbo- Sorb, and analyze them using LSC. The results of this research will be used as a technology to recover C-14 more safely and efficiently and will also be used to expand its application to the treatment of other wastes such as waste liquid and waste resin through simulated samples.
        124.
        2023.11 구독 인증기관·개인회원 무료
        Molten Salt Reactor (MSR) is one of the 4th generation nuclear power systems which is its verified technology in physically and chemically. Among the various salts used for MSR system, the eutectic composition of NaCl-MgCl2 system maintains the liquid state at around 450°C, in the same time, it has high solubility for nuclear fuel chlorides. This characteristic has high advantage for lowering the operating temperature for the MSR, which could reduce the problem of hightemperature corrosion by salt for structural materials significantly. In particular, since MgCl2 has the similar standard reduction potential with nuclear fuel, is used as a surrogate for, many basic researches have been conducted for verifying characteristic of MgCl2. It is well-known that main short-advantage of MgCl2 is hygroscopic properties. MgCl2 changes to MgCl2-xH2O state easily by absorbing moisture in air condition. The hydrated MgCl2 is producing MgOHCl by thermally decomposing at high temperature, the formed MgOHCl corrodes structural materials, even small amount of MgOHCl gives significant damage. Therefore, the purification of MgCl2 has been required for long-term operation of MSR using MgCl2 as a base salt. In this study, the purification of eutectic composition salt for NaCl-MgCl2 has been mainly performed by considering its thermodynamic properties and electrochemical characteristic, and the experimental results have been discussed.
        125.
        2023.11 구독 인증기관·개인회원 무료
        In the decommissioning process of nuclear power plants, Ni-59, Ni-63 and Fe-55 present in radioactive waste are crucial radionuclides used as fundamental indicators in determining waste treatment methods. However, due to their low-energy emissions, the chemical separation of these two radionuclides is essential compared to others. Therefore, this study aims to evaluate the suitability of various pre-treatment methods for decommissioning waste materials by conducting characteristic assessments at each chemical separation stage. The goal is to find the most optimized pre-treatment method for the analysis of Ni-59, Ni-63 and Fe-55 in decommissioning waste. The comparative evaluation results confirm that the chemical separation procedures for Fe and Ni are very stable in terms of stepwise recovery rates and the removal of interfering radionuclides. However, decommissioning waste materials, which mainly consist of concrete, metals, etc., possess unique properties, and a significant portion may be low-radioactivity waste suitable for on-site disposal. Considering that the chemical behavior and reaction characteristics may vary at each chemical separation stage depending on the matrix properties of the materials, it is considered necessary to apply cascading chemical separation or develop and apply individual chemical separation methods. This should be done by verifying and validating their effectiveness on actual decommissioning waste materials.
        126.
        2023.11 구독 인증기관·개인회원 무료
        To ensure the maintenance of the nuclear emergency response system, it is important to periodicaly conduct hazard assessments using up-to-date input variables. The results of this review are apllied to drills and exercises, enabling the inspection of emergency plan and response procedures. Therefore, this study aims to analyze off-site consequences according to the occurrence time of the Design Basis Accident (DBA) for the Hanaro Fuel Fabrication Facility (HFFF) by using the recent site-specific meteorological data and to review the appropriateness of urgent protective measures. MELCOR and SafeHanaro computer codes were used for radiation source-term estimation and environmental impact assessment, respectively. It was assumed that radioactive materials are released into environment for 2 hours due to the fire during the nuclear fuel sieving process. The following 12 scenarios for each occurrence time period was selected (0 am, 2 am, 4 am, 6 am, 8 am, 10 am, 12 pm, 2 pm, 4 pm, 6 pm, 8 pm, 10 pm) and the effective dose and thyroid dose in earlyand intermediate-phase were assessed. As a result, the most severe exposure-induced accident scenario is found to be as occurring at 0 am on July 15th, with the Most Exposed Individual (MEI) positioned 200 meters downwind from the facility. The committed effective dose for MEI is identified as to be 2.97E-02 mSv which has a significant margin against the IAEA's (Generic Intervention Level) GIL and (Generic Criteria) GC. During the passage of the radio-active plume, the estimated effective dose and thyroid dose due to inhalation were 2.97E-02 mSV (99.99%) and 5.06E-05 mSv (99.77%), respectively. External exposure appeared to be negligible. Meanwhile, the thyroid dose is noticeably below the criteria for decision-making for distribution of Potassium Iodide (KI). Accordingly, in order for local residents to participate in the exercise and drills, it is essential to develop scenarios considering simultaneous emergencies at multi-facilities and latenight accidents. In conclusion, this results will be used to improve the exercise plans for enhancing the nuclear or radiological emergency competencies of the KAERI.
