The Korea Atomic Energy Research Institute (KAERI) has facilities that are operated for the purpose of treating radioactive wastes and storing drums before sending them to a disposal site. Domestic regulations related to nuclear facility require radiological dose assessment resulting from release of gaseous radioactive effluent of nuclear facilities. In this study, ICRP-60-based dose conversion factors were applied to evaluate the radiation dose to residents in the event of operation and accident for the radioactive waste management facilities in KAERI. The radioactive gaseous effluent generated from each facility diffuse outside the exclusion area boundary (EAB), causing radiation exposure to residents. To evaluate the external exposure dose, the exposure pathways of cloudshine and radioactive contaminated soil were analyzed. The internal exposure dose was estimated by considering the exposure from respiration and ingestion of agricultural and livestock products. The maximum individual exposure dose was evaluated to be 1.71% compared to the dose limit. The assumed situation used for accidental scenarios are as follows; A fire inside the facility and falling of radioactive waste drum. It was a fire accident that caused the maximum exposure dose to individual and population living within an 80 km radius of the site. At the outer boundary of the low population zone (LPZ), the maximum effective dose and thyroid equivalent dose were estimated as 8.92 E-06% and 5.29 E-06%, respectively, compared to the dose limit. As a result of evaluating the radiological exposure dose from gaseous emissions, the radioactive waste treatment facilities and its supplementary facilities meet the regulations related to nuclear facility, and are operated safely in terms of radiological environmental impact assessment.
To construct and operate nuclear power plants (NPPs), it is mandatory to submit a radiation environmental impact assessment report in accordance with Article 10 and Article 20 of the Nuclear Safety Act. Additionally, in compliance with Article 136 of the Enforcement Regulations of the same law, KHNP (Korea Hydro & Nuclear Power) annually assesses radiation environmental effects and publishes the results for operating NPPs. Furthermore, since the legalization of emission plans submission in 2015, KHNP has been submitting emission plans for individual NPPs, starting with the Shin-Hanul 1 and 2 units in 2018. These emission plans specify the emission quantities that meet the dose criteria specified by the Nuclear Safety and Security Commission. Before 2002, KHNP used programs developed in the United States, such as GASPAR and LADTAP, for nearby radiation environmental impact assessments. Since then, KHNP has been using K-DOSE60, developed internally. K-DOSE60 incorporates environmental transport analysis models in line with U.S. regulatory guidance Regulatory Guide 1.109 and dose assessment models reflecting ICRP-60 recommendations. K-DOSE60 is a stand-alone program installed on individual user PCs, making it difficult to manage comprehensively when program revisions are needed. Additionally, during the preparation of emission plans and the licensing phase, improvements to KDOSE60’ s dose assessment methodology were identified. Furthermore, in 2022, regulatory guidelines regarding resident dose assessments were revised, leading to additional improvement requirements. Currently, E-DOSE60, being developed by KHNP, is a network-based program allowing for integrated configuration management within the KHNP network. E-DOSE60 is expected to be developed while incorporating the identified improvements from K-DOSE60, in response to emission plan licensing and regulatory guideline revisions. Key improvements include revisions to dose assessment methodologies for H-13 and C-14 following IAEA TRS-472, expansion of dose assessment points, and changes in socio-environmental factors. Furthermore, data such as site meteorological information and releases of radioactive substances in liquid and gaseous forms can be linked through a network, reducing the potential for human errors caused by manual data entry. Ultimately, E-DOSE60 is expected to optimize resident exposure dose assessment and enhance public trust in NPP operation.