        127.
        2023.11 구독 인증기관·개인회원 무료
        The inorganic scintillator used in gamma spectroscopy must have good efficiency in converting the kinetic energy of charged particles into light as well as high light output and high light detection efficiency. Accordingly, various studies have been conducted to enhance the net-efficiency. One way to improve the light yield has been studied by coating scintillators with various nanoparticles, so that the scintillation light can undergo resonance on surface between scintillators and nanoparticles resulting in higher light yield. In this study, an inorganic scintillator coated with CsPbBr3 perovskite nanocrystals using dip coating technique was proposed to improve scintillation light yield. The experiment was carried out by measuring scintillation light output, as the result of interaction between inorganic scintillator coated with CsPbBr3 perovskite nanocrystals and gamma-ray emitted from Cs-137 gamma source. The experimental results show that the channel corresponding to 662 keV full energy peak in the Cs-137 spectrum shifted to the right by 14.37%. Further study will be conducted to investigate the detailed relationships between the scintillation light yield and the characteristics of coated perovskite nanoparticles, such as diameter of nanoparticles, coated area ratio and width of coated region.
        128.
        2023.11 구독 인증기관·개인회원 무료
        The nuclear power plant (NPP) decommissioning market is expected to expand not only domestically but also overseas. Proven technologies must be applied to decommission NPP. This is based on Article 41-2, Paragraph 2 of the domestic ‘Enforcement Decree Of The Nuclear Safety Act’. Proven technology refers to technology that has verified that it can be applied in the field through demonstration. In other words, in order to carry out NPP decommissioning, verification must be done. Demonstration refers to reducing technological uncertainty and directly verifying services implemented in the field. From a technology commercialization perspective, demonstration requires an approach based on technology readiness level (TRL) from a technology perspective and market readiness level (MRL) from a market perspective. The characteristics of demonstration also differ depending on the characteristics of each field. The demonstration in the field of nuclear energy is the demonstration of demand matching. This is to confirm the feasibility of the technology in the company’s required environment. In order to perform demonstration, a scenario must be derived by reflecting demonstration design considerations. After evaluating the derived scenario, an actual assessment is conducted using lab-based demonstration/virtual environment demonstration/real environment demonstration. What must be preceded by an actual assessment is confirming the consumer’s requirements. In this study, the necessary environment and requirements of consumer’s to perform NPP decommissioning were reviewed. The domestic decommissioning procedure requirements management system presents decommissioning procedures, potential worker accidents, and worker requirements. In the case of foreign countries, it was confirmed that complex wide need, cost benefit, risk reduction, waste generation, operation, reliability and maintenance (RAM) improvement and quantitative measures were evaluated for the technology to be demonstrated. Also the requirements for demonstrating decommissioning need to a detailed review of actual decommissioning cases. Therefore, a comparison must be made between the requirements based on actual NPP decommissioning cases and the requirements derived from this research process. Afterwards, the empirical research approach proposed by the Ministry of Trade, Industry and Energy was applied. The empirical research approach proposed by the Ministry of Trade, Industry and Energy is to secure a track record over a certain period of time and performance under conditions similar to the actual environment in the final research stage at the TRL level 6 to 8. Through this, it will be possible to confirm the suitability of overseas technology for domestic application.
        129.