For the release of the nuclear power plant site after the decommissioning, a reliable exposure dose assessment considering the environmental impact of residual radionuclides is essentially required. In this study, the Derived Concentration Guideline Level (DCGL) for the hypothetically contaminated surface soil at the Wolsong nuclear power plant (NPP) unit 1 site was preliminarily calculated by using the RESRAD-OFFSITE computational code and compared with the other case studies. Moreover, radiation exposure dose for local residents and relevant exposure pathways were quantitatively analyzed based on the calculation model established through this work. For the target site modeling, the source term was determined by referring to the previous case studies regarding the nuclear power plant decommissioning, quantification analysis data of pressure tubes of Wolsong NPP unit 1, and radionuclide data estimated by using the MCNP/ORIGEN-2 code. In total, 14 different radioisotopes such as Ag-108m, C-14, Co-60, Cs-134/137, Fe-55, H-3, Nb-93m/94, Ni-63, Sb-125, Sn-121m, Sr-90, and Zr-93 were considered as target radionuclides. In addition, the geological structure model of the Wolsong NPP site was established based on the final safety analysis report of Wolsong NPP unit 1. The distribution coefficients (Kd) were taken from the JAEA-SDB to estimate the migration/retardation behavior of various radionuclides under the groundwater condition of the Wolsong NPP site. In the present work, the DCGL values were calculated according to the site release criterion of 0.1 mSv/yr, which indicates the radiation protection standard for the site release. Moreover, the exposure pathway and sensitivity analyses were conducted to assess the sensitive input parameters remarkably influencing the calculation result. For the evaluation of exposure dose for local residents, a site layout centered around Wolsong NPP unit 4, located in the closest proximity to the residents’ habitation area, was alternatively established and all potential exposure pathways were considered as a comprehensive resident farmer scenario. The results obtained from this study are expected to serve as a preliminary case study for the DCGL values regarding the surface soil at the Wolsong NPP unit 1 site and for evaluating the radiation exposure dose to local residents resulting from the residual radioactivity at the site after the decommissioning.
The decommissioning of Korea Research Reactor Units 1 and 2 (KRR 1&2), the first research reactors in South Korea, began in 1997 and the decommissioning status is currently proceeding with phase 3. It is expected that more than 5,000 tons of dismantled wastes will be generated as the contaminated building is demolished. Since these dismantled wastes must be disposed of in an efficient method considering economic feasibility, it is desirable to clearance extremely low-level wastes whose contamination is so minimal that the radiological risk is negligible. In Korea, in order to approve the clearance of radioactive waste, it must be proven that the nuclide concentration standards are met or that the dose to individuals and collectives is below the allowable dose value. At the KRR 1&2 decommissioning site, dismantled wastes have been steadily being disposed of through clearance procedure since 2021. Clearance was approved by the Korean Institute of Nuclear Safety (KINS) for one case of concrete waste in 2021 and two cases of metal waste in 2022. In 2023, the clearance of metal waste and asbestos waste has been approved so far, and in particular, this is the first case in Korea for asbestos waste. In this study, we compared the dose assessment methods and results of clearance wastes at the KRR 1&2 decommissioning site from 2021 to present. Dose assessment was conducted by applying the landfill scenario for concrete and asbestos and the recycling scenario for metal waste. The calculation codes used were RESRAD-onsite 7.2 and RESRAD-recycle 3.10. The dose conversion factors (DCF) for each age group (infant, 1y, 5y, 10y, 15y, adult) of the target nuclide used the values presented in ICRP-72, and in particular, geo-hydrological data of the actual landfill site was used as an input factor when evaluating landfill scenarios. As a result of the dose assessment, when landfilling concrete wastes in 2020, the personal dose and collective dose were evaluated the most at 2.80E+00 μSv/y and 4.83E-02 man·Sv/y, respectively.
The Korea Atomic Energy Research Institute (KAERI) is currently developing a process-based performance assessment model known as APro. Distinguished from the previous system-level safety assessment model developed by KAERI, APro exhibits the capacity to encompass a threedimensional biosphere domain, evolving over the long term. In this study, we elucidate the methodology employed in developing the dose assessment module of APro and present the module’s functionalities. The procedural steps underlying radiation dose calculations within the APro framework can be succinctly outlined as follows: 1) Definition of a landscape model, utilizing information derived from a specified snapshot period provided by the APro biosphere transport module; 2) Generation of unit biotope objects spanning the landscape; 3) Evaluation of radionuclide transfer within the soil medium; 4) Calculation of activity concentration for flora and fauna groups; 5) Assessment of the distribution of effective dose among representative human groups; 6) Progressing through successive time steps. The APro dose calculation module exhibits notable capabilities that encompass: 1) Accounting for radionuclide decay and ingrowth; 2) Facilitating transfer through unsaturated porous media; 3) Considering sorption effects; 4) Addressing the inheritance of radioactivity between various landscape models; 5) Offering customizable ecosystem parameters; 6) Providing flexibility for user-defined exposure pathways. Leveraging these functionalities of the dose assessment module, APro is proficient in evaluating the distribution of radiological doses and associated risks for representative population groups, all while accounting for the dynamic, long-term evolution of the biosphere, including alterations in land cover.
Collagen peptides have garnered significant attention as functional foods across multiple fields due to their capacity to regulate physiological and hormonal processes, offering numerous advantages. However, despite their broad range of applications, comprehensive research on the potential toxicity of these substances remains lacking. Therefore, this study sought to assess the acute oral toxicity of a collagen peptide derived from skate (Raja kenojei) skin (CPSS) in both rats and dogs. In the rat model, CPSS was orally administered at doses of 300 and 2,000 mg/kg to Sprague-Dawley rats. An escalating single-dose oral toxicity assessment at doses of 500, 1,000, and 2,000 mg/kg was carried out in beagle dogs with 3-day intervals between doses. Throughout the 14-day post-administration assessment period, clinical signs, mortality rates, changes in body weight, and necropsy observations were closely monitored. After oral administration, no signs of toxicity associated with CPSS were observed in either rats or dogs. Therefore, the oral LD50 (approximate lethal dose for 50% mortality) for CPSS in rats was determined to exceed 5,000 mg/kg, and the maximum tolerated dose for dogs was estimated to be above 2,000 mg/kg. Consequently, this study offers safety data on the use of CPSS in functional foods and medicinal applications.
In this research, the dose rate was measured using a backpack-type scan survey device at 4 sites in sites around Nuclear Power Plants (Kori, Wolsong, Hanbit, Hanul), and the radioactivity ratio for each nuclide was evaluated using an high-purity germanium (HPGe) detector. Kori, Wolsong and Hanul power plants were measured within 2 km of the power plant, and Hanbit power plants were measured about 6.7 km from the power plant. As a result of measuring the dose rate with a backpacktype scan survey device, the average dose rate was the lowest in the measurement site 1 at 0.090 μSv/h, and the highest in the measurement site 4 at 0.145 μSv/h. All measurement points showed the domestic environmental dose rate level. The data obtained by the scan survey was visualized using the classed post and gridding functions of the surfer program. As a result of measurement with the HPGe detector, 137Cs was not detected, and only natural nuclides were detected. Among the detected natural nuclides, the radioactivity ratio was the highest for 40K with an average of 94.56%, and the lowest for 214Pb with an average of 0.26%. The results of this research can be used as basic data for radiation environment surveys around nuclear power plants. Further studies are needed to evaluate the radiation impacts by region and environment through periodic measurements.
KHNP is carrying out international technical cooperation and joint research projects to decommission Wolsong unit 1 reactor. Construction data of the reactor structures, experience data on the pressure tube replacement projects, and the operation history were reviewed, and the amount of dismantled waste was calculated and waste was classified through activation analysis. By reviewing COG (CANDU owners Group) technical cooperation and experience in refurbishment projects, KHNP’s unique Wolsong unit 1 reactor decommissioning process was established, and basic design of a number of decommissioning equipment was carried out. Based on this, a study is being conducted to estimate the worker dose of dismantling workers. In order to evaluate the dose of external exposure of dismantling workers, detailed preparation and dismantling processes and radiation field evaluation of activated structures are required. The preparation process can be divided into dismantlement of existing facilities that interfere with the reactor dismantling work and construction of various facilities for the dismantlement process. Through process details, the work time, manpower, and location required for each process will be calculated. Radiation field evaluation takes into account changes in the shape of structures by process and calculates millions of areas by process, so integrated scripts are developed and utilized to integrate input text data. If the radiation field evaluation confirms that the radiation risk of workers is high, mutual feedback will be exchanged so that the process can be improved, such as the installation of temporary shields. The results of this study will be used as basic data for the final decommissioning plan for Wolsong unit 1. By reasonably estimating the dose of workers through computer analysis, safety will be the top priority when decommissioning.