        2023.11 구독 인증기관·개인회원 무료
        When dismantling a power plant, a large amount of radioactive tanks are generated, and it is estimated that a significant amount of sludge will accumulate inside the tanks during long-term operation. In the process of dismantling a radioactive tanks, it is important to know the composition of the sludge because the sludge present inside must first be removed and then disposed of. In the case of certain tanks, it can be predicted that corrosion products generated due to system corrosion are the main cause of sludge formation. However, in the case of some tanks, it is not easy to predict the sludge composition because various dispersed particles in addition to corrosion products may be mixed with the wastewater. Even if it is collected and analyzed, the sludge composition can change significantly depending on the operation history, so the analysis results cannot be considered representative of the composition. In the case of LHST, surfactant components introduced during the washing and shower process, oil components and dispersed particles dissolved by the surfactant accumulate inside the tank, making sludge difficult to remove. In addition, even if it is removed by ultra-high pressure spraying, unexpected problems may occur in the subsequent treatment process due to the surfactant contained therein. Therefore, it is necessary to analyze in more detail the characteristics of sludge accumulated in LHST and prepare countermeasures. A test procedure was prepared to evaluate the characteristics of sludge accumulating in LHST. According to the test results, the long-term sludge accumulation tendency of the LHST is summarized as follows. ① Initially, the sludge settling speed increases slowly until a surface sludge layer is formed. ② After the surface sludge layer is formed, the sludge rapidly settles until the sludge layer becomes somewhat thicker. ③ When the sludge layer is formed to a certain extent, the sludge escape rate increases and the sludge accumulation rate decreases again. It is assumed that the sludge escape speed is closely related to the fluid flow speed in the relevant area. It is believed that the combined effect of these phenomena will determine the thickness of the sludge layer that will accumulate inside the tank, but it was not possible to evaluate how much the sludge layer would accumulate based on the experimental results alone. However, it can be assumed that significant sludge accumulation occurred in areas where fluid flow was minimal and sludge formation nuclei easily accumulates.
        130.
        2023.11 구독 인증기관·개인회원 무료
        Economical radioactive soil treatment technology is essential to safely and efficiently treat of high-concentration radioactive areas and contaminated sites during operation of nuclear power plants at home and abroad. This study is to determine the performance of BERAD (Beautiful Environmental construction’s RAdioactive soil Decontamination system) before applying magnetic nanoparticles and adsorbents developed by the KAERI (Korea Atomic Energy Research Institute) which will be used in the national funded project to a large-capacity radioactive soil decontamination system. BERAD uses Soil Washing Process by US EPA (402-R-007-004 (2007)) and can decontaminate 0.5 tons of radioactive soil per hour through water washing and/or chemical washing with particle size separation. When contaminated soil is input to BERAD, the soil is selected and washed, and after going through a rinse stage and particle size separation stage, it discharges decontaminated soil separated by sludge of less than 0.075 mm. In this experiment, the concentrations of four general isotopes (A, B, C, and D which are important radioisotopes when soil is contaminated by them.) were analyzed by using ICP-MS to compare before and after decontamination by BERAD. Since BERAD is the commercial-scale pilot system that decontaminates relatively large amount of soil, so it is difficult to test using radioactive isotopes. So important general elements such as A, B, C, and D in soil were analyzed. In the study, BERAD decontaminated soil by using water washing. And the particle size of soil was divided into a total of six particle size sections with five sieves: 4 mm, 2 mm, 0.850 mm, 0.212 mm, and 0.075 mm. Concentrations of A, B, C, and D in the soil particles larger than 4 mm are almost the lowest regardless of before and after decontamination by BERAD. For soil particles less than 4 mm, the concentrations of C and D decreased constantly after BERAD decontamination. On the other hand, the decontamination efficiency of A and B decreased as the soil particle became smaller, but the concentrations of A and B increased for the soil particle below 0.075 mm. As a result, decontamination efficiency of one cycle using BERAD for all nuclides in soil particles between 4 mm and 0.075 mm is about 45% to 65 %.
        131.
        2023.11 구독 인증기관·개인회원 무료
        The Korea Research Institute of Standards and Science has developed certified reference materials (concrete, soil, and metal radioactive liquid) for measuring gamma-emitting radionuclides to improve and maintain the quality assurance and quality control of the radioactivity measurement in decommissioning nuclear power plants. The raw materials that make up each CRM were mixed in an appropriate ratio with radionuclides. For certification and homogeneity assessment, 10 bottles were randomly selected, two sub-samples were collected from each bottle, and radionuclides were measured via HPGe gamma spectrometry. The results of the homogeneity tests using a one-way analysis of variance on the radionuclides in the CRMs fulfilled the requirements of ISO Guide 35. Coincidence summing and self-absorption correction were performed on measurement results by introducing the Monte Carlo efficiency transfer code and Monte Carlo N-Particle transport code. In concrete analysis, the reference values for five radionuclides (60Co, 241Am, 134Cs, and 137Cs) in the CRM were in the range of 15-40 Bq/kg, and the expanded uncertainty was within 10% (k = 2). In soil analysis, the reference values for the 137Cs and 60Co were 118.7 and 124.4 Bq/kg, and the expanded uncertainty was within 10% (k = 2). In metal radioactive liquid analysis, the reference values for 134Cs, 137Cs and 60Co in the CRM were in the range of 200-270 Bq/kg, and the expanded uncertainty was within 7% (k = 2).