RUCAS (Recycling-Underlying Computational Dose Assessment System), a dose assessment program based on the RESRAD-RECYCLE framework, is designed to evaluate dose for recycling scenarios of radioactive waste in metals and concrete. To confirm the validity of the recycling scenarios provided by RUCAS, comparative evaluations will be conducted with RESRAD-RECYCLE for metal radioactive waste recycling scenarios and with MicroShield® for concrete radioactive waste recycling scenarios. In the evaluation of metal recycling scenarios without shielding, RUCAS showed similar results when compared to both MicroShield® and RESRAD-RECYCLE. This validates the function of dose assessments using RUCAS for metal recycling scenarios. However, when shielding was present, RUCAS produced results that were comparable to MicroShield®, but differed from those of RESRAD-RECYCLE. The underestimation of dose values up to 1.66E+08 times difference by RESRAD-RECYCLE could potentially decrease reliability and safety in evaluated doses, further emphasizing the importance of RUCAS. Because validation is also necessary for the expanded calculation capabilities resulting from methodological changes of RUCAS (i.e., various radiation source geometries), based on prior validations, it was determined that additional validations are required for different radiation source materials and shielding conditions. In case where the radiation source and shielding materials were identical, RUCAS and MicroShield® produced similar results according to both the Kalos et al. (1974) and Lin and Jiang (1996) methodologies. This demonstrates that the that differences in methodology are inconsequential when considering the same source and shielding materials. However, when the atomic number of the radiation source materials was larger than that of shielding material (HZ-LZ condition), RUCAS obtained results similar to MicroShield® only for the Kalos et al. (1974) methodology. While Lin and Jiang (1996) methodology yield higher results than MicroShield®. Lastly, in case where the atomic number of the radiation source material was smaller than that of the shielding material (LZ-HZ condition,) both methodologies yielded results comparable to MicroShield®. In conclusion, the validity of RUCAS’s shielding calculations has been verified, confirming improvements in dose assessment compared to RESRAD-RECYCLE. Additionally, we observed that shielding effectiveness calculations differ depending on the methodology of build-up effect. If the validity of these methodologies is confirmed, it is expected that selecting the most advantageous methodology for each condition will enable more rational dose assessments. Consequently, in future research, we plan to evaluate the validity of Lin and Jiang (1996) methodology using particle transport codes based on the Monte Carlo method, such as MCNP and Geant 4, rather than MicroShield®.
The Korean Nuclear Safety and Security Commission has established a general guideline for the disposal of high-level waste, which requires that radiological effects from a disposal facility should not exceed the regulatory safety indicator, a radiological risk. The post-closure safety assessment of the disposal facility aims to evaluate the radiological dose against a representative person, taking into account nuclide transport and exposure pathways and their corresponding probabilities. The biosphere is a critical component of radiation protection in a disposal system, and the biosphere model is concerned with nuclide transport through the surface medium and the doses to human beings due to the contaminated surface environment. In past studies by the Korea Atomic Energy Research Institute (KAERI), the biosphere model was constructed using a representative illustration of surface topographies and groundwater conditions, assuming that the representative surface environment would not change in the future. Each topography was conceptualized as a single compartment, and distributed surface contamination over the geometrical domain was abstracted into 0D. As a result, the existing biosphere model had limitations, such as a lack of quantitative descriptions of various transport and exposure pathways, and an inability to consider the evolution of the surface environment over time. These limitations hinder the accurate evaluation of radiological dose in the safety assessment. To overcome these limitations, recent developments in biosphere modeling have incorporated the nuclide transport process over a 2D or 3D domain, integrating the time-dependent evolution of the surface environment. In this study, we reviewed the methodology for biosphere modeling to assess the radiological dose given by distributed surface contamination over a 2D domain. Based on this review, we discussed the model requirements for a numerical module for biosphere dose assessment that will be implemented in the APro platform, a performance assessment tool being developed by the KAERI. Finally, we proposed a conceptual model for the numerical module of dose assessment.
n this research, the dose rate was measured using backpack-type scan survey device at 4 sites on Jeju Island, and the radioactivity ratio for each nuclide was evaluated using an high-purity germanium (HPGe) detector. As a result of measuring the dose rate with a backpack-type scan survey device, the average dose rate was the lowest in the measurement site 3 at 0.049 Sv/h, and the highest in the measurement site 1 at 0.066 Sv/h. The average dose rate of the 4 sites on Jeju Island was 0.056 Sv/h, and the dose rate on Jeju Island was lower than that of other regions. The data acquired by scan survey were interpreted using classed post and gridding function of surfer program. The radioactivity ratio of each nuclide in the gamma spectrum measured by the HPGe detector was the highest for K-40 with an average of 87.62%, and the lowest for Pb-214 with an average of 0.63%. In the case of the Jeju Island site, Cs-137 was detected, and the average radioactivity ratio of Cs-137 was 3.27%, which was the background level. The results of this research can be used as basic data on the radioactivity ratio for each nuclide and dose rate at the Jeju Island site. Further studies on the assessment of dose rates and radioactivity ratios in other regions are needed.