        132.
        2023.11 구독 인증기관·개인회원 무료
        KORAD (Korea Radioactive Waste Agency, http://www.korad.or.kr) has stored slightly contaminated ascon (asphalt coated concrete mixture) that was introduced to Gyeongju repository about a decade ago waiting for a final disposal. It is believed to be mainly contaminated by radioisotope 137Cs due to impurities introduced from the outside during the ascon manufacturing process. We studied characteristics of the radioactive waste to see whether this material would be proper enough to be disposed in Gyeongju LILW repository or be other ways to reduce the disposal volume including self-disposal before its final disposal otherwise. KORAD looked into the properness of characteristics of ascon in terms of WAC (Waste Acceptance Criteria) documented by KORAD that includes general chemical and physical properties of asphalt, density, size of grains, content of organic material and possibility of existence of chelate materials that qualitatively limited to be disposed by the criteria. And other associated characteristics such as gas generation and bio degradation were also investigated. Based on the data obtained from the study, we proposed various plausible solutions in associated with operational and disposal safety and economic view points. This study will be used for KORAD’s decision on how to control and safely dispose the spent ascon within a reasonable time period. And also those experiences may be applied for other LILW issues that require treatment or conditioning of radioactive wastes in the future.
        133.
        2023.11 구독 인증기관·개인회원 무료
        The presence of organic components in spent scintillation liquid should be considered during all steps of radioactive waste processing for final disposal. Scintillation liquids often referred to as cocktails are generated form radiochemical analyses of radionuclides, which mainly consists of mixtures of liquid organic materials such as toluene and xylene. Typical features of these liquid organic materials are volatility, combustibility and toxicity. These are the reason why special attention must be paid to the management of liquid organic radioactive wastes. To select an appropriate waste management strategy and to design the treatment process of spent scintillation cocktails, it is required to investigate the nature of the waste such as specific radioactivity and moisture content. The analysis results of spent scintillation liquid generated at Wolsong nuclear power plants will be discussed. An overview of the technical approaches available for the treatment of organic radioactive waste will be additionally provided.
        134.
        2023.11 구독 인증기관·개인회원 무료
        Most of the radioactive wastes generated during the nuclear fuel processing activities conducted by KEPCO Nuclear Fuel Co., Ltd. are classified as the categories of intermediate and low-level radioactive waste. These radioactive waste materials are intended for permanent disposal at a designated disposal site, adhering strictly to the waste acceptance criteria. To facilitate the safe transportation of radioactive waste to the disposal site, it is necessary to ensure that the waste drums maintain a level of criticality that complies with the waste acceptance criteria. This necessitates the maintenance of subcritical conditions, under immersion or optimal neutron moderation conditions. This paper presents a criticality safety assessment of concrete radioactive waste under the most conservative conditions of immersion and moderation conditions for waste drums. Specifically, In order to send radioactive waste, which is the subject of criticality analysis, to a disposal facility, pre-processing operations must be performed to ensure compliance with waste accepatance criteria. To meet the physical characteristics required by the accepance criteria, particles below 0.2 mm should not be included. Thus, a 0.3 mm sieve is used to separate particles lager than 0.3 mm, and only those particles are placed in drums. The drums should be filled to achieve a filling ratio of at least 85%. A criticality analysis was conducted using the KENO-VI of SCALE. The Criticality Safety Analysis Results of varying the filling ratio of concrete drums from 85% to 100% presented in an effective multiplication factor of 0.22484. Additionally, the effective multiplication factor presented to be 0.25384 under the optimal moderation conditions. This demonstrates full compliance with the USL and criticality technology standards set as 0.95.
        135.
        2023.11 구독 인증기관·개인회원 무료
        Concentrated effluent and spent ion exchange resins (IERs) from nuclear power plants (NPPs) were generated prior to the establishment of a disposal facility site and waste acceptance criteria have been temporarily stored at the NPPs because their suitability for disposal has not been confirmed. In particular, at the Kori Unit 1, which was the first to start the commercial operation in South Korea, the initially generated concentrated effluent and IERs are repackaged in large size of concrete containers and stored without provided regulation standard. The concentrated effluent is package as cementitious form in 200 L drums and repackaged in concrete containers, case of the IERs were solidified or dehydrated and repackaged in round concrete container. In this study, we review and propose a disposal plan for concentrated effluent and IERs repackaging drums that have not been confirmed to be suitable for disposal from the first operating nuclear power plant, Kori Unit 1, 2. First, the concentrated effluent was stored in four 200 L drums respectively, and then, it was again stored in concrete container and which was poured on top using grouted concrete. Therefore, the process was required by cutting concrete container for extracting the internal drums at first. Internal radioactive waste should be crushed to the suitable waste criteria and solidified, finally disposal in to the polymer concrete high integrity container (PC-HIC). IER was repackaged and disposal in square type of 200 L concrete drums respectively covered the cap. So, extracting the internal drums should be extracted after removing the cap of external concrete container. Cement solidification drums can be crushed and re-solidified or disposed in the PC-HIC. Stored IER after dehydrated can be disposal in PC-HIC. In conclusion, the container was used as a package that repackaging the concentrated effluent and IER was separated into two different types of waste depending on the level of contamination of radioactivity, the polluted area is disposed of as radioactivity contamination or the unspoiled area will be treated as self-disposal waste.
        136.
        2023.11 구독 인증기관·개인회원 무료
        Radioactive waste is typically disposed of using standard 200 and 320 L drums based on acceptance criteria. However, there have been no cases evaluating the disposal and suitability of 200 L steel drums for RI waste disposal. There has been a lack of prior assessments regarding the disposal and suitability of 200 L steel drums for the disposal of RI waste. Radioactive waste is transported to disposal facilities after disposal in containers, where the drums are loaded and temporarily stored. Subsequently, after repackaging the disposal drums, the repackaged drums are transported to disposal facilities by vehicle or ship for permanent disposal. Disposal containers can be susceptible to damage due to impacts during transportation, handling, and loading, leading to potential damage to the radiation primer coating during loading. Additionally, disposal containers may be subject to damage from electrochemical corrosion, necessitating the enhancement of corrosion resistance. Metal composite coatings can be employed to enhance both abrasion resistance and corrosion resistance. The application of metal composite coatings to disposal containers can improve the durability and radiation shielding performance of radioactive waste disposal containers. The thickness of radioactive waste disposal containers is determined through radioactive shielding analysis during the design process. The designed disposal containers undergo structural analysis, considering loading conditions based on the disposal environment. This paper focuses on evaluating the structural improvements achieved through the implementation of metal composite coatings with the goal of enhancing corrosion and abrasion resistance.
        137.
        2023.11 구독 인증기관·개인회원 무료
        The bentonite buffer material is a crucial component for disposing of high-level radioactive waste (HLW). Several additives have been proposed to enhance the performance of bentonite buffer materials. In this study, unconfined compression tests were conducted on bentonite mixtures as well as pure bentonite buffer material. Joomunjin and silica sands were added at a 30% ratio, and graphite was added at 3% along with bentonite. The unconfined compression strength (UCS) and elastic modulus of pure bentonite were found to be 20% to 50% higher than those of bentonite mixtures under similar dry density and water content conditions. This decrease in strength can be attributed to the reduced cross-sectional area available for bearing the applied load in the bentonitemixture. Furthermore, the 3% graphite-bentonite mixture exhibited a 10% to 30% higher UCS and elastic modulus compared to the 30% sand-bentonite mixtures. However, since the strength properties of additive-bentonite mixtures are lower than those of pure bentonite, it is essential to evaluate thermohydraulic-mechanical functional criteria when considering the use of bentonite mixtures as buffer materials.
        138.