The IAEA recommended considerations for exemption regulations of consumer products containing greater amounts of radioactive isotopes than the amounts specified for generic exemption. One of the major considerations is the expected exposure dose should be less than 10 μSv/y and 1 mSv/y for general cases and low probability cases, respectively, in all predictable scenarios. Under this recommendation, many countries evaluated the radiation dose for exposure scenarios of various products in consideration of the national circumstances and, then, established their own specific exemption regulation. In Republic of Korea, the “Regulation on substances excluded from radioactive isotopes” was legislated to specify consumer products excluded from regulation. However, as the usage status and product specifications has changed over time, it is necessary to periodically verify the validity of the regulation criteria in the view of exemption justification. In this study, we developed the use and disposal scenarios in consideration of the domestic use of thorium-containing gas mantle and evaluated radiation dose of each scenario accordingly. The gas mantles are used as a wick for gas lanterns and the maximum activity of natural thorium contained among the currently available gas mantles is 12.5 kBq. Radioactive isotopes in the decay chain of natural thorium can be divided into three groups according to their physical characteristics, and exposure routes suitable for each group were considered in dose calculation. Currently, most gas mantles are installed in camping lanterns. Therefore, we developed use scenarios related to camping. The average number of camping trips and time spent at the campground were set by the data from Korea Tourism Organization. Tent sizes and vehicle specifications were determined by referring to surveys and products in Korea. The used gas mantle is disposed of in a garbage bag for general waste and transported to landfill or incinerator. We determined the amount of gas mantle discarded in landfill and incinerator by the data from Korea Environment Corporation. The exposure time and amount handled by an individual were determined by considering the number of waste collection vehicles, landfills, and incinerators. Although we assumed the maximum activity of the gas mantle for conservative evaluation, the calculated radiation doses for the use and disposal scenarios were below the general requirement (i.e., 10 μSv/y) in all scenarios.
In Korea, it is expected that the decommissioning of nuclear reactors will increase due to the license termination of reactors constructed in the 1960s to the 80s. According to the investigation of KORAD, VLLW accounts for 67.10% of decommissioning wastes and amounts to about 413,336 drums. Due to their huge amount, it is necessary to create an appropriate decommissioning waste management plan even though VLLW is disposed at the second-phase disposal facility of the Gyeongju repository. For efficient reduction in decommissioning wastes, it is required to actively use a clearance of metallic and concrete radioactive wastes. Regulations of nuclear safety and security commission notice that the radioactive waste can be reused or recycled if it meets the clearance criterion, 10 μSv·y−1 for individual dose. Therefore, it is important to develop a computational code which calculate individual doses for each scenario, and determine whether the clearance criterion is satisfied. However, in the case of metallic waste, RESRAD-RECYCLE used in dose assessment for the clearance has no longer been maintained or updated since 2005 and there is no code for recycling of concrete waste. For this reason, a dose assessment code RUCAS (Recycle-Underlying Computational dose Assessment System) has been developed by Ulsan National Institute of Science and Technology (UNIST). A point kernel method is adopted into external dose assessment model to calculate more realistic options, which are various geometries of source, and shielding effect. In the case of internal radiation, equations of internal dose from IAEA are used. This research conducts a verification of dose assessment model for recycling of metallic radioactive waste. RESRAD-RECYCLE is the comparison object and results from RESRAD-RECYCLE validation report are referenced. Targets are 14 recycling scenarios composed up to the smelting metal step of four steps, which are arising scrap metal, smelting scrap metal, and fabrication of metal product, and reusing/recycling of product. Seven isotopes, which are Ac-227, Am-241, Co-60, Cs-137, Pu-239, Sr- 90, and Zn-65, are selected for calculation. Validation results for external dose vary by isotopes, but show acceptable differences. It seems to be caused by difference in the calculation method. In the case of internal dose using same calculation formula, results are exactly matched to RESRAD-RECYCLE for all isotopes. Consequently, RUCAS can conduct functions supported by RESRAD-RECYCLE well and future work will be conducted related to domestic recycling scenarios considering public acceptance, and verification with radiation shielding codes for various geometries of source.