        2023.11 구독 인증기관·개인회원 무료
        The effect of various physicochemical processes, such as seawater intrusion, on the performance of the engineered barrier should be closely analyzed to precisely assess the safety of high-level radioactive waste repository. In order to evaluate the impact of such processes on the performance of the engineered barrier, a thermal-hydrological-chemical model was developed by using COMSOL Multiphysics and PHREEQC. The coupling of two software was achieved through the application of a sequential non-iterative approach. Model verification was executed through a comparative analysis between the outcomes derived from the developed model and those obtained in prior investigations. Two data were in a good agreement, demonstrating the model is capable of simulating aqueous speciation, adsorption, precipitation, and dissolution. Using the developed model, the geochemical evolution of bentonite buffer under a general condition was simulated as a base case. The model domain consists of 0.5 m of bentonite and 49.5 m of granite. The uraninite (UO2) was assigned at the canister-bentonite interface as the potential source of uranium. Assuming the lifetime of canister as 1,000 years, the porewater mixing without uranium leakage was simulated for 1,000 years. After then, the uranium leakage through the dissolution of uraninite was initiated and simulated for additional 1,000 years. In the base case model, where the porewater mixing between the bentonite and granite was the only considered process, the gypsum tended to dissolve throughout the bentonite, while it precipitated in the vicinity of bentonite-granite boundary. However, the precipitation and dissolution of gypsum only showed a limited effect on the performance of the bentonite. Due to the low solubility of uraninite in the reduced environment, only infinitesimal amounts of uranium dissolved and transported through the bentonite. Additional cases considering various environmental processes, such as seawater or cement porewater intrusion, will be further investigated.
        139.
        2023.11 구독 인증기관·개인회원 무료
        The operation time of a disposal repository is generally more than one hundred years except for the institutional control phase. The structural integrity of a repository can be regarded as one of the most important research issues from the perspective of a long-term performance assessment, which is closely related to the public acceptance with regard to the nuclear safety. The objective of this study is to suggest the methodology for quantitative evaluation of structural integrity in a nuclear waste repository based on the adaptive artificial intelligence (AI), fractal theory, and acoustic emission (AE) monitoring. Here, adaptive AI means that the advanced AI model trained additionally based on the expert’s decision, engineering & field scale tests, numerical studies etc. in addition to the lab. test. In the process of a methodology development, AE source location, wave attenuation, the maximum AE energy and crack type classification were subsequently studied from the various lab. tests and Mazars damage model. The developed methodology for structural integrity was also applied to engineering scale concrete block (1.3 m × 1.3 m × 1.3 m) by artificial crack generation using a plate jacking method (up to 30 MPa) in KURT (KAERI Underground Research Tunnel). The concrete recipe used in engineering scale test was same as that of Gyeongju low & intermediate level waste repository. From this study, the reliability for AE crack source location, crack type classification, and damage assessment increased and all the processes for the technology development were verified from the Korea Testing Laboratory (KTL) in 2022.
        140.
        2023.11 구독 인증기관·개인회원 무료
        In 2012, POSIVA selected a bentonite-based (montmorillonite) block/pellet as the backfilling solution for the deposition tunnel in the application for a construction license for the deep geological repository of high-level radioactive waste in Finland. However, in the license application (i.e. SC-OLA) for the operation submitted to the Finnish Government in 2021, the design for backfilling was changed to a granular mixture consisting of bentonite (smectite) pellets crushed to various sizes, based on NAGRA’s buffer solution. In this study, as part of the preliminary design of the deep geological repository system in Korea, we reviewed history and its rationale for the design change of Finland’s deposition tunnel backfilling solution. After the construction license was granted by the Finnish Government in 2015, POSIVA conducted various lab- and full-scale in-situ tests to evaluate the producibility and performance of two design alternatives (i.e. block/pellet type and granular type) for backfilling. Principal demonstration tests and their results are summarized as follows: (a) Manufacturing of blocks using three types of materials (Friedland, IBeco RWC, and MX-80): Cracking and jointing under higher pressing loads were found. Despite adjusting the pressing process, similar phenomena were observed. (b) 1:6 scale experiment: Confirmation of density difference inhomogeneity due to the swelling of block/pellet backfill and void filling due to swelling behavior into the mass loss area of block/pellet. (c) FISST (Full-Scale In situ system Test): Identification of technical unfeasibility due to the inefficient (too manual) installation process of blocks/pellets and development of an efficient granular in-situ backfilling solution to resolve the disadvantage. (d) LUCOEX-FE (Large Underground Concept Experiments – Full-scale Emplacement) experiment: Confirmation of dense/homogeneous constructability and performance of granular backfilling solution. In conclusion, the simplified granular backfill system is more feasible compared to the block/ pellet system from the perspective of handling, production, installation, performance, and quality control. It is presumed that various experimental and engineering researches should be preceded reflecting specific disposal conditions even though these results are expected to be applied as key data and/or insights for selecting the backfilling solution in the domestic deep geological repository.